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Register a new userFloquet engineering of molecular dynamics via infrared coupling
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We discuss Floquet engineering of dissipative molecular systems through periodic driving of an infrared-active vibrational transition, either directly or via a cavity mode. Following a polaron quantum Langevin equations approach, we derive correlation functions and stationary quantities showing strongly modified optical response of the infrared-dressed molecule. The coherent excitation of molecular vibrational modes, in combination with the modulation of electronic degrees of freedom due to vibronic coupling can lead to both enhanced vibronic coherence as well as control over vibrational sideband amplitudes. The additional coupling to an infrared cavity allows for the controlled suppression of undesired sidebands, an effect stemming from the Purcell enhancement of vibrational relaxation rates.
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We propose to manipulate the statistic properties of the photons transport nonreciprocally via quadratic optomechanical coupling. We present a scheme to generate quadratic optomechanical interactions in the normal optical modes of a whispering-gallery-mode (WGM) optomechanical system by eliminating the linear optomechanical couplings via anticrossing of different modes. By optically pumping the WGM optomechanical system in one direction, the effective quadratic optomechanical coupling in that direction will be enhanced significantly, and nonreciprocal photon blockade will be observed consequently. Our proposal has potential applications for the on-chip nonreciprocal single-photon devices.
Floquet engineering, modulating quantum systems in a time periodic way, lies at the central part for realizing novel topological dynamical states. Thanks to the Floquet engineering, various new realms on experimentally simulating topological materials have emerged. Conventional Floquet engineering, however, only applies to time periodic non-dissipative Hermitian systems, and for the quantum systems in reality, non-Hermitian process with dissipation usually occurs. So far, it remains unclear how to characterize topological phases of periodically driven non-Hermitian systems via the frequency space Floquet Hamiltonian. Here, we propose the non-Floquet theory to identify different Floquet topological phases of time periodic non-Hermitian systems via the generation of Floquet band gaps in frequency space. In non-Floquet theory, the eigenstates of non-Hermitian Floquet Hamiltonian are temporally deformed to be of Wannier-Stark localization. Remarkably, we show that different choices of starting points of driving period can result to different localization behavior, which effect can reversely be utilized to design detectors of quantum phases in dissipative oscillating fields. Our protocols establish a fundamental rule for describing topological features in non-Hermitian dynamical systems and can find its applications to construct new types of Floquet topological materials.
We develop the Floquet-Magnus expansion for a classical equation of motion under a periodic drive that is applicable to both isolated and open systems. For classical systems, known approaches based on the Floquet theorem fail due to the nonlinearity and the stochasticity of their equations of motion (EOMs) in contrast to quantum ones. Here, employing their master equation, we successfully extend the Floquet methodology to classical EOMs to obtain their Floquet-Magnus expansions, thereby overcoming this difficulty. Our method has a wide range of application from classical to quantum as long as they are described by differential equations including the Langevin equation, the Gross-Pitaevskii equation, and the time-dependent Ginzburg-Landau equation. By analytically evaluating the higher-order terms of the Floquet-Magnus expansion, we find that it is, at least asymptotically, convergent and well approximates the relaxation to their prethermal or non-equilibrium steady states. To support these analytical findings, we numerically analyze two examples: (i) the Kapitza pendulum with friction and (ii) laser-driven magnets described by the stochastic Landau-Lifshitz-Gilbert equation. In both cases, the effective EOMs obtained from their Floquet-Magnus expansions correctly reproduce their exact time evolution for a long time up to their non-equilibrium steady states. In the example of driven magnets, we demonstrate the controlled generations of a macroscopic magnetization and a spin chirality by laser and discuss possible applications to spintronics.
The presence of quantum scars, athermal eigenstates of a many-body Hamiltonian with finite energy density, leads to absence of ergodicity and long-time coherent dynamics in closed quantum systems starting from simple initial states. Such non-ergodic coherent dynamics, where the system does not explore its entire phase space, has been experimentally observed in a chain of ultracold Rydberg atoms. We show, via study of a periodically driven Rydberg chain, that the drive frequency acts as a tuning parameter for several reentrant transitions between ergodic and non-ergodic regimes. The former regime shows rapid thermalization of correlation functions and absence of scars in the spectrum of the systems Floquet Hamiltonian. The latter regime, in contrast, has scars in its Floquet spectrum which control the long-time coherent dynamics of correlation functions. Our results open a new possibility of drive frequency-induced tuning between ergodic and non-ergodic dynamics in experimentally realizable disorder-free quantum many-body systems.
We provide a general discussion of the Liouvillian spectrum for a system coupled to a non-Markovian bath using Floquet theory. This approach is suitable when the system is described by a time-convolutionless master equation with time-periodic rates. Surprisingly, the periodic nature of rates allow us to have a stroboscopic divisible dynamical map at discrete times, which we refer to as Floquet stroboscopic divisibility. We illustrate the general theory for a Schrodinger cat which is roaming inside a non-Markovian bath, and demonstrate the appearance of stroboscopic revival of the cat at later time after its death. Our theory may have profound implications in entropy production in non-equilibrium systems.
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