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Register a new userEvidence for the general dominance of proton shells in low-energy fission
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A regular pattern, revealing the leading role of the light-fragment nuclear charge, is found to emerge from a consistent analysis of the experimental information collected recently on low-energy asymmetric fission of neutron-deficient nuclei around lead. The observation is corroborated by a theoretical investigation within a microscopic framework, suggesting the importance of proton configurations driven by quadrupole-octupole correlations. This is in contrast to the earlier theoretical interpretations in terms of dominant neutron shells. The survey of a wider area of the nuclear chart by a semi-empirical approach points to the lack of understanding of the competition between the different underlying macroscopic and microscopic forces in a quantitative manner. Combined with previously identified stabilizing forces, the present finding shows a striking connection between the old (actinide) and new (pre-actinide) islands of asymmetric fission which could steer the strive for an unified theory of fission.
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We analyze recent data from high-momentum-transfer $(p,pp)$ and $(p,ppn)$ reactions on Carbon. For this analysis, the two-nucleon short-range correlation (NN-SRC) model for backward nucleon emission is extended to include the motion of the NN-pair in the mean field. The model is found to describe major characteristics of the data. Our analysis demonstrates that the removal of a proton from the nucleus with initial momentum 275-550 MeV/c is $92^{+8}_{-18}%$ of the time accompanied by the emission of a correlated neutron that carries momentum roughly equal and opposite to the initial proton momentum. Within the NN-SRC dominance assumption the data indicate that the probabilities of $pp$ or $nn$ SRCs in the nucleus are at least a factor of six smaller than that of $pn$ SRCs. Our result is the first estimate of the isospin structure of NN-SRCs in nuclei, and may have important implication for modeling the equation of state of asymmetric nuclear matter.
The Hauser-Feshbach fission fragment decay model, $mathtt{HF^3D}$, which calculates the statistical decay of fission fragments, has been expanded to include multi-chance fission, up to neutron incident energies of 20 MeV. The deterministic decay takes as input pre-scission quantities - fission probabilities and the average energy causing fission - and post-scission quantities - yields in mass, charge, total kinetic energy, spin, and parity. From these fission fragment initial conditions, the full decay is followed through both prompt and delayed particle emissions, allowing for the calculation of prompt neutron and $gamma$ properties, such as multiplicity and energy distributions, both independent and cumulative fission yields, and delayed neutron observables. In this work, we describe the implementation of multi-chance fission into the $mathtt{HF^3D}$ model, and show an example of prompt and delayed quantities beyond first-chance fission, using the example of neutron-induced fission on $^{235}$U. This expansion represents significant progress in consistently modeling the emission of prompt and delayed particles from fissile systems.
Several sources of angular anisotropy for fission fragments and prompt neutrons have been studied in neutron-induced fission reactions. These include kinematic recoils of the target from the incident neutron beam and the fragments from the emission of the prompt neutrons, preferential directions of the emission of the fission fragments with respect to the beam axis due to the population of particular transition states at the fission barrier, and forward-peaked angular distributions of pre-equilibrium neutrons which are emitted before the formation of a compound nucleus. In addition, there are several potential sources of angular anisotropies that are more difficult to disentangle: the angular distributions of prompt neutrons from fully accelerated fragments or from scission neutrons, and the emission of neutrons from fission fragments that are not fully accelerated. In this work, we study the effects of the first group of anisotropy sources, particularly exploring the correlations between the fission fragment anisotropy and the resulting neutron anisotropy. While kinematic effects were already accounted for in our Hauser-Feshbach Monte Carlo code, $mathtt{CGMF}$, anisotropic angular distributions for the fission fragments and pre-equilibrium neutrons resulting from neutron-induced fission on $^{233,234,235,238}$U, $^{239,241}$Pu, and $^{237}$Np have been introduced for the first time. The effects of these sources of anisotropy are examined over a range of incident neutron energies, from thermal to 20 MeV, and compared to experimental data from the Chi-Nu liquid scintillator array. The anisotropy of the fission fragments is reflected in the anisotropy of the prompt neutrons, especially as the outgoing energy of the prompt neutrons increases, allowing for an extraction of the fission fragment anisotropy to be made from a measurement of the neutrons.
Potential energy surfaces and fission barriers of superheavy nuclei are analyzed in the macroscopic-microscopic model. The Lublin-Strasbourg Drop (LSD) is used to obtain the macroscopic part of the energy, whereas the shell and pairing energy corrections are evaluated using the Yukawa-folded potential. A standard flooding technique has been used to determine the barrier heights. It was shown the Fourier shape parametrization containing only three deformation parameters reproduces well the nuclear shapes of nuclei on their way to fission. In addition, the non-axial degree of freedom is taken into account to describe better the form of nuclei around the ground state and in the saddles region. Apart from the symmetric fission valley, a new very asymmetric fission mode is predicted in most superheavy nuclei. The fission fragment mass distributions of considered nuclei are obtained by solving the 3D Langevin equations.
The atomic numbers and the masses of fragments formed in quasi-fission reactions have been simultaneously measured at scission in 48 Ti + 238 U reactions at a laboratory energy of 286 MeV. The atomic numbers were determined from measured characteristic fluorescence X-rays whereas the masses were obtained from the emission angles and times of flight of the two emerging fragments. For the first time, thanks to this full identification of the quasi-fission fragments on a broad angular range, the important role of the proton shell closure at Z = 82 is evidenced by the associated maximum production yield, a maximum predicted by time dependent Hartree-Fock calculations. This new experimental approach gives now access to precise studies of the time dependence of the N/Z (neutron over proton ratios of the fragments) evolution in quasi-fission reactions.
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