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Fission fragment distributions and their impact on the r-process nucleosynthesis in neutron star mergers

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 Publication date 2021
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and research's language is English




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Neutron star (NS) merger ejecta offer a viable site for the production of heavy r-process elements with nuclear mass numbers A >140. The crucial role of fission recycling is responsible for the robustness of this site against many astrophysical uncertainties. Here, we introduce new improvements to our scission-point model, called SPY, to derive the fission fragment distribution for all neutron-rich fissioning nuclei of relevance in r-process calculations. These improvements include a phenomenological modification of the scission distance and a smoothing procedure of the distribution. Such corrections lead to a much better agreement with experimental fission yields. Those yields are also used to estimate the number of neutrons emitted by the excited fragments on the basis of different neutron evaporation models. Our new fission yields are extensively compared to those predicted by the so-called GEF model. The impact of fission on the r-process nucleosynthesis in binary neutron mergers is also reanalyzed. Two scenarios are considered, the first one with low initial electron fraction is subject to intense fission recycling, in contrast to the second one which includes weak interactions on nucleons. The various regions of the nuclear chart responsible for fission recycling during the neutron irradiation as well as after freeze-out are discussed. The contribution fission processes may have to the final abundance distribution is also studied in detail in the light of newly defined quantitative indicators describing the fission recycling, the fission seeds and the fission progenitors. In particular, those allow us to estimate the contribution of fission to the final abundance distribution stemming from specific heavy nuclei. Calculations obtained with SPY and GEF fission fragment distributions are compared for both r-process scenarios.



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Comparing observational abundance features with nucleosynthesis predictions of stellar evolution or explosion simulations can scrutinize two aspects: (a) the conditions in the astrophysical production site and (b) the quality of the nuclear physics input utilized. We test the abundance features of r-process nucleosynthesis calculations for the dynamical ejecta of neutron star merger simulations based on three different nuclear mass models: The Finite Range Droplet Model (FRDM), the (quenched version of the) Extended Thomas Fermi Model with Strutinsky Integral (ETFSI-Q), and the Hartree-Fock-Bogoliubov (HFB) mass model. We make use of corresponding fission barrier heights and compare the impact of four different fission fragment distribution models on the final r-process abundance distribution. In particular, we explore the abundance distribution in the second r-process peak and the rare-earth sub-peak as a function of mass models and fission fragment distributions, as well as the origin of a shift in the third r-process peak position. The latter has been noticed in a number of merger nucleosynthesis predictions. We show that the shift occurs during the r-process freeze-out when neutron captures and {beta}-decays compete and an (n,{gamma})-({gamma},n) equilibrium is not maintained anymore. During this phase neutrons originate mainly from fission of material above A = 240. We also investigate the role of {beta}-decay half-lives from recent theoretical advances, which lead either to a smaller amount of fissioning nuclei during freeze-out or a faster (and thus earlier) release of fission neutrons, which can (partially) prevent this shift and has an impact on the second and rare-earth peak as well.
Simulations of r-process nucleosynthesis require nuclear physics information for thousands of neutron-rich nuclear species from the line of stability to the neutron drip line. While arguably the most important pieces of nuclear data for the r-process are the masses and beta decay rates, individual neutron capture rates can also be of key importance in setting the final r-process abundance pattern. Here we consider the influence of neutron capture rates in forming the A~80 and rare earth peaks.
146 - Stephane Goriely , 2011
Although the rapid neutron-capture process, or r-process, is fundamentally important for explaining the origin of approximately half of the stable nuclei with A > 60, the astrophysical site of this process has not been identified yet. Here we study r-process nucleosynthesis in material that is dynamically ejected by tidal and pressure forces during the merging of binary neutron stars (NSs) and within milliseconds afterwards. For the first time we make use of relativistic hydrodynamical simulations of such events, defining consistently the conditions that determine the nucleosynthesis, i.e., neutron enrichment, entropy, early density evolution and thus expansion timescale, and ejecta mass. We find that 10^{-3}-10^{-2} solar masses are ejected, which is enough for mergers to be the main source of heavy (A > 140) galactic r-nuclei for merger rates of some 10^{-5} per year. While asymmetric mergers eject 2-3 times more mass than symmetric ones, the exact amount depends weakly on whether the NSs have radii of ~15 km for a stiff nuclear equation of state (EOS) or ~12 km for a soft EOS. R-process nucleosynthesis during the decompression becomes largely insensitive to the detailed conditions because of efficient fission recycling, producing a composition that closely follows the solar r-abundance distribution for nuclei with mass numbers A > 140. Estimating the light curve powered by the radioactive decay heating of r-process nuclei with an approximative model, we expect high emission in the B-V-R bands for 1-2 days with potentially observable longer duration in the case of asymmetric mergers because of the larger ejecta mass.
314 - A.E. Lovell , P. Talou , I. Stetcu 2020
Several sources of angular anisotropy for fission fragments and prompt neutrons have been studied in neutron-induced fission reactions. These include kinematic recoils of the target from the incident neutron beam and the fragments from the emission of the prompt neutrons, preferential directions of the emission of the fission fragments with respect to the beam axis due to the population of particular transition states at the fission barrier, and forward-peaked angular distributions of pre-equilibrium neutrons which are emitted before the formation of a compound nucleus. In addition, there are several potential sources of angular anisotropies that are more difficult to disentangle: the angular distributions of prompt neutrons from fully accelerated fragments or from scission neutrons, and the emission of neutrons from fission fragments that are not fully accelerated. In this work, we study the effects of the first group of anisotropy sources, particularly exploring the correlations between the fission fragment anisotropy and the resulting neutron anisotropy. While kinematic effects were already accounted for in our Hauser-Feshbach Monte Carlo code, $mathtt{CGMF}$, anisotropic angular distributions for the fission fragments and pre-equilibrium neutrons resulting from neutron-induced fission on $^{233,234,235,238}$U, $^{239,241}$Pu, and $^{237}$Np have been introduced for the first time. The effects of these sources of anisotropy are examined over a range of incident neutron energies, from thermal to 20 MeV, and compared to experimental data from the Chi-Nu liquid scintillator array. The anisotropy of the fission fragments is reflected in the anisotropy of the prompt neutrons, especially as the outgoing energy of the prompt neutrons increases, allowing for an extraction of the fission fragment anisotropy to be made from a measurement of the neutrons.
$textbf{Background}$ More than half of all the elements heavier than iron are made by the rapid neutron capture process (or r process). For very neutron-rich astrophysical conditions, such at those found in the tidal ejecta of neutron stars, nuclear fission determines the r-process endpoint, and the fission fragment yields shape the final abundances of $110le A le 170$ nuclei. The knowledge of fission fragment yields of hundreds of nuclei inhabiting very neutron-rich regions of the nuclear landscape is thus crucial for the modeling of heavy-element nucleosynthesis. $textbf{Purpose}$ In this study, we propose a model for the fast calculation of fission fragment yields based on the concept of shell-stabilized prefragments defined with help of the nucleonic localization functions. $textbf{Methods}$ To generate realistic potential energy surfaces and nucleonic localizations, we apply Skyrme Density Functional Theory. The distribution of the neck nucleons among the two prefragments is obtained by means of a statistical model. $textbf{Results}$ We benchmark the method by studying the fission yields of $^{178}$Pt, $^{240}$Pu, $^{254}$Cf, and $^{254,256,258}$Fm and show that it satisfactorily explains the experimental data. We then make predictions for $^{254}$Pu and $^{290}$Fm as two representative cases of fissioning nuclei that are expected to significantly contribute during the r-process nucleosynthesis occurring in neutron star mergers. $textbf{Conclusions}$ The proposed framework provides an efficient alternative to microscopic approaches based on the evolution of the system in a space of collective coordinates all the way to scission. It can be used to carry out global calculations of fission fragment distributions across the r-process region.
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