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Measurement of the bulk radioactive contamination of detector-grade silicon with DAMIC at SNOLAB

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 Added by Ariel Matalon
 Publication date 2020
  fields Physics
and research's language is English




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We present measurements of bulk radiocontaminants in the high-resistivity silicon CCDs from the DAMIC at SNOLAB experiment. We utilize the exquisite spatial resolution of CCDs to discriminate between $alpha$ and $beta$ decays, and to search with high efficiency for the spatially-correlated decays of various radioisotope sequences. Using spatially-correlated $beta$ decays, we measure a bulk radioactive contamination of $^{32}$Si in the CCDs of $140 pm 30$ $mu$Bq/kg, and place an upper limit on bulk $^{210}$Pb of $< 160~mu$Bq/kg. Using similar analyses of spatially-correlated bulk $alpha$ decays, we set limits of $< 11$ $mu$Bq/kg (0.9 ppt) on $^{238}$U and of $< 7.3$ $mu$Bq/kg (1.8 ppt) on $^{232}$Th. The ability of DAMIC CCDs to identify and reject spatially-coincident backgrounds, particularly from $^{32}$Si, has significant implications for the next generation of silicon-based dark matter experiments, where $beta$s from $^{32}$Si decay will likely be a dominant background. This capability demonstrates the readiness of the CCD technology to achieve kg-scale dark matter sensitivity.



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We introduce the fully-depleted charge-coupled device (CCD) as a particle detector. We demonstrate its low energy threshold operation, capable of detecting ionizing energy depositions in a single pixel down to 50 eVee. We present results of energy calibrations from 0.3 keVee to 60 keVee, showing that the CCD is a fully active detector with uniform energy response throughout the silicon target, good resolution (Fano ~0.16), and remarkable linear response to electron energy depositions. We show the capability of the CCD to localize the depth of particle interactions within the silicon target. We discuss the mode of operation and unique imaging capabilities of the CCD, and how they may be exploited to characterize and suppress backgrounds. We present the first results from the deployment of 250 um thick CCDs in SNOLAB, a prototype for the upcoming DAMIC100. DAMIC100 will have a target mass of 0.1 kg and should be able to directly test the CDMS-Si signal within a year of operation.
We present measurements of radioactive contamination in the high-resistivity silicon charge-coupled devices (CCDs) used by the DAMIC experiment to search for dark matter particles. Novel analysis methods, which exploit the unique spatial resolution of CCDs, were developed to identify $alpha$ and $beta$ particles. Uranium and thorium contamination in the CCD bulk was measured through $alpha$ spectroscopy, with an upper limit on the $^{238}$U ($^{232}$Th) decay rate of 5 (15) kg$^{-1}$ d$^{-1}$ at 95% CL. We also searched for pairs of spatially correlated electron tracks separated in time by up to tens of days, as expected from $^{32}$Si-$^{32}$P or $^{210}$Pb-$^{210}$Bi sequences of $beta$ decays. The decay rate of $^{32}$Si was found to be $80^{+110}_{-65}$ kg$^{-1}$ d$^{-1}$ (95% CI). An upper limit of $sim$35 kg$^{-1}$ d$^{-1}$ (95% CL) on the $^{210}$Pb decay rate was obtained independently by $alpha$ spectroscopy and the $beta$ decay sequence search. These levels of radioactive contamination are sufficiently low for the successful operation of CCDs in the forthcoming 100 g DAMIC detector.
55 - Richard W. Kadel 2016
The high energy spectrum of alpha particles emitted from a single isotope uniformly contaminating a bulk solid has a flat energy spectrum with a high end cutoff energy equal to the maximal alpha kinetic energy ($T_{alpha}$) of the decay. In this flat region of the spectrum, we show the surface rate $r_btext{,(Bq/keV-cm}^{2})$ arising from a bulk alpha contamination $rho_b$ (Bq/cm$^3$) from a single isotope is given by $r_b =rho_b Delta R/ 4 Delta E $, where $Delta E = E_1-E_2>0 $ is the energy interval considered (keV) in the flat region of the spectrum and $Delta R = R_2-R_1$, where $R_2$ ($R_1$) is the amount of the bulk material (cm) necessary to degrade the energy of the alpha from $T_{alpha}$ to $E_2$ ($E_1$). We compare our calculation to a rate measurement of alphas from $^{147}$Sm, ($15.32%,pm,0.03%$ of Sm($nat$) and half life of $(1.06,pm,0.01)times,10^{11} text{yr}$, and find good agreement, with the ratio between prediction to measurement of $100.2%pm 1.6%,text{(stat)}pm 2.1%,text{(sys)}$. We derive the condition for the flat spectrum, and also calculate the relationship between the decay rate measured at the surface for a [near] surface contamination with an exponential dependence on depth and an a second case of an alpha source with a thin overcoat. While there is excellent agreement between our implementation of the sophisticated Monte Carlo program SRIM and our intuitive model in all cases, both fail to describe the measured energy distribution of a $^{148}$Gd alpha source with a thin ($sim200mu$g/cm$^2$) Au overcoat. We discuss possible origins of the disagreement and suggest avenues for future study.
The Deep Underground Neutrino Experiment (DUNE) is a leading-edge, international experiment for neutrino science and proton decay studies. This experiment is looking for answers regarding several fundamental questions about the nature of matter and the evolution of the universe: origin of matter, unification of forces, physics of black holes. Two far detector prototypes using two distinct technologies have been developed at CERN. The prototypes are testing and validating the liquid argon time projection chamber technology (LArTPC). In neutrino physics, as well as in any experiment with rare interaction rate, the good knowledge of the radioactive backgrounds is important to the success of the study. Unlike most of the charged particles or short lived neutral particles, muons and neutrons represent the main sources of background for this kind of experiments. In this paper, we have considered two sources of neutrons: cosmic neutrons and neutrons coming from the accelerating tunnel. Also, cosmic muons are taken into account. The contribution of these particles to the production of radioactive isotopes inside the active volume of the detector in comparison to the one corresponding to muons is shown. Also, simulations of nuclear reactions for the processes of interest for investigating the radioactive background due to the lack of measurements or insufficient experimental data are presented. The results presented are of interest for the future underground DUNE experiment.
The light yield and the time resolution of different types of 3 m long scintillating bars instrumented with wavelength shifting fibres and read out by different models of silicon photomultipliers have been measured at a test beam at the T9 area at the CERN Proton Synchrotron. The results obtained with different configurations are presented. A time resolution better than 800 ps, constant along the bar length within 20%, and a light yield of ~ 140 (70) photoelectrons are obtained for bars 3 m long, 4.5 (5) cm wide and 2 (0.7) cm thick. These results nicely match the requirements for the Muon Detector of the SHiP experiment.
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