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Register a new userOn the Influence of Delay Line Uncertainty in THz Time-Domain Spectroscopy
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Terahertz time-domain spectroscopy (THz TDS) is a well-known tool for material analysis in the terahertz frequency band. One crucial system component in every time-domain spectrometer is the delay line which is necessary to accomplish the sampling of the electric field over time. Despite the fact that most of the uncertainty sources in TDS have been discussed, the delay line uncertainty has not been considered in detail. We model the impact of delay line uncertainty on the acquired THz TDS data. Interferometric measurements of the delay line precision and THz time-domain data are used to validate the theoretical model.
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An optical buffer having a large delay-bandwidth-product -- a critical component for future all-optical communications networks -- remains elusive. Central to its realization is a controllable inline optical delay line, previously accomplished via engineered dispersion in optical materials or photonic structures constrained by a low delay-bandwidth product. Here we show that space-time wave packets whose group velocity in free space is continuously tunable provide a versatile platform for constructing inline optical delay lines. By spatio-temporal spectral-phase-modulation, wave packets in the same or in different spectral windows that initially overlap in space and time subsequently separate by multiple pulse widths upon free propagation by virtue of their different group velocities. Delay-bandwidth products of ~100 for pulses of width ~1 ps are observed, with no fundamental limit on the system bandwidth.
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We report on the group delay observed in continuous-wave terahertz spectroscopy based on photomixing with phase-sensitive homodyne detection. We discuss the different contributions of the experimental setup to the phase difference Deltaphi( u) between transmitter arm and receiver arm. A simple model based on three contributions yields a quantitative description of the overall behavior of Deltaphi( u). Firstly, the optical path-length difference gives rise to a term linear in frequency. Secondly, the ultra-wideband log-spiral antennae effectively radiate and receive in a frequency-dependent active region, which in the most simple model is an annular area with a circumference equal to the wavelength. The corresponding term changes by roughly 6 pi between 100 GHz and 1 THz. The third contribution stems from the photomixer impedance. In contrast, the derivative (dDeltaphi / d u) is dominated by the contribution of periodic modulations of Deltaphi( u) caused by standing waves, e.g., in the photomixers Si lenses. Furthermore, we discuss the Fourier-transformed spectra, which are equivalent to the waveform in a time-domain experiment. In the time domain, the group delay introduced by the log-spiral antennae gives rise to strongly chirped signals, in which low frequencies are delayed. Correcting for the contributions of antennae and photomixers yields sharp peaks or pulses and thus facilitates a time-domain-like analysis of our continuous-wave data.
We report a broadband terahertz time-domain spectroscopy (THz-TDS) which enables twenty vibrational modes of adenosine nucleoside to be resolved in a wide frequency range of 1-20 THz. The observed spectroscopic features of adenosine are in good agreement with the published spectra obtained using Fourier Transform Infrared Spectroscopy (FTIR) and Raman spectroscopy. This much-extended bandwidth leads to enhanced material characterization capability as it provides spectroscopic information on both intra-molecular and inter-molecular vibrations. In addition, we also report a low-cost Frequency Modulation Continuous Wave (FMCW) imaging system which has a fast measurement speed of 40,000 waveforms per second. Cross-sectional imaging capability through cardboard has also been demonstrated using its excellent penetration capability at a frequency range of 76-81 GHz. We anticipate that the integration of these two complementary imaging technologies would be highly desirable for many real-world applications because it provides both spectroscopic discrimination and penetration capabilities in a single instrument.
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