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Register a new userControl and modulation of droplet vaporization rates via competing ferro- and electro-hydrodynamics
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Modification and control over the vaporization kinetics of microfluidic droplets may have strong utilitarian implications in several scientific and technological applications. The article reports the control over the vaporization kinetics of pendent droplets under the influence of competing internal electrohydrodynamic and ferrohydrodynamic advection. Experimental and theoretical studies are performed and the morphing of vaporization kinetics of electrically conducting and paramagnetic fluid droplets using orthogonal electric and magnetic stimuli is established. Analysis of the observations reveals that the electric field has a domineering influence compared to the magnetic field. While the magnetic field is noted to aid the vaporization rates, the electric field is observed to decelerate the same. Neither the vapour diffusion dominated kinetics nor the field induced modified surface tension can explain the observed vaporization behaviours. Velocimetry within the droplet shows largely modified internal ferro and electrohydrodynamic advection, which is noted to be the crux of the mechanism towards modified vaporization rates. A mathematical treatment is proposed and takes into account the roles played by the governing Hartmann, electrohydrodynamic, interaction, the thermal and solutal Marangoni, and the electro and magneto Prandtl and Schmidt numbers. It is observed that the morphing of the thermal and solutal Marangoni numbers by the electromagnetic interaction number plays the dominant role towards morphing the advection dynamics. The model is able to predict the internal advection velocities accurately. The findings may hold significant promise towards smart control and tuning of vaporization kinetics in microhydrodynamics transport paradigms.
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In this article we report the atypical and anomalous evaporation kinetics of saline sessile droplets on surfaces with elevated temperatures. In a previous we showed that saline sessile droplets evaporate faster compared to water droplets when the substrates are not heated. In the present study we discover that in the case of heated surfaces, the saline droplets evaporate slower than the water counterpart, thereby posing a counter-intuitive phenomenon. The reduction in the evaporation rates is directly dependent on the salt concentration and the surface wettability. Natural convection around the droplet and thermal modulation of surface tension is found to be inadequate to explain the mechanisms. Flow visualisations using particle image velocimetry PIV reveals that the morphed advection within the saline droplets is a probable reason behind the arrested evaporation. Infrared thermography is employed to map the thermal state of the droplets. A thermosolutal Marangoni based scaling analysis is put forward. It is observed that the Marangoni and internal advection borne of thermal and solutal gradients are competitive, thereby leading to the overall decay of internal circulation velocity, which reduces the evaporation rates. The theoretically obtained advection velocities conform to the experimental results. This study sheds rich insight on a novel yet anomalous species transport behaviour in saline droplets.
The levitation of a volatile droplet on a highly superheated surface is known as the Leidenfrost effect. Wetting state during transition from full wetting of a surface by a droplet at room temperature to Leidenfrost bouncing, i.e., zero-wetting at high superheating, is not fully understood. Here, visualizations of droplet thermal and wetting footprint in the Leidenfrost transition state are presented using two optical techniques: mid-infrared thermography and wetting sensitive total internal reflection imaging under carefully selected experimental conditions, impact Weber number < 10 and droplet diameter < capillary length, using an indium-tin-oxide coated sapphire heater. The experimental regime was designed to create relatively stable droplet dynamics, where the effects of oscillatory and capillary instabilities were minimized. The thermography for ethanol droplet in Leidenfrost transition state (superheat range of 82K-97K) revealed thermal footprint with a central hot zone surrounded by a cooler periphery, indicative of a partial wetting state during Leidenfrost transition. High-speed total internal reflection imaging also confirmed the partial wetting footprint such that there are wetting areas around a central non-wetting zone. Result presented here using ethanol as a test fluid shed light on the geometry and dynamics of a volatile droplet footprint in Leidenfrost transition state.
An electrohydrodynamic (EHD) flow in a point-to-ring corona configuration is investigated experimentally, analytically and via a multiphysics numerical model. The interaction between the accelerated ions and the neutral gas molecules is modeled as an external body force in the Navier-Stokes equation (NSE). The gas flow characteristics are solved from conservation principles with spectral methods. The analytical and numerical simulation results are compared against experimental measurements of the cathode voltage, ion concentration, and velocity profiles. A nondimensional parameter, X, is formulated as the ratio of the local electric force to the inertial term in the NSE. In the region of X > 1, the electric force dominates the flow dynamics, while in the X << 1 region, the balance of viscous and inertial terms yields traditional pipe flow characteristics.
The article experimentally reveals and theoretically establishes the influence of electric fields on the evaporation kinetics of pendant droplets. It is shown that the evaporation kinetics of saline pendant droplets can be augmented by the application of an external alternating electric field. The evaporation behaviour is modulated by an increase in the field strength and frequency. The classical diffusion driven evaporation model is found insufficient in predicting the improved evaporation rates. The change in surface tension due to field constraint is insufficient for explaining the observed physics. Consequently, the internal hydrodynamics of the droplet is probed employing particle image velocimetry. It is revealed that the electric field induces enhanced internal advection, which improves the evaporation rates. A scaled analytical model is proposed to understand the role of internal electrohydrodynamics, electrothermal and the electrosolutal effects. Stability maps reveal that the advection is caused nearly equally by the electrosolutal and electrothermal effects within the droplet. The model is able to illustrate the influence played by the governing thermal and solutal Marangoni number, the electro Prandtl and electro Schmidt number, and the associated Electrohydrodynamic number. The magnitude of the internal circulation can be well predicted by the proposed model, which validates the proposed mechanism.
The study reports the aspects of postimpact hydrodynamics of ferrofluid droplets on superhydrophobic SH surfaces in the presence of a horizontal magnetic field. A wide gamut of dynamics was observed by varying the impact Weber number We, the Hartmann number Ha and the magnetic field strength manifested through the magnetic Bond number Bom. For a fixed We 60, we observed that at moderately low Bom 300, droplet rebound off the SH surface is suppressed. The noted We is chosen to observe various impact outcomes and to reveal the consequent ferrohydrodynamic mechanisms. We also show that ferrohydrodynamic interactions leads to asymmetric spreading, and the droplet spreads preferentially in a direction orthogonal to the magnetic field lines. We show analytically that during the retraction regime, the kinetic energy of the droplet is distributed unequally in the transverse and longitudinal directions due to the Lorentz force. This ultimately leads to suppression of droplet rebound. We study the role of Bom at fixed We 60, and observed that the liquid lamella becomes unstable at the onset of retraction phase, through nucleation of holes, their proliferation and rupture after reaching a critical thickness only on SH surfaces, but is absent on hydrophilic surfaces. We propose an analytical model to predict the onset of instability at a critical Bom. The analytical model shows that the critical Bom is a function of the impact We, and the critical Bom decreases with increasing We. We illustrate a phase map encompassing all the post impact ferrohydrodynamic phenomena on SH surfaces for a wide range of We and Bom.
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