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Register a new userTransition strength measurements to guide magic wavelength selection in optically trapped molecules
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Optical trapping of molecules with long coherence times is crucial for many protocols in quantum information and metrology. However, the factors that limit the lifetimes of the trapped molecules remain elusive and require improved understanding of the underlying molecular structure. Here we show that measurements of vibronic line strengths in weakly and deeply bound $^{88}$Sr$_2$ molecules, combined with textit{ab initio} calculations, allow for unambiguous identification of vibrational quantum numbers. This, in turn, enables the construction of refined excited potential energy curves that inform the selection of magic wavelengths which facilitate long vibrational coherence. We demonstrate Rabi oscillations between far-separated vibrational states that persist for nearly 100 ms.
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We investigate the rovibrational population redistribution of polar molecules in the electronic ground state induced by spontaneous emission and blackbody radiation. As a model system we use optically trapped LiCs molecules formed by photoassociation in an ultracold two-species gas. The population dynamics of vibrational and rotational states is modeled using an ab-initio electric dipole moment function and experimental potential energy curves. Comparison with the evolution of the v=3 electronic ground state yields good qualitative agreement. The analysis provides important input to assess applications of ultracold LiCs molecules in quantum simulation and ultracold chemistry.
The zero crossing of the dynamic differential scalar polarizability of the $S_{1/2}-D_{5/2}$ clock transition in $^{138}$Ba$^+$ has been determined to be $459.1614(28),$THz. Together with previously determined matrix elements and branching ratios, this tightly constrains the dynamic differential scalar polarizability of the clock transition over a large wavelength range ($gtrsim 700,$nm). In particular it allows an estimate of the blackbody radiation shift of the clock transition at room temperature.
Optical clocks benefit from tight atomic confinement enabling extended interrogation times as well as Doppler- and recoil-free operation. However, these benefits come at the cost of frequency shifts that, if not properly controlled, may degrade clock accuracy. Numerous theoretical studies have predicted optical lattice clock frequency shifts that scale nonlinearly with trap depth. To experimentally observe and constrain these shifts in an $^{171}$Yb optical lattice clock, we construct a lattice enhancement cavity that exaggerates the light shifts. We observe an atomic temperature that is proportional to the optical trap depth, fundamentally altering the scaling of trap-induced light shifts and simplifying their parametrization. We identify an operational magic wavelength where frequency shifts are insensitive to changes in trap depth. These measurements and scaling analysis constitute an essential systematic characterization for clock operation at the $10^{-18}$ level and beyond.
D1 magic wavelengths have been predicted for the alkali atoms but are not yet observed to date. We experimentally confirm a D1 magic wavelength that is predicted to lie at 615.87 nm for $^{23}$Na, which we then use to trap and image individual atoms with 80.0(6)% efficiency and without having to modulate the trapping and imaging light intensities. We further demonstrate that the mean loading efficiency remains as high as 74.2(7)% for a 1D array of eight atoms. Leveraging on the absence of trap intensity modulation and lower trap depths afforded by the D1 light, we achieve an order-of-magnitude reduction on the tweezer laser power requirements and a corresponding increase in the scalability of atom arrays. The methods reported here are applicable to all the alkalis, including those that are attractive candidates for dipolar molecule assembly, Rydberg dressing, or are fermionic in nature.
Recent progresses on quantum control of cold atoms and trapped ions in both the scientific and technological aspects greatly advance the applications in precision measurement. Thanks to the exceptional controllability and versatility of these massive quantum systems, unprecedented sensitivity has been achieved in clocks, magnetometers and interferometers based on cold atoms and ions. Besides, these systems also feature many characteristics that can be employed to facilitate the applications in different scenarios. In this review, we briefly introduce the principles of optical clocks, cold atom magnetometers and atom interferometers used for precision measurement of time, magnetic field, and inertial forces. The main content is then devoted to summarize some recent experimental and theoretical progresses in these three applications, with special attention being paid to the new designs and possibilities towards better performance. The purpose of this review is by no means to give a complete overview of all important works in this fast developing field, but to draw a rough sketch about the frontiers and show the fascinating future lying ahead.
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