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Register a new userFrom triple-point materials to multiband nodal links
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Added by
Patrick M. Lenggenhager
Publication date
2020
fields
Physics
and research's language is
English
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We study a class of topological materials which in their momentum-space band structure exhibit three-fold degeneracies known as triple points. Focusing specifically on $mathcal{P}mathcal{T}$-symmetric crystalline solids with negligible spin-orbit coupling, we find that such triple points can be stabilized by little groups containing a three-, four- or six-fold rotation axis, and we develop a classification of all possible triple points as type-A vs. type-B according to the absence vs. presence of attached nodal-line arcs. Furthermore, by employing the recently discovered non-Abelian band topology, we argue that a rotation-symmetry-breaking strain transforms type-A triple points into multi-band nodal links. Although multi-band nodal-line compositions were previously theoretically conceived and related to topological monopole charges, a practical condensed-matter platform for their manipulation and inspection has hitherto been missing. By reviewing the known triple-point materials with weak spin-orbit coupling, and by performing first-principles calculations to predict new ones, we identify suitable candidates for the realization of multi-band nodal links in applied strain. In particular, we report that an ideal compound to study this phenomenon is Li$_2$NaN, in which the conversion of triple points to multi-band nodal links facilitates largely tunable density of states and optical conductivity with doping and strain, respectively.
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Acoustic phonon in a crystalline solid is a well-known and ubiquitous example of elementary excitation with a triple degeneracy in the band structure. Because of the Nambu-Goldstone theorem, this triple degeneracy is always present in the phonon band structure. Here, we show that the triple degeneracy of acoustic phonons can be characterized by a topological charge $mathfrak{q}$ that is a property of three-band systems with $mathcal{PT}$ symmetry, where $mathcal{P}$ and $mathcal{T}$ are the inversion and the time-reversal symmetries, respectively. We therefore call triple points with nontrivial $mathfrak{q}$ the topological acoustic triple point (TATP). The topological charge $mathfrak{q}$ can equivalently be characterized by the skyrmion number of the longitudinal mode, or by the Euler number of the transverse modes, and this strongly constrains the nodal structure around the TATP. The TATP can also be symmetry-protected at high-symmetry momenta in the band structure of phonons and spinless electrons by the $O_h$ and the $T_h$ groups. The nontrivial wavefunction texture around the TATP can induce anomalous thermal transport in phononic systems and orbital Hall effect in electronic systems. Our theory demonstrates that the gapless points associated with the Nambu-Goldstone theorem are an avenue for discovering new classes of degeneracy points with distinct topological characteristics.
Triple nodal points are degeneracies of energy bands in momentum space at which three Hamiltonian eigenstates coalesce at a single eigenenergy. For spinless particles, the stability of a triple nodal point requires two ingredients: rotation symmetry of order three, four or six; combined with mirror or space-time-inversion symmetry. However, despite ample studies of their classification, robust boundary signatures of triple nodal points have until now remained elusive. In this work, we first show that pairs of triple nodal points in semimetals and metals can be characterized by Stiefel-Whitney and Euler monopole invariants, of which the first one is known to facilitate higher-order topology. Motivated by this observation, we then combine symmetry indicators for corner charges and for the Stiefel-Whitney invariant in two dimensions with the classification of triple nodal points for spinless systems in three dimensions. The result is a complete higher-order bulk-boundary correspondence, where pairs of triple nodal points are characterized by fractional jumps of the hinge charge. We present minimal models of the various species of triple nodal points carrying higher-order topology, and illustrate the derived correspondence on Sc$_3$AlC which becomes a higher-order triple-point metal in applied strain. The generalization to spinful systems, in particular to the WC-type triple-point material class, is briefly outlined.
We propose a general and tunable platform to realize high-density arrays of quantum spin-valley Hall kink (QSVHK) states with spin-valley-momentum locking based on a two-dimensional hexagonal topological insulator. Through the analysis of Berry curvature and topological charge, the QSVHK states are found to be topologically protected by the valley-inversion and time-reversal symmetries. Remarkably, the conductance of QSVHK states remains quantized against either nonmagnetic or long-range magnetic disorder, verified by the Green function calculations. Based on first-principles results, we show that QSVHK states, protected with a gap up to 287 meV, can be realized in bismuthene by alloy engineering, surface functionalization, or electric field, supporting non-volatile applications of spin-valley filters, valves, and waveguides even at room temperature.
For three-dimensional metals, Landau levels disperse as a function of the magnetic field and the momentum wavenumber parallel to the field. In this two-dimensional parameter space, it is shown that two conically-dispersing Landau levels can touch at a diabolical point -- a Landau-Dirac point. The conditions giving rise to Landau-Dirac points are shown to be magnetic breakdown (field-induced quantum tunneling) and certain crystallographic spacetime symmetry. Both conditions are realizable in topological nodal-line metals, as we exemplify with CaP$_3$. A Landau-Dirac point reveals itself in anomalous batman-like peaks in the magnetoresistance, as well as in the onset of optical absorption linearly evolving to zero frequency as a function of the field magnitude/orientation.
Recently, it was pointed out that all chiral crystals with spin-orbit coupling (SOC) can be Kramers Weyl semimetals (KWSs) which possess Weyl points pinned at time-reversal invariant momenta. In this work, we show that all achiral non-centrosymmetric materials with SOC can be a new class of topological materials, which we term Kramers nodal line metals (KNLMs). In KNLMs, there are doubly degenerate lines, which we call Kramers nodal lines (KNLs), connecting time-reversal invariant momenta. The KNLs create two types of Fermi surfaces, namely, the spindle torus type and the octdong type. Interestingly, all the electrons on octdong Fermi surfaces are described by two-dimensional massless Dirac Hamiltonians. These materials support quantized optical conductance in thin films. We further show that KNLMs can be regarded as parent states of KWSs. Therefore, we conclude that all non-centrosymmetric metals with SOC are topological, as they can be either KWSs or KNLMs.
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