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Register a new userAdiabatically Induced Orbital Magnetization
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A semiclassical theory for the orbital magnetization due to adiabatic evolutions of Bloch electronic states is proposed. It renders a unified theory for the periodic-evolution pumped orbital magnetization and the orbital magnetoelectric response in insulators by revealing that these two phenomena are the only instances where the induced magnetization is gauge invariant. This theory also accounts for the electric-field induced intrinsic orbital magnetization in two-dimensional metals and Chern insulators. We illustrate the orbital magnetization pumped by microscopic local rotations of atoms, which correspond to phonon modes with angular momentum, in toy models based on honeycomb lattice, and the results are comparable to the pumped spin magnetization via strong Rashba spin orbit coupling. We also show the vital role of the orbital magnetoelectricity in validating the Mott relation between the intrinsic nonlinear anomalous Hall and Ettingshausen effects.
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We propose an orbital magnetothermal effect wherein a temperature gradient generates an orbital magnetization (OM) for Bloch electrons, and we present a unified theory for electrically and thermally induced OM, valid for both metals and insulators. We reveal that there exists an intrinsic response of OM, for which the susceptibilities are completely determined by the band geometric quantities such as interband Berry connections, interband orbital moments, and the quantum metric. The theory can be readily combined with first-principles calculations to study real materials. As an example, we calculate the OM response in CrI$_{3}$ bilayers, where the intrinsic contribution dominates. The temperature scaling of intrinsic and extrinsic responses, the effect of phonon drag, and the phonon angular momentum contribution to OM are discussed.
We show that a controllable dc magnetization is accumulated in a junction comprising a quantum dot coupled to non-magnetic reservoirs if the junction is subjected to a time-dependent spin-orbit interaction. The latter is induced by an ac electric field generated by microwave irradiation of the gated junction. The magnetization is caused by inelastic spin-flip scattering of electrons that tunnel through the junction, and depends on the polarization of the electric field: a circularly polarized field leads to the maximal effect, while there is no effect in a linearly polarized field. Furthermore, the magnetization increases as a step function (smoothened by temperature) as the microwave photon energy becomes larger than the absolute value of the difference between the single energy level on the quantum dot and the common chemical potential in the leads.
In systems with time-reversal symmetry, the orbital magnetization is zero in equilibrium. Recently, it has been proposed that the orbital magnetization can be induced by an electric current in a helical crystal structure in the same manner as that in a classical solenoid. In this paper, we extend this theory and study the current-induced orbital magnetization in a broader class of systems without inversion symmetry. First, we consider polar metals which have no inversion symmetry. We find that the current-induced orbital magnetization appears in a direction perpendicular to the electric current even without spin-orbit coupling. Using the perturbation method, we physically clarify how the current-induced orbital magnetization appears in polar metals. As an example, we calculate the current-induced orbital magnetization in SnP, and find that it might be sufficiently large for measurement. Next, we consider a two-dimensional system without inversion symmetry. We establish a method to calculate the current-induced orbital magnetization in the in-plane direction by using real-space coordinates in the thickness direction. By applying this theory to surfaces and interfaces of insulators, we find that an electric current along surfaces and interfaces induces an orbital magnetization perpendicular to the electric current.
Flexible ferromagnetic rings are spin-chain magnets, in which the magnetic and mechanical subsystems are coupled. The coupling is achieved through the tangentially oriented anisotropy axis. The possibility to operate the mechanics of the nanomagnets by controlling their magnetization is an important issue for the nanorobotics applications. A minimal model for the deformable curved anisotropic Heisenberg ferromagnetic wire is proposed. An equilibrium phase diagram is constructed for the closed loop geometry: (i) A vortex state with vanishing total magnetic moment is typical for relatively large systems; in this case the wire has the form of a regular circle. (ii) A topologically trivial onion state with the planar magnetization distribution is realized in small enough systems; magnetic loop is elliptically deformed. By varying geometrical and elastic parameters a phase transition between the vortex and onion states takes place. The detailed analytical description of the phase diagram is well confirmed by numerical simulations.
Microwave radiation applied to single-molecule magnets can induce large magnetization changes when the radiation is resonant with transitions between spin levels. These changes are interpreted as due to resonant heating of the sample by the microwaves. Pulsed-radiation studies show that the magnetization continues to decrease after the radiation has been turned off with a rate that is consistent with the spins characteristic relaxation rate. The measured rate increases with pulse duration and microwave power, indicating that greater absorbed radiation energy results in a higher sample temperature. We also performed numerical simulations that qualitatively reproduce many of the experimental results. Our results indicate that experiments aimed at measuring the magnetization dynamics between two levels resonant with the radiation must be done much faster than the >20-microsecond time scales probed in these experiments.
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