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Electrohydrodynamics of dielectric droplet collision with variant wettability surfaces

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 Added by Purbarun Dhar
 Publication date 2020
  fields Physics
and research's language is English




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In this article, we report experimental and semi analytical findings to elucidate the electrohydrodynamics EHD of a dielectric liquid droplet impact on superhydrophobic SH and hydrophilic surfaces. A wide range of Weber numbers We and electro-capillary numbers Cae is covered to explore the various regimes of droplet impact EHD. We show that for a fixed We 60, droplet rebound on SH surface is suppressed with increase of electric field intensity. At high Cae, instead of the usual uniform radial contraction, the droplets retract faster in orthogonal direction to the electric field and spread along the direction of the electric field. This prevents the accumulation of sufficient kinetic energy to achieve the droplet rebound phenomena. For certain values of We and Ohnesorge number Oh, droplets exhibit somersault like motion during rebound. Subsequently we propose a semi analytical model to explain the field induced rebound phenomenon on SH surfaces. Above a critical Cae 4.0, EHD instability causes fingering pattern via evolution of spire at the rim. Further, the spreading EHD on both hydrophilic and SH surfaces are discussed. On both wettability surfaces and for a fixed We, the spreading factor shows an increasing trend with increase in Cae. We have formulated an analytical model based on energy conservation to predict the maximum spreading diameter. The model predictions hold reasonably good agreement with the experimental observations. Finally, a phase map was developed to explain the post impact droplet dynamics on SH surfaces for a wide range of We and Cae.



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The transport of small quantities of liquid on a solid surface is inhibited by the resistance to motion caused by the contact between the liquid and the solid. To overcome such resistance, motion can be externally driven through gradients in electric fields, but these all inconveniently involve the input of external energy. Alternatively, gradients in physical shape and wettability - the conical shape of cactus spines to create self-propelled motion. However, such self-propelled motion to date has limited success in overcoming the inherent resistance to motion of the liquid contact with the solid. Here we propose a simple solution in the form of shaped-liquid surface, where solid topographic structures at one length scale provides the base for a smaller length-scale liquid conformal layer. This dual-length scale render possible slippery surfaces with superhydrophobic properties. Combined to an heterogeneous topography, it provides a gradient in liquid-on-liquid wettability with minimal resistance to motion and long range directional self-propelled droplet transport. Moreover, the liquid-liquid contact enables impacting droplets to be captured and transported, even when the substrate is inverted. These design principles are highly beneficial for droplet transport in microfluidics, self-cleaning surfaces, fog harvesting and in heat transfer.
The deformation of a viscous liquid droplet suspended in another liquid and subject to an applied electric field is a classic multiphase flow problem best described by the Melcher-Taylor leaky dielectric model. The main assumption of the model is that any net charge in the system is concentrated on the interface between the two liquids as a result of the jump in Ohmic currents from the bulk. Upon application of the field, the drop can either attain a steady prolate or oblate shape with toroidal circulating flows both inside and outside arising from tangential stresses on the interface due to action of the field on the surface charge distribution. Since the pioneering work of cite{taylor1966}, there have been numerous computational and theoretical studies to predict the deformations measured in experiments. Most existing theoretical models, however, have either neglected transient charge relaxation or nonlinear charge convection by the interfacial flow. In this work, we develop a novel small-deformation theory accurate to second order in electric capillary number ${O}(Ca_E^2)$ for the complete Melcher-Taylor model that includes transient charge relaxation, charge convection by the flow, as well as transient shape deformation. The main result of the paper is the derivation of coupled evolution equations for the induced electric multipoles and for the shape functions describing the deformations on the basis of spherical harmonics. Our results, which are consistent with previous models in the appropriate limits, show excellent agreement with fully nonlinear numerical simulations based on an axisymmetric boundary-element formulation and with existing experimental data in the small-deformation regime.
The influence of miscibility and liquid wettability during droplet impact onto thin wall films is investigated experimentally. Despite similar liquid properties and impact conditions, differences in the splashing limit, the crown extension and the duration of the ascending phase are observed. These differences are related to the interfacial tension of the droplet/wall-film liquid pairs, which is linked to their miscibility and wettability. More precisely, by calculating the crown surface energy, we show that the energy stored in the interface between droplet and wall-film (if any) is not negligible and leads to smaller crown extensions and the need of more kinetic energy to initiate splashing. Similarly, by calculating a modified capillary time taking into account all surface and interfacial tensions, we show that the interfacial tension acts as a non-negligible recoiling force, which reduces the duration of the ascending phase. The dynamics of this ascending phase is well captured for different wall-film thicknesses if accounting for the variations of the liquid masses in movement. Overall, droplet/wall-film interactions can be seen as inertio-capillary systems where the interfacial tension between droplet and wall film plays a significant role in the storage of energy and in the crown kinetics during the impact process. Besides, this analysis highlights that viscous losses have already a significant effect during the crown extension phase, by dissipating almost half of the initial energies for droplet impact onto thin wall films, and most likely by influencing the capillary time scale through damping.
409 - Chengming He , Lianjie Yue , 2021
Recent studies have demonstrated the significant roles of droplet self-spin motion in affecting the head-on collision of binary droplets. In this paper, we present a computational study by using the Volume-of-Fluid (VOF) method to investigate the spin-affected droplet separation of off-center collisions, which are more probable in reality and phenomenologically richer than head-on collisions. Different separation modes are identified through a parametric study with varying spinning speed and impact parameter. A prominent finding is that increasing the droplet spinning speed tends to suppress the reflexive separation and to promote the stretching separation. Physically, the reflexive separation is suppressed because the increased rotational energy reduces the excessive reflexive kinetic energy within the droplet, which is the cause for the droplet reflexive separation. The stretching separation is promoted because the increased droplet angular momentum enhances the local stretching flow within the droplet, which tends to separate the droplet. The roles of orbital angular momentum and spin angular momentum in affecting the droplet separation are further substantiated by studying the collision between two spinning droplets with either the same or opposite chirality. In addition, a theoretical model based on conservation laws is proposed to qualitatively describe the boundaries of coalescence-separation transition influenced by droplet self-spin motion.
The article reports droplet evaporation kinetics on inclined substrates. Comprehensive experimental and theoretical analyses of the droplet evaporation behaviour for different substrate declination, wettability and temperatures have been presented. Sessile droplets with substrate declination exhibit distorted shape and evaporate at different rates compared to droplets on the same horizontal substrate and is characterized by more often changes in regimes of evaporation. The slip stick and jump stick modes are prominent during evaporation. For droplets on inclined substrates, the evaporative flux is also asymmetric and governed by the initial contact angle dissimilarity. Due to smaller contact angle at the rear contact line, it is the zone of a higher evaporative flux. Particle image velocimetry shows the increased internal circulation velocity within the inclined droplets. Asymmetry in the evaporative flux leads to higher temperature gradients, which ultimately enhances the thermal Marangoni circulation near the rear of the droplet where the evaporative flux is highest. A model is adopted to predict the thermal Marangoni advection velocity, and good match is obtained. The declination angle and imposed thermal conditions interplay and lead to morphed evaporation kinetics than droplets on horizontal heated surfaces. Even weak movements of the TL alter the evaporation dynamics significantly, by changing the shape of the droplet from ideally elliptical to almost spherical cap, which ultimately reduces the evaporative flux. The life time of the droplet is modelled by modifying available models for non-heated substrate, to account for the shape asymmetry. The present findings may find strong implications towards microscale thermo-hydrodynamics.
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