No Arabic abstract
We examine the far-field optical response, under-plane wave excitation in the presence of a static magnetic field, of core-shell nanoparticles involving a gyroelectric component, either as the inner or the outer layer, through analytic calculations based on appropriately extended Mie theory. We focus on absorption and scattering of light by bismuth-substituted yttrium iron garnet (Bi:YIG) nanospheres and nanoshells, combined with excitonic materials such as organic-molecule aggregates or two-dimensional transition-metal dichalcogenides, and discuss the hybrid character of the modes emerging from the coupling of the two constituents. We observe the excitation of strong magneto-optic phenomena and explore, in particular, the response and tunability of a magneto-transverse light current, indicative of the photonic Hall effect. We show how interaction between the Bi:YIG and excitonic layers leads to a pair of narrow bands of highly directional scattering, emerging from the aforementioned hybridization, which can be tuned at will by adjusting the geometrical or optical parameters of the system. Our theoretical study introduces optically anisotropic media as promising templates for strong coupling in nanophotonics, offering a means to combine tunable magnetic and optical properties, with potential implications both in the design of all-dielectric photonic devices but also in novel clinical applications.
The dispersion properties of exciton polaritons in multiple-quantum-well based resonant photonic crystals are studied. In the case of structures with an elementary cell possessing a mirror symmetry with respect to its center, a powerful analytical method for deriving and analyzing dispersion laws of the respective normal modes is developed. The method is used to analyze band structure and dispersion properties of several types of resonant photonic crystals, which would not submit to analytical treatment by other approaches. These systems include multiple quantum well structures with an arbitrary periodic modulation of the dielectric function and structures with a complex elementary cell. Special attention was paid to determining conditions for superradiance (Bragg resonance) in these structures, and to the properties of the polariton stop band in the case when this condition is fulfilled (Bragg structures). The dependence of the band structure on the angle of propagation, the polarization of the wave, and the effects due to exciton homogeneous and inhomogeneous broadenings are considered, as well as dispersion properties of excitations in near-Bragg structures.
We examine the current-induced dynamics of a skyrmion that is subject to both structural and bulk inversion asymmetry. There arises a hybrid type of Dzyaloshinskii-Moriya interaction (DMI) which is in the form of a mixture of interfacial and bulk DMIs. Examples include crystals with symmetry classes C$_n$ as well as magnetic multilayers composed of a ferromagnet with a noncentrosymmetric crystal and a nonmagnet with strong spin-orbit coupling. As a striking result, we find that, in systems with a hybrid DMI, the spin-orbit-torque-induced skyrmion Hall angle is asymmetric for the two different skyrmion polarities ($pm 1$ given by out-of-plane core magnetization), even allowing one of them to be tuned to zero. We propose several experimental ways to achieve the necessary straight skyrmion motion (with zero Hall angle) for racetrack memories, even without antiferromagnetic interactions or any interaction with another magnet. Our results can be understood within a simple picture by using a global spin rotation which maps the hybrid DMI model to an effective model containing purely interfacial DMI. The formalism directly reveals the effective spin torque and effective current that result in qualitatively different dynamics. Our work provides a way to utilize symmetry breaking to eliminate detrimental phenomena as hybrid DMI eliminates the skyrmion Hall angle.
We theoretically analyse the hybrid Mie-exciton optical modes arising from the strong coupling of excitons in organic dyes or transition-metal dichalcogenides with the Mie resonances of high-index dielectric nanoparticles. Detailed analytic calculations show that silicon--exciton core--shell nanoparticles are characterised by a richness of optical modes which can be tuned through nanoparticle dimensions to produce large anticrossings in the visible or near infrared, comparable to those obtained in plexcitonics. The complex magnetic-excitonic nature of these modes is understood through spectral decomposition into Mie-coefficient contributions, complemented by electric and magnetic near-field profiles. In the frequency range of interest, absorptive losses in silicon are sufficiently low to allow observation of several periods of Rabi oscillations in strongly coupled emitter-particle architectures, as confirmed here by discontinuous Galerkin time-domain calculations for the electromagnetic field beat patterns. These results suggest that Mie resonances in high-index dielectrics are promising alternatives for plasmons in strong-coupling applications in nanophotonics, while the coupling of magnetic and electric modes opens intriguing possibilities for external control.
We propose theoretically a reconfigurable two-dimensional (2D) hexagonal sonic crystal with higher-order topology protected by the six-fold, $C_6$, rotation symmetry. The acoustic band gap and band topology can be controlled by rotating the triangular scatterers in each unit-cell. In the nontrivial phase, the sonic crystal realizes the topological spin Hall effect in a higher-order fashion: (i) The edge states emerging in the bulk band gap exhibits partial spin-momentum locking and are gapped due to the reduced spatial symmetry at the edges. (ii) The gapped edge states, on the other hand, stabilize the topological corner states emerging in the edge band gap. The partial spin-momentum locking is manifested as pseudo-spin-polarization of edge states away from the time-reversal invariant momenta, where the pseudospin is emulated by the acoustic orbital angular momentum. We reveal the underlying topological mechanism using a corner topological index based on the symmetry representation of the acoustic Bloch bands.
We investigate the excitonic dynamics in MoSe2 monolayer and bulk samples by femtosecond transient absorption microscopy. Excitons are resonantly injected by a 750-nm and 100-fs laser pulse, and are detected by a probe pulse tuned in the range of 790 - 820 nm. We observe a strong density-dependent initial decay of the exciton population in monolayers, which can be well described by the exciton-exciton annihilation. Such a feature is not observed in the bulk under comparable conditions. We also observe the saturated absorption induced by exciton phase-space filling in both monolayers and the bulk, which indicates their potential applications as saturable absorbers.