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Register a new userAdvances in Nb3Sn superconducting radiofrequency cavities towards first practical accelerator applications
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Nb3Sn is a promising next-generation material for superconducting radiofrequency cavities, with significant potential for both large scale and compact accelerator applications. However, so far, Nb3Sn cavities have been limited to cw accelerating fields <18 MV/m. In this paper, new results are presented with significantly higher fields, as high as 24 MV/m in single cell cavities. Results are also presented from the first ever Nb3Sn-coated 1.3 GHz 9-cell cavity, a full-scale demonstration on the cavity type used in production for the European XFEL and LCLS-II. Results are presented together with heat dissipation curves to emphasize the potential for industrial accelerator applications using cryocooler-based cooling systems. The cavities studied have an atypical shiny visual appearance, and microscopy studies of witness samples reveal significantly reduced surface roughness and smaller film thickness compared to typical Nb3Sn films for superconducting cavities. Possible mechanisms for increased maximum field are discussed as well as implications for physics of RF superconductivity in the low coherence length regime. Outlook for continued development is presented.
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We report on an effort to improve the performance of superconducting radiofrequency cavities by the use of heat treatment in a temperature range sufficient to dissociate the natural surface oxide. We find that the residual resistance is significantly decreased, and we find an unexpected reduction in the BCS resistance. Together these result in extremely high quality factor values at relatively large accelerating fields Eacc ~20 MV/m: Q0 of 3-4x10^11 at <1.5 K and Q0 ~5x10^10 at 2.0 K. In one cavity, measurements of surface resistance versus temperature showed an extremely small residual resistance of just 0.63+/-0.06 nOhms at 16 MV/m. SIMS measurements confirm that the oxide was significantly dissociated, but they also show the presence of nitrogen after heat treatment. We also present studies of surface oxidation via exposure to air and to water, as well as the effects of very light surface removal via HF rinse. The possibilities for applications and the planned future development are discussed.
As a result of a collaboration between Jefferson Lab and niobium manufacturer CBMM, ingot niobium was explored as a possible material for superconducting radiofrequency (SRF) cavity fabrication. The first single cell cavity from large grain high purity niobium was fabricated and successfully tested at Jefferson Lab in 2004. This pioneering work triggered research activities in other SRF laboratories around the world. Large grain niobium became not only an interesting alternative material for cavity builders, but also material scientists and surface scientists were eager to participate in the development of this material. Most of the original expectations for this material of being less costly and allowing less expensive fabrication and treatment procedures at the same performance levels in cavities have been met. Many single cell cavities made from material of different suppliers have been tested successfully and several multi-cell cavities have shown the performances comparable to the best cavities made from standard poly-crystalline niobium. Several 9-cell cavities fabricated by Research Instruments and tested at DESY exceeded the best performing fine grain cavities with a record accelerating gradient of Eacc = 45.6 MV/m. Recently- at JLab- by using a new furnace treatment procedure a single cell cavity made of ingot niobium performed at a remarkably high Q0-value (~5x10^10) at an accelerating gradient of ~20 MV/m, at 2K. Such performance levels push the state-of-the art of SRF technology to new limits and are of great interest for future accelerators. This contribution reviews the development of ingot niobium technology and attempts to make a case for this material being the choice for future accelerators.
We report on atomic-scale analyses of grain boundary (GB) structures and segregation in Nb3Sn coatings on Nb, prepared by the vapor-diffusion process, for superconducting radiofrequency (SRF) cavity applications, utilizing atom-probe tomography, high-resolution scanning transmission electron-microscopy and first-principles calculations. We demonstrate that the chemical composition of Nb3Sn GBs is correlated strongly with the diffusion of Sn and Nb at GBs during the coating process. In a sample coated with a relatively large Sn flux, we observe an interfacial width of Sn segregation at a GB of ~3 nm, with a maximum concentration of ~35 at.%. After post-annealing at 1100 oC for 3 h, the Sn segregated at GBs disappears and Nb segregation is observed subsequently at GBs, indicating that Nb diffused into the Nb3Sn GBs from the Nb substrate. It is also demonstrated that the amount of Sn segregation in a Nb3Sn coating can be controlled by: (i) Sn flux; and (ii) the temperatures of the Nb substrates and Sn source, which may affect the overall kinetics including GB diffusion of Sn and Nb. An investigation of the correlation between the chemical compositions of GBs and Nb3Sn SRF cavity performance reveals that the Nb3Sn SRF cavities with the best performance (high-quality factors at high accelerating electric-field gradients) do not exhibit Sn segregation at GBs. Our results suggest that the chemical compositions of GBs in Nb3Sn coatings for SRF cavities can be controlled by GB engineering and can be utilized to optimize fabrication of high-quality Nb3Sn coatings for SRF cavities.
Even when cooled through its transition temperature in the presence of an external magnetic field, a superconductor can expel nearly all external magnetic flux. This Letter presents an experimental study to identify the parameters that most strongly influence flux trapping in high purity niobium during cooldown. This is critical to the operation of superconducting radiofrequency cavities, in which trapped flux degrades the quality factor and therefore cryogenic efficiency. Flux expulsion was measured on a large survey of 1.3 GHz cavities prepared in various ways. It is shown that both spatial thermal gradient and high temperature treatment are critical to expelling external magnetic fields, while surface treatment has minimal effect. For the first time, it is shown that a cavity can be converted from poor expulsion behavior to strong expulsion behavior after furnace treatment, resulting in a substantial improvement in quality factor. Future plans are described to build on this result in order to optimize treatment for future cavities.
We report an atomic-scale analysis of the microstructure of Nb3Sn coating on Nb prepared by vapor diffusion process for superconducting radiofrequency (SRF) cavity application using transmission electron microscopy (TEM). Epitaxial growth of Nb3Sn on the Nb substrate is found and four types of orientation relationships at the Nb3Sn/Nb interface are identified by electron diffraction or high-resolution scanning transmission electron microscopy (STEM) analysis. Thin Nb3Sn grains are observed in regions with low Sn flux and they have the specific orientation relationship, Nb3Sn (1-20)//Nb (-111) and Nb3Sn (002)//Nb (0-11). The Nb3Sn/Nb interface of thin grains had a large lattice mismatch, 12.3 at.%, and a high density of misfit dislocations was observed by HR-STEM. Based on our microstructural analysis of the thin grains, we conclude that the thin regions are probably a result of a slow interfacial reaction with this particular orientation relationship at the interface. The Sn-deficient regions are seen to form initially at the Nb3Sn/Nb interface and remain in the grains due to the slow diffusion of Sn in bulk Nb3Sn. The formation of Sn-deficient regions and the effects of strain and interfacial energies on the formation of Sn-deficient regions at various interfaces were also estimated by first-principle calculation. The finding of orientation relationships at the Nb3Sn/Nb interface provides important information about the formation of defects in Nb3Sn coatings such as large thin regions, Sn-deficient regions, which are critical to the performance of Nb3Sn superconducting radiofrequency cavities for accelerators.
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