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Register a new userSymmetry broken Chern insulators and magic series of Rashba-like Landau level crossings in magic angle bilayer graphene
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Flat-bands in magic angle twisted bilayer graphene (MATBG) have recently emerged as a rich platform to explore strong correlations, superconductivity and mag-netism. However, the phases of MATBG in magnetic field, and what they reveal about the zero-field phase diagram remain relatively unchartered. Here we use magneto-transport and Hall measurements to reveal a rich sequence of wedge-like regions of quantized Hall conductance with Chern numbers C = +(-)1, +(-)2, +(-)3, +(-)4 which nucleate from integer fillings of the moire unit cell v = +(-)3, +(-)2, +(-)1, 0 correspondingly. We interpret these phases as spin and valley polarized Chern insulators, equivalent to quantum Hall ferro-magnets. The exact sequence and correspondence of Chern numbers and filling factors suggest that these states are driven directly by electronic interactions which specifically break time-reversal symmetry in the system. We further study quantum magneto-oscillation in the yet unexplored higher energy dispersive bands with a Rashba-like dis-persion. Analysis of Landau level crossings enables a parameter-free comparison to a newly derived magic series of level crossings in magnetic field and provides constraints on the parameters w0 and w1 of the Bistritzer-MacDonald MATBG Hamiltonian. Over-all, our data provides direct insights into the complex nature of symmetry breaking in MATBG and allows for quantitative tests of the proposed microscopic scenarios for its electronic phases.
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Magic-angle twisted bilayer graphene (MATBG) exhibits a range of correlated phenomena that originate from strong electron-electron interactions. These interactions make the Fermi surface highly susceptible to reconstruction when $ pm 1, pm 2, pm 3$ electrons occupy each moir e unit cell and lead to the formation of correlated insulating, superconducting and ferromagnetic phases. While some phases have been shown to carry a non-zero Chern number, the local microscopic properties and topological character of many other phases remain elusive. Here we introduce a set of novel techniques hinging on scanning tunneling microscopy (STM) to map out topological phases in MATBG that emerge in finite magnetic field. By following the evolution of the local density of states (LDOS) at the Fermi level with electrostatic doping and magnetic field, we visualize a local Landau fan diagram that enables us to directly assign Chern numbers to all observed phases. We uncover the existence of six topological phases emanating from integer fillings in finite fields and whose origin relates to a cascade of symmetry-breaking transitions driven by correlations. The spatially resolved and electron-density-tuned LDOS maps further reveal that these topological phases can form only in a small range of twist angles around the magic-angle value. Both the microscopic origin and extreme sensitivity to twist angle differentiate these topological phases from the Landau levels observed near charge neutrality. Moreover, we observe that even the charge-neutrality Landau spectrum taken at low fields is considerably modified by interactions and exhibits an unexpected splitting between zero Landau levels that can be as large as ${sim },3-5$ meV. Our results show how strong electronic interactions affect the band structure of MATBG and lead to the formation of correlation-enabled topological phases.
We show that the flat bands in the chiral model of magic-angle twisted bilayer graphene remain exactly flat in the presence of a perpendicular magnetic field. This is shown by an exact mapping between the model and the lowest Landau level wavefunctions at an effective magnetic field, in which the external field is either augmented or reduced by one flux quantum per unit cell. When the external field reaches one flux quantum per unit cell, the model exhibits a topological phase transition. These findings allow us to analyze a Jain-series of Fractional Chern Insulators states in the exactly flat band, and to point out an unconventional dependence of the energy gap on the magnetic field.
Fractional Chern insulators (FCIs) are lattice analogues of fractional quantum Hall states that may provide a new avenue toward manipulating non-abelian excitations. Early theoretical studies have predicted their existence in systems with energetically flat Chern bands and highlighted the critical role of a particular quantum band geometry. Thus far, however, FCI states have only been observed in Bernal-stacked bilayer graphene aligned with hexagonal boron nitride (BLG/hBN), in which a very large magnetic field is responsible for the existence of the Chern bands, precluding the realization of FCIs at zero field and limiting its potential for applications. By contrast, magic angle twisted bilayer graphene (MATBG) supports flat Chern bands at zero magnetic field, and therefore offers a promising route toward stabilizing zero-field FCIs. Here we report the observation of eight FCI states at low magnetic field in MATBG enabled by high-resolution local compressibility measurements. The first of these states emerge at 5 T, and their appearance is accompanied by the simultaneous disappearance of nearby topologically-trivial charge density wave states. Unlike the BLG/hBN platform, we demonstrate that the principal role of the weak magnetic field here is merely to redistribute the Berry curvature of the native Chern bands and thereby realize a quantum band geometry favorable for the emergence of FCIs. Our findings strongly suggest that FCIs may be realized at zero magnetic field and pave the way for the exploration and manipulation of anyonic excitations in moire systems with native flat Chern bands.
Interactions among electrons and the topology of their energy bands can create novel quantum phases of matter. Most topological electronic phases appear in systems with weak electron-electron interactions. The instances where topological phases emerge only as a result of strong interactions are rare, and mostly limited to those realized in the presence of intense magnetic fields. The discovery of flat electronic bands with topological character in magic-angle twisted bilayer graphene (MATBG) has created a unique opportunity to search for new strongly correlated topological phases. Here we introduce a novel local spectroscopic technique using a scanning tunneling microscope (STM) to detect a sequence of topological insulators in MATBG with Chern numbers C = $pm$ 1, $pm$ 2, $pm$ 3, which form near $ u$ = $pm$ 3, $pm$ 2, $pm$ 1 electrons per moire unit cell respectively, and are stabilized by the application of modest magnetic fields. One of the phases detected here (C = +1) has been previously observed when the sublattice symmetry of MATBG was intentionally broken by hexagonal boron nitride (hBN) substrates, with interactions playing a secondary role. We demonstrate that strong electron-electron interactions alone can produce not only the previously observed phase, but also new and unexpected Chern insulating phases in MATBG. The full sequence of phases we observed can be understood by postulating that strong correlations favor breaking time-reversal symmetry to form Chern insulators that are stabilized by weak magnetic fields. Our findings illustrate that many-body correlations can create topological phases in moire systems beyond those anticipated from weakly interacting models.
Magic-angle twisted bilayer graphene (MA-TBG) exhibits intriguing quantum phase transitions triggered by enhanced electron-electron interactions when its flat-bands are partially filled. However, the phases themselves and their connection to the putative non-trivial topology of the flat bands are largely unexplored. Here we report transport measurements revealing a succession of doping-induced Lifshitz transitions that are accompanied by van Hove singularities (VHS) which facilitate the emergence of correlation-induced gaps and topologically non-trivial sub-bands. In the presence of a magnetic field, well quantized Hall plateaus at filling of 1, 2, 3 carriers per moire-cell reveal the sub-band topology and signal the emergence of Chern insulators with Chern-numbers, ! = !, !, !, respectively. Surprisingly, for magnetic fields exceeding 5T we observe a VHS at a filling of 3.5, suggesting the possibility of a fractional Chern insulator. This VHS is accompanied by a crossover from low-temperature metallic, to high-temperature insulating behavior, characteristic of entropically driven Pomeranchuk-like transitions,
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