No Arabic abstract
We study the ultrafast demagnetization of Ni/NiMn and Co/NiMn ferromagnetic/antiferromagnetic bilayer systems after excitation by a laser pulse. We probe the ferromagnetic order of Ni and Co using magnetic circular dichroism in time-resolved pump--probe resonant X-ray reflectivity. Tuning the sample temperature across the antiferromagnetic ordering temperature of the NiMn layer allows to investigate effects induced by the magnetic order of the latter. The presence of antiferromagnetic order in NiMn speeds up the demagnetization of the ferromagnetic layer, which is attributed to bidirectional laser-induced superdiffusive spin currents between the ferromagnetic and the antiferromagnetic layer.
We use time-resolved x-ray resonant magnetic scattering (tr-XRMS) at the Co M$_{2,3}$- and Tb O$_1$-edges to study ultrafast demagnetization in an amorphous Co$_{88}$Tb$_{12}$ alloy with stripe domains. Combining the femtosecond temporal with nanometer spatial resolution of our experiment, we demonstrate that the equilibrium spin texture of the thin film remains unaltered by the optical pump-pulse on ultrashort timescales ($<$1 ps). However, after $simeq$ 4 ps, we observe the onset of a significant domain wall broadening, which we attribute to a reduction of the uniaxial magnetic anisotropy of the system, due to energy transfer to the lattice. Static temperature dependent magnetometry measurements combined with analytical modeling of the magnetic structure of the thin film corroborate this interpretation.
We demonstrate that ferromagnetic and antiferromagnetic excitations can be triggered by the dynamical spin accumulations induced by the bulk and surface contributions of the spin Hall effect. Due to the spin-orbit interaction, a time-dependent spin density is generated by an oscillatory electric field applied parallel to the atomic planes of Fe/W(110) multilayers. For symmetric trilayers of Fe/W/Fe in which the Fe layers are ferromagnetically coupled, we demonstrate that only the collective out-of-phase precession mode is excited, while the uniform (in-phase) mode remains silent. When they are antiferromagnetically coupled, the oscillatory electric field sets the Fe magnetizations into elliptical precession motions with opposite angular velocities. The manipulation of different collective spin-wave dynamical modes through the engineering of the multilayers and their thicknesses may be used to develop ultrafast spintronics devices. Our work provides a general framework that probes the realistic responses of materials in the time or frequency domain.
With reduced dimensionality, it is often easier to modify the properties of ultra-thin films than their bulk counterparts. Strain engineering, usually achieved by choosing appropriate substrates, has been proven effective in controlling the properties of perovskite oxide films. An emerging alternative route for developing new multifunctional perovskite is by modification of the oxygen octahedral structure. Here we report the control of structural oxygen octahedral rotation in ultra-thin perovskite SrRuO3 films by the deposition of a SrTiO3 capping layer, which can be lithographically patterned to achieve local control. Using a scanning Sagnac magnetic microscope, we show increase in the Curie temperature of SrRuO3 due to the suppression octahedral rotations revealed by the synchrotron x-ray diffraction. This capping-layer-based technique may open new possibilities for developing functional oxide materials.
The recent experiment [Y. Wang et al., Science 366, 1125 (2019)] on magnon-mediated spin-transfer torque (MSTT) was interpreted in terms of a picture where magnons are excited within an antiferromagnetic insulator (AFI), by applying nonequilibrium electronic spin density at one of its surfaces, so that their propagation across AFI deprived of conduction electrons eventually leads to reversal of magnetization of a ferromagnetic metal (FM) attached to the opposite surface of AFI. We employ a recently developed time-dependent nonequilibrium Green functions combined with the Landau-Lifshitz-Gilbert equation (TDNEGF+LLG) formalism to evolve conduction electrons quantum-mechanically while they interact via self-consistent back-action with localized magnetic moments described classically by atomistic spin dynamics solving a system of LLG equations. Upon injection of square current pulse as the initial condition, TDNEGF+LLG simulations of FM-polarizer/AFI/FM-analyzer junctions show that reversal of localized magnetic moments within FM-analyzer is less efficient, in the sense of requiring larger pulse height and its longer duration, than conventional electron-mediated STT (ESTT) driving magnetization switching in standard FM-polarizer/normal-metal/FM-analyzer spin valve. Since both electronic, generated by spin pumping from AFI, and magnonic, generated by direct transmission from AFI, spin currents are injected into the FM-analyzer, its localized magnetic moments will experience combined MSTT and ESTT. Nevertheless, by artificially turning off ESTT we demonstrate that MSTT plays a dominant role whose understanding, therefore, paves the way for all-magnon-driven magnetization switching devices with no electronic parts.
We present a thorough analysis of the foundations of models of stabilization of negative capacitance (NC) in a ferroelectric (FE) layer by capacitance matching to a dielectric layer, which claim that the FE is stabilized in a low polarization state without FE polarization switching (non-switching), showing that the concept is fundamentally flawed and unphysical. We also analyze experimental evidence concluding that there is no data supporting the need to invoke such stabilization; rather, conventional models of ferroelectric polarization switching suffice to account for the effects observed. We analyze experimental evidence that at least in some of the model systems for which this effect has been claimed, categorically rule out stabilized non-switching NC. Microscopic measurements recently published as supporting non-switching stabilized NC actually rule them out, since the ferroelectric in a stack sandwiched between two dielectric layers was found to be in a mixed domain state (high polarizations within each domain) rather than in the low polarization state predicted by non-switching stabilized NC models. Nonetheless, since stabilized NC (corresponding to a minimum in free energy) is not physically impossible, it would be useful to move the research efforts to investigating scenarios and systems in which this effect is possible and expected and assess whether they are useful and practical for low power electronics.