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Register a new userTopological magnons for thermal Hall transport in frustrated magnets with bond-dependent interactions
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Thermal transport in topologically-ordered phases of matter provides valuable insights as it can detect the charge-neutral quasiparticles that would not directly couple to electromagnetic probes. An important example is edge heat transport of Majorana fermions in a chiral spin liquid, which leads to a half-quantized thermal Hall conductivity. This signature is precisely what has recently been measured in $alpha$-RuCl$_3$ under external magnetic fields. The plateau-like behavior of the half-quantized thermal Hall conductivity as a function of external magnetic field, and the peculiar sign change depending on the magnetic field orientation, has been proposed as strong evidence for the non-Abelian Kitaev spin liquid. Alternatively, for in-plane magnetic fields, it was theoretically shown that such a sign structure can also arise from topological magnons in the field-polarized state. In this work, we investigate the full implications of topological magnons as heat carriers on thermal transport measurements. We first prove analytically that for any commensurate order with a finite magnetic unit cell, reversing the field direction leads to a sign change in the magnon thermal Hall conductivity in two-dimensional systems. We verify this proof numerically with nontrivial magnetic orders as well as the field-polarized state in Kitaev magnets subjected to an in-plane field. In the case of a tilted magnetic field, whereby there exist both finite in-plane and out-of-plane field components, we find that the plateau-like behavior of the thermal Hall conductivity and the sign change upon reversing the in-plane component of the magnetic field arise in the partially-polarized state, as long as the in-plane field contribution to the Zeeman energy is significant. While these results are consistent with the experimental observations, we comment on other aspects requiring investigation in future studies.
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Recently, the observation of large thermal Hall conductivities in correlated insulators with no apparent broken symmetry have generated immense interest and debates on the underlying ground states. Here, considering frustrated magnets with bond-dependent interactions, which are realized in the so-called Kitaev materials, we theoretically demonstrate that a large thermal Hall conductivity can originate from a classical ground state without any magnetic order. We discover a novel liquid state of magnetic vortices, which are inhomogeneous spin textures embedded in the background of polarized spins, under out-of-plane magnetic fields. In the classical regime, different configurations of vortices form a degenerate manifold. We study the static and dynamical properties of the magnetic vortex liquid state at zero and finite temperatures. In particular, we show that the spin excitation spectrum resembles a continuum of nearly flat Chern bands, which ultimately leads to a large thermal Hall conductivity. Possible connections to experiments are discussed.
We study periodically driven pure Kitaev model and ferromagnetic phase of the Kitaev-Heisenberg model on the honeycomb lattice by off-resonant linearly and circularly-polarized lights at zero magnetic field. Using a combination of linear spin wave and Floquet theories, we show that the effective time-independent Hamiltonians in the off-resonant regime map onto the corresponding anisotropic static spin model, plus a tunable photoinduced magnetic field along the $[111]$ direction, which precipitates Floquet topological magnons and chiral magnon edge modes. They are tunable by the light amplitude and polarization. Similarly, we show that the thermal Hall effect induced by the Berry curvature of the Floquet topological magnons can also be tuned by the laser field. Our results pave the way for ultrafast manipulation of topological magnons in irradiated Kitaev magnets, and could play a pivotal role in the investigation of ultrafast magnon spin current generation in Kitaev materials.
In the field of quantum magnetism, the advent of numerous spin-orbit assisted Mott insulating compounds, such as the family of Kitaev materials, has led to a growing interest in studying general spin models with non-diagonal interactions that do not retain the SU(2) invariance of the underlying spin degrees of freedom. However, the exchange frustration arising from these non-diagonal and often bond-directional interactions for two- and three-dimensional lattice geometries poses a serious challenge for numerical many-body simulation techniques. In this paper, we present an extended formulation of the pseudo-fermion functional renormalization group that is capable of capturing the physics of frustrated quantum magnets with generic (diagonal and off-diagonal) two-spin interaction terms. Based on a careful symmetry analysis of the underlying flow equations, we reveal that the computational complexity grows only moderately, as compared to models with only diagonal interaction terms. We apply the formalism to a kagome antiferromagnet which is augmented by general in-plane and out-of-plane Dzyaloshinskii-Moriya (DM) interactions, as argued to be present in the spin liquid candidate material herbertsmithite. We calculate the complete ground state phase diagram in the strength of in-plane and out-of-plane DM couplings, and discuss the extended stability of the spin liquid of the unperturbed kagome antiferromagnet in the presence of these couplings.
We study the Kitaev-Heisenberg-$Gamma$-$Gamma$ model that describes the magnetism in strong spin-orbit coupled honeycomb lattice Mott insulators. In strong $[111]$ magnetic fields that bring the system into the fully polarized paramagnetic phase, we find that the spin wave bands carry nontrivial Chern numbers over large regions of the phase diagram implying the presence of chiral magnon edge states. In contrast to other topological magnon systems, the topological nontriviality of these systems results from the presence of magnon number non-conserving terms in the Hamiltonian. Since the effects of interactions are suppressed by $J/h$, the validity of the single particle picture is tunable making paramagnetic phases particularly suitable for the exploration of this physics. Using time dependent DMRG and interacting spin wave theory, we demonstrate the presence of the chiral edge mode and its evolution with field.
We analyze the magnon excitations in pyrochlore iridates with all-in-all-out (AIAO) antiferromagnetic order, focusing on their topological features. We identify the magnetic point group symmetries that protect the nodal-line band crossings and triple-point degeneracies that dominate the Berry curvature. We find three distinct regimes of magnon band topology, as a function of the ratio of Dzyaloshinskii-Moriya (DM) interaction to the antiferromagnetic exchange. We show how the thermal Hall response provides a unique probe of the topological magnon band structure in AIAO systems.
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