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Register a new userEnhanced superconductivity in FeSe/SrTiO$_3$ from the combination of forward scattering phonons and spin fluctuations
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We study the effect of combining spin fluctuations and forward scattering electron-phonon ({eph}) coupling on the superconductivity in the FeSe/SrTiO$_3$ system modeled by a phenomenological two-band Hubbard model with long-range {eph} interactions. We treat the electron and phonon degrees of freedom on an equal footing using a emph{fully} self-consistent FLEX plus Migdal-Eliashberg calculation, which includes a self-consistent determination of the spin fluctuation spectrum. Based on FeSe monolayers, we focus on the case where one of the bands lies below the Fermi level (i.e. incipient), and demonstrate that the combined interactions can enhance or suppress $T_c$, depending on their relative strength. For a suitable choice of parameters, the spin-fluctuation mechanism yields a $T_c approx 46.8$ K incipient $s_pm$ superconductor, consistent with surface-doped FeSe thin films. A forward-focused {eph} interaction further enhances the $T_c$, as observed in monolayer FeSe on SrTiO$_3$.
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Elucidating the microscopic origin of nematic order in iron-based superconducting materials is important because the interactions that drive nematic order may also mediate the Cooper pairing. Nematic order breaks fourfold rotational symmetry in the iron plane, which is believed to be driven by either orbital or spin degrees of freedom. However, as the nematic phase often develops at a temperature just above or coincides with a stripe magnetic phase transition, experimentally determining the dominant driving force of nematic order is difficult. Here, we use neutron scattering to study structurally the simplest iron-based superconductor FeSe, which displays a nematic (orthorhombic) phase transition at $T_s=90$ K, but does not order antiferromagnetically. Our data reveal substantial stripe spin fluctuations, which are coupled with orthorhombicity and are enhanced abruptly on cooling to below $T_s$. Moreover, a sharp spin resonance develops in the superconducting state, whose energy (~4 meV) is consistent with an electron boson coupling mode revealed by scanning tunneling spectroscopy, thereby suggesting a spin fluctuation-mediated sign-changing pairing symmetry. By normalizing the dynamic susceptibility into absolute units, we show that the magnetic spectral weight in FeSe is comparable to that of the iron arsenides. Our findings support recent theoretical proposals that both nematicity and superconductivity are driven by spin fluctuations.
Mono- and multilayer FeSe thin films grown on SrTiO$_mathrm{3}$ and BiTiO$_mathrm{3}$ substrates exhibit a greatly enhanced superconductivity over that found in bulk FeSe. A number of proposals have been advanced for the mechanism of this enhancement. One possibility is the introduction of a cross-interface electron-phonon ($e$-$ph$) interaction between the FeSe electrons and oxygen phonons in the substrates that is peaked in the forward scattering (small ${bf q}$) direction due to the two-dimensional nature of the interface system. Motivated by this, we explore the consequences of such an interaction on the superconducting state and electronic structure of a two-dimensional system using Migdal-Eliashberg theory. This interaction produces not only deviations from the expectations of conventional phonon-mediated pairing but also replica structures in the spectral function and density of states, as probed by angle-resolved photoemission spectroscopy, scanning tunneling microscopy/spectroscopy, and quasi-particle interference imaging. We also discuss the applicability of Migdal-Eliashberg theory for a situation where the ep interaction is peaked at small momentum transfer and in the FeSe/STO system.
Magnetic fluctuations in the molecular-intercalated FeSe superconductor Li{x}(ND2){y}(ND3){1-y}Fe2Se2 (Tc = 43K) have been measured by inelastic neutron scattering from a powder sample. The strongest magnetic scattering is observed at a wave vector Q ~ 1.4 A^{-1}, which is not consistent with the (pi,0) nesting wave vector that characterizes magnetic fluctuations in several other iron-based superconductors, but is close to the (pi, pi/2) position found for A{x}Fe{2-y}Se2 systems. At the energies probed (~ 5kB Tc), the magnetic scattering increases in intensity with decreasing temperature below Tc, consistent with the superconductivity-induced magnetic resonance found in other iron-based superconductors.
Superconductivity in LaNiPO is disrupted by small (~5%) amounts of non-stoichiometry on the lanthanum site, even though the electronic contribution to the heat capacity increases with increasing non-stoichiometry. All samples also exhibit specific heat anomalies consistent with the presence of ferromagnetic spin fluctuations (Tsf ~ 14 K). Comparison of layered nickel phosphide and nickel borocarbide superconductors reveals different structure-property correlations in the two families.
We use density functional theory to study the structure and the band structure of the monolayer FeSe deposited on the SrTiO$_3$ substrate with the additional layer of Se between them. Top of the SrTiO$_3$ is formed by the double TiO layer with and without oxygen vacancies. Several structures with different arrangements of the additional Se atoms above the double TiO layer is considered. Equilibrium structures were found and the band structures for them were obtained. Near the $Gamma=(0,0,0)$ point of the Brillouin zone, the hole Fermi surface pockets persist and, additionally, an electron pocket appears. Thus neither the presence of the additional Se layer nor the oxygen vacancies in the double TiO layer leads to the sinking of hole bands below the Fermi level near the $Gamma$ point. Necessity to include the strong electronic correlations into account is discussed.
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