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Search for alpha decay of naturally occurring osmium nuclides accompanied by gamma quanta

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 Added by Rita Bernabei
 Publication date 2020
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and research's language is English




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A search for $alpha$ decay of naturally occurring osmium isotopes to the lowest excited levels of daughter nuclei has been performed by using an ultra-low-background Broad-Energy Germanium $gamma$-detector with a volume of 112 cm$^3$ and an ultra-pure osmium sample with a mass of 118 g at the Gran Sasso National Laboratory of the INFN (Italy). The isotopic composition of the osmium sample has been measured with high precision using Negative Thermal Ionisation Mass Spectrometry. After 15851 h of data taking with the $gamma$-detector no effect has been detected, and lower limits on the $alpha$ decays were set at level of $lim T_{1/2}sim 10^{15}-10^{19}$ yr. The limits for the $alpha$ decays of $^{184}$Os and $^{186}$Os to the first excited levels of daughter nuclei, $T_{1/2}(^{184}$Os$)geq 6.8times10^{15}$ yr and $T_{1/2}(^{186}$Os$)geq3.3times10^{17}$ yr (at 90% C.L.), exceed the present theoretical estimates of the decays half-lives. For $^{189}$Os and $^{192}$Os also decays to the ground states of the daughter nuclei were searched for due to the instability of the daughter nuclides relative to $beta$ decay.



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The first ever search for $alpha$ decays to the first excited state in Yb was performed for six isotopes of hafnium (174, 176, 177, 178, 179, 180) using a high purity Hf-sample of natural isotopic abundance with a mass of 179.8 g. For $^{179}$Hf, also $alpha$ decay to the ground state of $^{175}$Yb was searched for thanks to the $beta$-instability of the daughter nuclide $^{175}$Yb. The measurements were conducted using an ultra low-background HPGe-detector system located 225 m underground. After 75 d of data taking no decays were detected but lower bounds for the half-lives of the decays were derived on the level of $lim T_{1/2}sim 10^{15}-10^{18}$~a. The decay with the shortest half-life based on theoretical calculation is the decay of $^{174}$Hf to the first $2^+$ 84.3~keV excited level of $^{170}$Yb. The experimental lower bound was found to be $T_{1/2}geq 3.3times 10^{15}$ a.
131 - A. Marinov , A. Pape , Y. Kashiv 2011
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Evidence for the existence of long-lived neutron-deficient isotopes has been found in a study of naturally-occurring Th using iductively coupled plasma-sector field mass spectrometry. They are interpreted as belonging to the recently discovered class of long-lived high spin super- and hyperdeformed isomers.
Double-beta processes in $^{184}$Os and $^{192}$Os were searched for over 15851 h at the Gran Sasso National Laboratory (LNGS) of the I.N.F.N. by using a 118 g ultra-pure osmium sample installed on the endcap of a 112 cm$^3$ ultra-low-background broad-energy germanium detector. New limits on double-electron capture and electron capture with positron emission in $^{184}$Os were set at the level of $lim T_{1/2} sim 10^{16}-10^{17}$ yr. In particular the $2 u$2K and $2 u$KL decays of $^{184}$Os to the ground state of $^{184}$W are restricted as $T_{1/2}geq3.0times 10^{16}$ yr and $T_{1/2}geq2.0times 10^{16}$ yr, respectively. A lower limit on the half-life for the double-beta decay of $^{192}$Os to the first excited level of $^{192}$Pt was set as $lim T_{1/2}=2.0times 10^{20}$ yr at 90% C.L.
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