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Domain Walls in a Row-Wise Antiferromagnetic Mn Monolayer

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 Added by Andre Kubetzka
 Publication date 2020
  fields Physics
and research's language is English




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We investigate magnetic domain walls in a single fcc Mn layer on Re(0001) employing spin-polarized STM, atom manipulation, and spin dynamics simulations. The low symmetry of the row-wise antiferromagnetic (1Q) state leads to a new type of domain wall which connects rotational 1Q domains by a transient 2Q state with characteristic 90$^circ$ angles between neighboring magnetic moments. The domain wall properties depend on their orientation and their width of about 2 nm essentially results from a balance of Heisenberg and higher-order exchange interactions. Atom manipulation allows domain wall imaging with atomic spin-resolution, as well as domain wall positioning, and we demonstrate that the force to move an atom is anisotropic on the 1Q domain.



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We consider a domain wall in the mesoscopic quasi-one-dimensional sample (wire or stripe) of weakly anisotropic two-sublattice antiferromagnet, and estimate the probability of tunneling between two domain wall states with different chirality. Topological effects forbid tunneling for the systems with half-integer spin S of magnetic atoms which consist of odd number of chains N. External magnetic field yields an additional contribution to the Berry phase, resulting in the appearance of two different tunnel splittings in any experimental setup involving a mixture of odd and even N, and in oscillating field dependence of the tunneling rate with the period proportional to 1/N.
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An antiferromagnetic domain wall in a thermal gradient is found to experience a force towards colder regions upon the application of a uniform magnetic field along the easy axis. This force increases with the strength of the applied field and, for sufficiently high values, it overcomes the entropic force the that pushes wall towards the hotter regions. The force is proportional to the thermal gradient and it shows a linear dependence with the net magnetic moment of the domain wall induced by the field. The origin of this force lies on the increase of the domain wall reflectivity due the field-induced sizable break of antiferromagnetic order inside it, which turns it into an efficient barrier for magnons, which transfer linear momentum to the domain wall when they are reflected on it
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The control of domain walls or spin textures is crucial for spintronic applications of antiferromagnets. Despite many efforts, it has been challenging to directly visualize antiferromagnetic domains or domain walls with nanoscale resolution, especially in magnetic field. Here, we report magnetic imaging of domain walls in several uniaxial antiferromagnets, the topological insulator MnBi$_2$Te$_4$ family and the Dirac semimetal EuMnBi$_2$, using cryogenic magnetic force microscopy (MFM). Our MFM results reveal higher magnetic susceptibility or net moments inside the domain walls than in domains. Domain walls in these antiferromagnets form randomly with strong thermal and magnetic field dependences. The direct visualization of domain walls and domain structure in magnetic field will not only facilitate the exploration of intrinsic phenomena in topological antiferromagnets, but also open a new path toward control and manipulation of domain walls or spin textures in functional antiferromagnets.
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