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Register a new userAbsorption Saturation is Tailorable in the Strong Light-Matter Coupling Regime
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Added by
Raffaele Colombelli
Publication date
2020
fields
Physics
and research's language is
English
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It is well known that optical absorption saturation of intersubband transitions in doped semiconductor quantum wells is independent of the introduced doping in the absence of a cavity. When inserting the system in a resonator, we show that this remains valid only in the weak light-matter coupling regime. In the strong light-matter coupling regime instead, we demonstrate that absorption saturation is no more doping independent and it is instead tailorable. Based on this unified formalism for saturation in weak and strong coupling, we provide designs for semiconductor saturable absorption (SESAM) mirrors and bistable systems operating in the mid-infrared range of the electromagnetic spectrum and with extremely low saturation intensities. Countering intuition, we show that the most suitable region to exploit low saturation intensities is not the ultra-strong coupling regime, but is instead at the onset of strong light-matter coupling.
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Light-matter interactions can occur when an ensemble of molecular resonators is placed in a confined electromagnetic field. In the strong coupling regime the rapid exchange of energy between the molecules and the electromagnetic field results in the emergence of hybrid light-matter states called polaritons. Multiple criteria exist to define the strong coupling regime, usually by comparing the splitting of the polariton bands with the linewidths of the uncoupled modes. Here we highlight the limitations of these criteria and study strong coupling using spectroscopic ellipsometry, a commonly used optical characterisation technique. We identify a new signature of strong coupling in ellipsometric phase spectra. Combining ellipsometric amplitude and phase spectra yields a distinct topological feature that we suggest could serve as a new criterion for strong coupling. Our results introduce the idea of ellipsometric topology and could provide further insight into the transition from the weak to strong coupling regime.
The optical properties of transition metal dichalcogenide monolayers are widely dominated by excitons, Coulomb-bound electron-hole pairs. These quasi-particles exhibit giant oscillator strength and give rise to narrow-band, well-pronounced optical transitions, which can be brought into resonance with electromagnetic fields in microcavities and plasmonic nanostructures. Due to the atomic thinness and robustness of the monolayers, their integration in van der Waals heterostructures provides unique opportunities for engineering strong light-matter coupling. We review first results in this emerging field and outline future opportunities and challenges.
In transition metal dichalcogenides layers of atomic scale thickness, the electron-hole Coulomb interaction potential is strongly influenced by the sharp discontinuity of the dielectric function across the layer plane. This feature results in peculiar non-hydrogenic excitonic states, in which exciton-mediated optical nonlinearities are predicted to be enhanced as compared to their hydrogenic counterpart. To demonstrate this enhancement, we performed optical transmission spectroscopy of a MoSe$_2$ monolayer placed in the strong coupling regime with the mode of an optical microcavity, and analyzed the results quantitatively with a nonlinear input-output theory. We find an enhancement of both the exciton-exciton interaction and of the excitonic fermionic saturation with respect to realistic values expected in the hydrogenic picture. Such results demonstrate that unconventional excitons in MoSe$_2$ are highly favourable for the implementation of large exciton-mediated optical nonlinearities, potentially working up to room temperature.
The ultra-strong light-matter coupling regime has been demonstrated in a novel three-dimensional inductor-capacitor (LC) circuit resonator, embedding a semiconductor two-dimensional electron gas in the capacitive part. The fundamental resonance of the LC circuit interacts with the intersubband plasmon excitation of the electron gas at $omega_c = 3.3$~THz with a normalized coupling strength $2Omega_R/omega_c = 0.27$. Light matter interaction is driven by the quasi-static electric field in the capacitors, and takes place in a highly subwavelength effective volume $V_{mathrm{eff}} = 10^{-6}lambda_0^3$ . This enables the observation of the ultra-strong light-matter coupling with $2.4times10^3$ electrons only. Notably, our fabrication protocol can be applied to the integration of a semiconductor region into arbitrary nano-engineered three dimensional meta-atoms. This circuit architecture can be considered the building block of metamaterials for ultra-low dark current detectors.
We present a detailed study of the electroluminescence of intersubband devices operating in the light-matter strong coupling regime. The devices have been characterized by performing angle resolved spectroscopy that shows two distinct light intensity spots in the momentum-energy phase diagram. These two features of the electroluminescence spectra are associated with photons emitted from the lower polariton branch and from the weak coupling of the intersubband transition with an excited cavity mode. The same electroluminescent active region has been processed into devices with and without the optical microcavity to illustrate the difference between a device operating in the strong and weak coupling regime. The spectra are very well simulated as the product of the polariton optical density of states, and a function describing the energy window in which the polariton states are populated. The voltage evolution of the spectra shows that the strong coupling regime allows the observation of the electroluminescence at energies otherwise inaccessible.
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