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Register a new userTowards 1% single photon nonlinearity with periodically-poled lithium niobate microring resonators
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The absence of the single-photon nonlinearity has been a major roadblock in developing quantum photonic circuits at optical frequencies. In this paper, we demonstrate a periodically-poled thin film lithium niobate microring resonator (PPLNMR) that reaches 5,000,000%/W second harmonic conversion efficiency---almost 20-fold enhancement over the state-of-the-art---by accessing its largest $chi^{(2)}$ tensor component $d_{33}$ via quasi-phase matching. The corresponding single photon coupling rate $g/2pi$ is estimated to be 1.2 MHz, which is an important milestone as it approaches the dissipation rate $kappa/2pi$ of best available lithium niobate microresonators developed in the community. Using a figure of merit defined as $g/kappa$, our devices reach a single photon nonlinearity approaching 1%. We show that, by further scaling of the device, it is possible to improve the single photon nonlinearity to a regime where photon-blockade effect can be manifested.
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Lithium niobate (LN), dubbed by many as the silicon of photonics, has recently risen to the forefront of chip-scale nonlinear optics research since its demonstration as an ultralow-loss integrated photonics platform. Due to its significant quadratic nonlinearity ($chi^{(2)}$), LN inspires many important applications such as second-harmonic generation (SHG), spontaneous parametric down-conversion, and optical parametric oscillation. Here, we demonstrate high-efficiency SHG in dual-resonant, periodically poled z-cut LN microrings, where quasi-phase matching is realized by field-assisted domain engineering. Meanwhile, dual-band operation is accessed by optimizing the coupling conditions in fundamental and second-harmonic bands via a single pulley waveguide. As a result, when pumping a periodically poled LN microring in the low power regime at around 1617nm, an on-chip SHG efficiency of 250,000%/W is achieved, a state-of-the-art value reported among current integrated photonics platforms. An absolute conversion efficiency of 15% is recorded with a low pump power of 115$mu$W in the waveguide. Such periodically poled LN microrings also present a versatile platform for other cavity-enhanced quasi-phase matched $chi^{(2)}$ nonlinear optical processes.
Prospective integrated quantum optical technologies will combine nonlinear optics and components requiring cryogenic operating temperatures. Despite the prevalence of integrated platforms exploiting $chi^{(2)}$-nonlinearities for quantum optics, for example used for quantum state generation and frequency conversion, their material properties at low temperatures are largely unstudied. Here, we demonstrate the first second harmonic generation in a fiber-coupled lithium niobate waveguide at temperatures down to 4.4K. We observe a reproducible shift in the phase-matched pump wavelength within the telecom band, in addition to transient discontinuities while temperature cycling. Our results establish lithium niobate as a versatile nonlinear photonic integration platform compatible with cryogenic quantum technologies.
The amplified spontaneous emission from a superluminescent diode was frequency doubled in a periodically poled lithium niobate waveguide crystal. The temporally incoherent radiation of such a superluminescent diode is characterized by a relatively broad spectral bandwidth and thermal-like photon statistics, as the measured degree of second order coherence, g$^{(2)}$(0)=1.9$pm$0.1, indicates. Despite the non-optimized scenario in the spectral domain, we achieve six orders of magnitude higher conversion efficiency than previously reported with truly incoherent light. This is possible by using single spatial mode radiation and quasi phase matched material with a waveguide architecture. This work is a principle step towards efficient frequency conversion of temporally incoherent radiation in one spatial mode to access wavelengths where no radiation from superluminescent diodes is available, especially with tailored quasi phase matched crystals. The frequency doubled light might find use in applications and quantum optics experiments.
Temporal cloaks have inspired the innovation of research on security and efficiency of quantum and fiber communications for concealing temporal events. The existing temporal cloaking approaches possessing ps ~ns cloaking windows employed the third-order nonlinearity mostly. Here we explore a temporal cloak for perpetually concealing pulse events using high efficiency second-order nonlinearity. A temporal pulse event was cloaked as a continuous wave with constant intensity and restored by polarization dependent sum frequency generation processes between the continuous wave and probe. The variety of quasi phase-matching second-order nonlinear processes in periodically poled lithium niobate make sure the pulse event cannot be filched during transmission. The proposed temporal cloak predicts hopeful applications in information security of photonic integrated circuit on lithium niobite thin film.
Lithium niobate on insulator (LNOI), regarded as an important candidate platform for optical integration due to its excellent nonlinear, electro-optic and other physical properties, has become a research hotspot. Light source, as an essential component for integrated optical system, is urgently needed. In this paper, we reported the realization of 1550-nm band on-chip LNOI microlasers based on erbium-doped LNOI ring cavities with loaded quality factors higher than one million, which were fabricated by using electron beam lithography and inductively coupled plasma reactive ion etching processes. These microlasers demonstrated a low pump threshold of ~20 {mu}W and stable performance under the pump of a 980-nm band continuous laser. Comb-like laser spectra spanning from 1510 nm to 1580 nm were observed in high pump power regime, which lays the foundation of the realization of pulsed laser and frequency combs on rare-earth ion doped LNOI platform. This work has effectively promoted the development of on-chip integrated active LNOI devices.
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