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Large-Scale, Precision Xenon Doping of Liquid Argon

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 Added by Neil McFadden
 Publication date 2020
  fields Physics
and research's language is English




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The detection of scintillation light from liquid argon is an experimental technique key to a number of current and future nuclear/particle physics experiments, such as neutrino physics, neutrinoless double beta decay and dark matter searches. Although the idea of adding small quantities of xenon (doping) to enhance the light yield has attracted considerable interest, this technique has never been demonstrated at the necessary scale or precision. Here we report on xenon doping in a 100 l cryogenic vessel. Xenon doping was performed in four concentrations of 1.00$pm$0.06 ppm, 2.0$pm$0.1 ppm, 5.0$pm$0.3 ppm, and 10.0$pm$0.5 ppm. These measurements represent the most precise xenon doping measurements as of publishing. We observed an increase in average light yield by a factor of 1.92$pm$0.12(syst)$pm$0.02(stat) at a dopant concentration of 10 ppm.



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The use of xenon-doped liquid argon is a promising alternative for large pure liquid-argon TPCs. Not only xenon-doped liquid argon enhances the light production, mitigating the possible suppression due to impurities, but also it increases the wavelength of the scintillation light, enlarging the effective Rayleigh scattering length and improving the detection uniformity. ProtoDUNE Dual-Phase is a 300-ton active volume LAr TPC, a prototype for the Deep Underground Neutrino Experiment (DUNE), a dual-site experiment for long-baseline neutrino oscillation studies, neutrino astrophysics and nucleon decay searches. ProtoDUNE Dual-Phase took cosmic muon data at CERN with pure liquid argon and with xenon-doped liquid argon for over a year. The impact of the presence of xenon in the scintillation light and its comparison with the pure liquid argon data will be presented. These results are of interest to any future large LAr TPCs.
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Scintillation from noble gases is an important technique in particle physics including neutrino beam experiments, neutrino-less double beta-decay and dark matter searches. In liquid argon, the possibility of enhancing the light yield by the addition of a small quantity of xenon (doping at 10-1000 ppm) has been of particular interest. While the pathway for energy transfer between argon and xenon excimers is well known, the time-dependence of the process has not been fully studied in the context of a physics-based model. In this paper we present a model of the energy transfer process together with a fit to xenon-doped argon data. We have measured the diffusion limited rate constant as a function of xenon dopant. We find that the time dependence of the energy transfer is consistent with diffusion-limited reactions. Additionally, we find that commercially obtained argon can have a small xenon component (4 ppm). Our result will facilitate the use of xenon-doped liquid argon in future experiments.
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