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A six-octave optical frequency comb from a scalable few-cycle erbium fiber laser

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 Added by Daniel Lesko
 Publication date 2020
  fields Physics
and research's language is English




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A compact and robust coherent laser light source that provides spectral coverage from the ultraviolet to infrared is desirable for numerous applications, including heterodyne super resolution imaging[1], broadband infrared microscopy[2], protein structure determination[3], and standoff atmospheric trace-gas detection[4]. Addressing these demanding measurement problems, laser frequency combs[5] combine user-defined spectral resolution with sub-femtosecond timing and waveform control to enable new modalities of high-resolution, high-speed, and broadband spectroscopy[6-9]. In this Letter we introduce a scalable source of near-single-cycle, 0.56 MW pulses generated from robust and low-noise erbium fiber (Er:fiber) technology, and we use it to generate a frequency comb that spans six octaves from the ultraviolet (350 nm) to mid-infrared (22500 nm). The high peak power allows us to exploit the second-order nonlinearities in infrared-transparent, nonlinear crystals (LiNbO$_3$, GaSe, and CSP) to provide a robust source of phase-stable infrared ultra-short pulses with simultaneous spectral brightness exceeding that of an infrared synchrotron[10]. Additional cascaded second-order nonlinearities in LiNbO$_3$ lead to comb generation with four octaves of simultaneous coverage (0.350 to 5.6 $mu$m). With a comb-tooth linewidth of 10 kHz at 193 THz, we realize a notable spectral resolving power exceeding 10$^{10}$ across 0.86 PHz of bandwidth. We anticipate that this compact and accessible technology will open new opportunities for multi-band precision spectroscopy, coherent microscopy, ultra-high sensitivity nanoscopy, astronomical spectroscopy, and precision carrier-envelope phase (CEP) stable strong field phenomena.



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We present a laser frequency comb based upon a 250 MHz mode-locked erbium-doped fiber laser that spans more than 300 terahertz of bandwidth, from 660 nm to 2000 nm. The system generates 1.2 nJ, 70 fs pulses at 1050 nm by amplifying the 1580 nm laser light in Er:fiber, followed by nonlinear broadening to 1050 nm and amplification in Yb:fiber. Extension of the frequency comb into the visible is achieved by supercontinuum generation from the 1050 nm light. Comb coherence is verified with cascaded f-2f interferometry and comparison to a frequency stabilized laser.
132 - J. Millo , R. Boudot , M. Lours 2009
In this letter, we report on all-optical fiber approach to the generation of ultra-low noise microwave signals. We make use of two erbium fiber mode-locked lasers phase locked to a common ultra-stable laser source to generate an 11.55 GHz signal with an unprecedented relative phase noise of -111 dBc/Hz at 1 Hz from the carrier.The residual frequency instability of the microwave signals derived from the two optical frequency combs is below 2.3 10^(-16) at 1s and about 4 10^(-19) at 6.5 10^(4)s (in 5 Hz bandwidth, three days continuous operation).
Optical frequency combs provide equidistant frequency markers in the infrared, visible and ultra-violet and can link an unknown optical frequency to a radio or microwave frequency reference. Since their inception frequency combs have triggered major advances in optical frequency metrology and precision measurements and in applications such as broadband laser-based gas sensing8 and molecular fingerprinting. Early work generated frequency combs by intra-cavity phase modulation while to date frequency combs are generated utilizing the comb-like mode structure of mode-locked lasers, whose repetition rate and carrier envelope phase can be stabilized. Here, we report an entirely novel approach in which equally spaced frequency markers are generated from a continuous wave (CW) pump laser of a known frequency interacting with the modes of a monolithic high-Q microresonator13 via the Kerr nonlinearity. The intrinsically broadband nature of parametric gain enables the generation of discrete comb modes over a 500 nm wide span (ca. 70 THz) around 1550 nm without relying on any external spectral broadening. Optical-heterodyne-based measurements reveal that cascaded parametric interactions give rise to an optical frequency comb, overcoming passive cavity dispersion. The uniformity of the mode spacing has been verified to within a relative experimental precision of 7.3*10(-18).
While the performance of mode-locked fiber lasers has been improved significantly, the limited gain bandwidth restricts them to generate ultrashort pulses approaching a few cycles or even shorter. Here we present a novel method to achieve few cycle pulses (~5 cycles) with ultra-broad spectrum (~400 nm). To our best knowledge, this is the shortest pulse width and broadest spectrum directly generated from fiber lasers. It is noteworthy that a dramatic ultrashort pulse evolution can be stabilized in a laser oscillator by the unique nonlinear processes of a self-similar evolution as a nonlinear attractor in the gain fiber and a perfect saturable absorber action of the Mamyshev oscillator.
We report an all-polarization-maintaining fiber optic approach to generating sub-2 cycle pulses at 2 {mu}m and a corresponding octave-spanning optical frequency comb. Our configuration leverages mature Er:fiber laser technology at 1.5 {mu}m to provide a seed pulse for a thulium-doped fiber amplifier that outputs 330 mW average power at 100 MHz repetition rate. Following amplification, nonlinear self-compression in fiber decreases the pulse duration to 9.5 fs, or 1.4 optical cycles. Approximately 32 % of the energy sits within the pulse peak, and the polarization extinction ratio is more than 15 dB. The spectrum of the ultrashort pulse spans from 1 {mu}m to beyond 2.4 {mu}m and enables direct measurement of the carrier-envelope offset frequency using only 12 mW, or ~3.5 % of the total power. Our approach employs only commercially-available fiber components, resulting in a turnkey amplifier design that is compact, and easy to reproduce in the larger community. Moreover, the overall design and self-compression mechanism are scalable in repetition rate and power. As such, this system should be useful as a robust frequency comb source in the near-infrared or as a pump source to generate mid-infrared frequency combs.
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