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Register a new userGeneration and manipulation of chiral terahertz waves emitted from the three-dimensional topological insulator Bi2Te3
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Arbitrary manipulation of broadband terahertz waves with flexible polarization shaping at the source has great potential in expanding real applications such as imaging, information encryption, and all-optically coherent control of terahertz nonlinear phenomena. Topological insulators featuring unique spin-momentum locked surface state have already exhibited very promising prospects in terahertz emission, detection and modulation, which may lay a foundation for future on-chip topological insulator-based terahertz systems. However, polarization shaped terahertz emission with prescribed manners of arbitrarily manipulated temporal evolution of the amplitude and electric-field vector direction based on topological insulators have not yet been explored. Here we systematically investigated the terahertz radiation from topological insulator Bi2Te3 nanofilms driven by femtosecond laser pulses, and successfully realized the generation of efficient chiral terahertz waves with controllable chirality, ellipticity, and principle axis. The convenient engineering of the chiral terahertz waves was interpreted by photogalvanic effect induced photocurrent, while the linearly polarized terahertz waves originated from linear photogalvanic effect induced shift currents. We believe our works not only help further understanding femtosecond coherent control of ultrafast spin currents in light-matter interaction but also provide an effective way to generate spin-polarized terahertz waves and accelerate the proliferation of twisting the terahertz waves at the source.
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The interplay between real-space topological lattice defects and the reciprocal-space topology of energy bands can give rise to novel phenomena, such as one-dimensional topological modes bound to screw dislocations in three-dimensional topological insulators. We obtain direct experimental observations of dislocation-induced helical modes in an acoustic analog of a weak three-dimensional topological insulator. The spatial distribution of the helical modes is found through spin-resolved field mapping, and verified numerically by tight-binding and finite-element calculations. These one-dimensional helical channels can serve as robust waveguides in three-dimensional media. Our experiment paves the way to studying novel physical modes and functionalities enabled by topological lattice defects in three-dimensional classical topological materials.
The Terahertz or millimeter wave frequency band (300 GHz - 3 THz) is spectrally located between microwaves and infrared light and has attracted significant interest for applications in broadband wireless communications, space-borne radiometers for Earth remote sensing, astrophysics, and imaging. In particular optically generated THz waves are of high interest for low-noise signal generation. In particular optically generated THz waves are of high interest for low-noise signal generation. Here, we propose and demonstrate stabilized terahertz wave generation using a microresonator-based frequency comb (microcomb). A unitravelling-carrier photodiode (UTC-PD) converts low-noise optical soliton pulses from the microcomb to a terahertz wave at the solitons repetition rate (331 GHz). With a free-running microcomb, the Allan deviation of the Terahertz signal is 4.5*10^-9 at 1 s measurement time with a phase noise of -72 dBc/Hz (-118 dBc/Hz) at 10 kHz (10 MHz) offset frequency. By locking the repetition rate to an in-house hydrogen maser, in-loop fractional frequency stabilities of 9.6*10^-15 and 1.9*10^-17 are obtained at averaging times of 1 s and 2000 s respectively, limited by the maser reference signal. Moreover, the terahertz signal is successfully used to perform a proof-of-principle demonstration of terahertz imaging of peanuts. Combining the monolithically integrated UTC-PD with an on-chip microcomb, the demonstrated technique could provide a route towards highly stable continuous terahertz wave generation in chip-scale packages for out-of-the-lab applications. In particular, such systems would be useful as compact tools for high-capacity wireless communication, spectroscopy, imaging, remote sensing, and astrophysical applications.
Photonic topological insulators (PTIs) exhibit robust photonic edge states protected by band topology, similar to electronic edge states in topological band insulators. Standard band theory does not apply to amorphous phases of matter, which are formed by non-crystalline lattices with no long-range positional order but only short-range order. Among other interesting properties, amorphous media exhibit transitions between glassy and liquid phases, accompanied by dramatic changes in short-range order. Here, we experimentally investigate amorphous variants of a Chern-number-based PTI. By tuning the disorder strength in the lattice, we demonstrate that photonic topological edge states can persist into the amorphous regime, prior to the glass-to-liquid transition. After the transition to a liquid-like lattice configuration, the signatures of topological edge states disappear. This interplay between topology and short-range order in amorphous lattices paves the way for new classes of non-crystalline topological photonic materials.
Highly efficient terahertz (THz) wave sources based on difference frequency generation (DFG) process in nonlinear optical crystals play an important role for the applications of THz wave. In order to find more novel nonlinear crystals, here we theoretically investigate the generation of THz wave using the isomorphs of periodically poled $mathrm{KTiOPO_4}$ (PPKTP), including periodically poled RTP, KTA, RTA and CTA. By solving the cascaded difference frequency coupled wave equations, it is found that the intensities of the THz wave generated from the cascaded difference frequency processes are improved by 5.27, 2.87, 2.82, 3.03, and 2.76 times from the non-cascaded cases for KTP, RTP, KTA, RTA and CTA, respectively. The effects of the crystal absorption, the phase mismatch and the pump intensity are also analyzed in detail. This study might help to provide a stronger THz radiation source based on the nonlinear crystals.
Fine control of the chiral light-matter interaction at the nanoscale, by exploiting designed metamaterial architecture, represents a cutting-edge craft in the field of biosensing, quantum and classic nanophotonics. Recently, artificially engineered 3D nanohelices have demonstrated programmable wide chiroptical properties by tuning materials and architecture, but fundamental diffractive aspects that are to the origin of chiral resonances still remain elusive. Here, we proposed a novel concept of three-dimensional chiral MetaCrystal, where the chiroptical properties are finely tuned by in-plane and out-of-plane diffractive coupling. Different chiral dipolar modes can be excited along the helix arms, generating far field optical resonances and radiation pattern with in-plane side lobes and suggesting that a combination of efficient dipole excitation and diffractive coupling matching controls the collective oscillations among the neighbor helices in the chiral MetaCrystal. This concept enables the tailorability of chiral properties in a broad spectral range for a plethora of forefront applications, since the proposed compact chiral MetaCrystal can be suitable for integration with quantum emitters and can open perspectives in novel schemes of enantiomeric detection.
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