We present experiments on polarization gradient cooling of Ca$^+$ multi-ion Coulomb crystals in a linear Paul trap. Polarization gradient cooling of the collective modes of motion whose eigenvectors have overlap with the symmetry axis of the trap is achieved by two counter-propagating laser beams with mutually orthogonal linear polarizations that are blue-detuned from the S$_{1/2}$ to P$_{1/2}$ transition. We demonstrate cooling of linear chains of up to 51 ions and 2D-crystals in zig-zag configuration with 22 ions. The cooling results are compared with numerical simulations and the predictions of a simple model of cooling in a moving polarization gradient.
The electronic and motional degrees of freedom of trapped ions can be controlled and coherently coupled on the level of individual quanta. Assembling complex quantum systems ion by ion while keeping this unique level of control remains a challenging task. For many applications, linear chains of ions in conventional traps are ideally suited to address this problem. However, driven motion due to the magnetic or radio-frequency electric trapping fields sometimes limits the performance in one dimension and severely affects the extension to higher dimensional systems. Here, we report on the trapping of multiple Barium ions in a single-beam optical dipole trap without radio-frequency or additional magnetic fields. We study the persistence of order in ensembles of up to six ions within the optical trap, measure their temperature and conclude that the ions form a linear chain, commonly called a one-dimensional Coulomb crystal. As a proof-of-concept demonstration, we access the collective motion and perform spectrometry of the normal modes in the optical trap. Our system provides a platform which is free of driven motion and combines advantages of optical trapping, such as state-dependent confinement and nano-scale potentials, with the desirable properties of crystals of trapped ions, such as long-range interactions featuring collective motion. Starting with small numbers of ions, it has been proposed that these properties would allow the experimental study of many-body physics and the onset of structural quantum phase transitions between one- and two-dimensional crystals.
Light-induced control of ions within small Coulomb crystals is investigated. By intense intracavity optical standing wave fields, subwavelength localization of individual ions is achieved for one-, two-, and three-dimensional crystals. Based on these findings, we illustrate numerically how the application of such optical potentials can be used to tailor the normal mode spectra and patterns of multi-dimensional Coulomb crystals. The results represent, among others, important steps towards controlling the crystalline structure of Coulomb crystals, investigating heat transfer processes at the quantum limit and quantum simulations of many-body systems.
Electromagnetically-induced-transparency (EIT) cooling is a ground-state cooling technique for trapped particles. EIT offers a broader cooling range in frequency space compared to more established methods. In this work, we experimentally investigate EIT cooling in strings of trapped atomic ions. In strings of up to 18 ions, we demonstrate simultaneous ground state cooling of all radial modes in under 1 ms. This is a particularly important capability in view of emerging quantum simulation experiments with large numbers of trapped ions. Our analysis of the EIT cooling dynamics is based on a novel technique enabling single-shot measurements of phonon numbers, by rapid adiabatic passage on a vibrational sideband of a narrow transition.
We investigate the dynamics of an ion sympathetically cooled by another laser-cooled ion or small ion crystal. To this end, we develop simple models of the cooling dynamics in the limit of weak Coulomb interactions. Experimentally, we create a two-ion crystal of Ca$^+$ and Al$^+$ by photo-ionization of neutral atoms produced by laser ablation. We characterize the velocity distribution of the laser-ablated atoms crossing the trap by time-resolved fluorescence spectroscopy. We observe neutral atom velocities much higher than the ones of thermally heated samples and find as a consequence long sympathethic cooling times before crystallization occurs. Our key result is a new technique for detecting the loading of an initially hot ion with energy in the eV range by monitoring the motional state of a Doppler-cooled ion already present in the trap. This technique not only detects the ion but also provides information about dynamics of the sympathetic cooling process.
Ion Coulomb crystals are currently establishing themselves as a highly controllable test-bed for mesoscopic systems of statistical mechanics. The detailed experimental interrogation of the dynamics of these crystals however remains an experimental challenge. In this work, we show how to extend the concepts of multi-dimensional nonlinear spectroscopy to the study of the dynamics of ion Coulomb crystals. The scheme we present can be realized with state-of-the-art technology and gives direct access to the dynamics, revealing nonlinear couplings even in the presence of thermal excitations. We illustrate the advantages of our proposal showing how two-dimensional spectroscopy can be used to detect signatures of a structural phase transition of the ion crystal, as well as resonant energy exchange between modes. Furthermore, we demonstrate in these examples how different decoherence mechanisms can be identified.