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Register a new userEffective Waves for Random Three-dimensional Particulate Materials
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How do you take a reliable measurement of a material whose microstructure is random? When using wave scattering, the answer is often to take an ensemble average (average over time or space). By ensemble averaging we can calculate the average scattered wave and the effective wavenumber. To date, the literature has focused on calculating the effective wavenumber for a plate filled with particles. One clear unanswered question was how to extend this approach to a material of any geometry and for any source. For example, does the effective wavenumber depend on only the microstructure, or also on the material geometry? In this work, we demonstrate that the effective wavenumbers depend on only microstructure and not the geometry, though beyond the long wavelength limit there are multiple effective wavenumbers. We show how to calculate the average wave scattered from a random particulate material of any shape, and for broad frequency ranges. As an example, we show how to calculate the average wave scattered from a sphere filled with particles.
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For over 70 years it has been assumed that scalar wave propagation in (ensemble-averaged) random particulate materials can be characterised by a single effective wavenumber. Here, however, we show that there exist many effective wavenumbers, each contributing to the effective transmitted wave field. Most of these contributions rapidly attenuate away from boundaries, but they make a significant contribution to the reflected and total transmitted field beyond the low-frequency regime. In some cases at least two effective wavenumbers have the same order of attenuation. In these cases a single effective wavenumber does not accurately describe wave propagation even far away from boundaries. We develop an efficient method to calculate all of the contributions to the wave field for the scalar wave equation in two spatial dimensions, and then compare results with numerical finite-difference calculations. This new method is, to the authors knowledge, the first of its kind to give such accurate predictions across a broad frequency range and for general particle volume fractions.
Effective medium theory aims to describe a complex inhomogeneous material in terms of a few important macroscopic parameters. To characterise wave propagation through an inhomogeneous material, the most crucial parameter is the effective wavenumber. For this reason, there are many published studies on how to calculate a single effective wavenumber. Here we present a proof that there does not exist a unique effective wavenumber; instead, there are an infinite number of such (complex) wavenumbers. We show that in most parameter regimes only a small number of these effective wavenumbers make a significant contribution to the wave field. However, to accurately calculate the reflection and transmission coefficients, a large number of the (highly attenuating) effective waves is required. For clarity, we present results for scalar (acoustic) waves for a two-dimensional material filled (over a half space) with randomly distributed circular cylindrical inclusions. We calculate the effective medium by ensemble averaging over all possible inhomogeneities. The proof is based on the application of the Wiener-Hopf technique and makes no assumption on the wavelength, particle boundary conditions/size, or volume fraction. This technique provides a simple formula for the reflection coefficient, which can be explicitly evaluated for monopole scatterers. We compare results with an alternative numerical matching method.
The random-field Ising model (RFIM), one of the basic models for quenched disorder, can be studied numerically with the help of efficient ground-state algorithms. In this study, we extend these algorithm by various methods in order to analyze low-energy excitations for the three-dimensional RFIM with Gaussian distributed disorder that appear in the form of clusters of connected spins. We analyze several properties of these clusters. Our results support the validity of the droplet-model description for the RFIM.
We present results on the first excited states for the random-field Ising model. These are based on an exact algorithm, with which we study the excitation energies and the excitation sizes for two- and three-dimensional random-field Ising systems with a Gaussian distribution of the random fields. Our algorithm is based on an approach of Frontera and Vives which, in some cases, does not yield the true first excited states. Using the corrected algorithm, we find that the order-disorder phase transition for three dimensions is visible via crossings of the excitations-energy curves for different system sizes, while in two-dimensions these crossings converge to zero disorder. Furthermore, we obtain in three dimensions a fractal dimension of the excitations cluster of d_s=2.42(2). We also provide analytical droplet arguments to understand the behavior of the excitation energies for small and large disorder as well as close to the critical point.
Three-dimensional (3D) antiferromagnets with random magnetic anisotropy (RMA) experimentally studied to date do not have random single-ion anisotropies, but rather have competing two-dimensional and three-dimensional exchange interactions which can obscure the authentic effects of RMA. The magnetic phase diagram Fe$_{x}$Ni$_{1-x}$F$_{2}$ epitaxial thin films with true random single-ion anisotropy was deduced from magnetometry and neutron scattering measurements and analyzed using mean field theory. Regions with uniaxial, oblique and easy plane anisotropies were identified. A RMA-induced glass region was discovered where a Griffiths-like breakdown of long-range spin order occurs.
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