No Arabic abstract
We characterize the terahertz (THz) generation of N-benzyl-2-methyl-4-nitroaniline (BNA), with crystals ranging in thickness from 123-700 {mu}m. We compare excitation using 800-nm and 1250 to 1500-nm wavelengths. Pumping BNA with 800-nm wavelengths and longer near-infrared wavelengths results in a broad spectrum, producing out to 6 THz using a 100-fs pump, provided the BNA crystal is thin enough. ~200 {mu}m or thinner crystals are required to produce a broad spectrum with an 800-nm pump, whereas ~300 {mu}m thick crystals are optimal for broadband THz generation using the longer wavelengths. We report the favorable THz generation and optical characteristics of our BNA crystals that make them attractive for broadband, high-field THz generation, and we also find significant differences to BNA results reported in other works.
In this work, we demonstrate BNAs high potential for efficient generation of high power THz using ytterbium laser wavelengths. We study the generation theoretically and experimentally using laser wavelength of 960-1150 nm. Broadband pulses of 0-7 THz and high efficiency of 0.6% are demonstrated.
Highly efficient terahertz (THz) wave sources based on difference frequency generation (DFG) process in nonlinear optical crystals play an important role for the applications of THz wave. In order to find more novel nonlinear crystals, here we theoretically investigate the generation of THz wave using the isomorphs of periodically poled $mathrm{KTiOPO_4}$ (PPKTP), including periodically poled RTP, KTA, RTA and CTA. By solving the cascaded difference frequency coupled wave equations, it is found that the intensities of the THz wave generated from the cascaded difference frequency processes are improved by 5.27, 2.87, 2.82, 3.03, and 2.76 times from the non-cascaded cases for KTP, RTP, KTA, RTA and CTA, respectively. The effects of the crystal absorption, the phase mismatch and the pump intensity are also analyzed in detail. This study might help to provide a stronger THz radiation source based on the nonlinear crystals.
We report an experimental demonstration of thermal tuning of resonance frequency in a planar terahertz metamaterial consisting of a gold split-ring resonator array fabricated on a bulk single crystal strontium titanate (SrTiO3) substrate. Cooling the metamaterial starting from 409 K down to 150 K causes about 50% shift in resonance frequency as compare to its room temperature resonance, and there is very little variation in resonance strength. The resonance shift is due to the temperature-dependent refractive index (or the dielectric constant) of the strontium titanate. The experiment opens up avenues for designing tunable terahertz devices by exploiting the temperature sensitive characteristic of high dielectric constant substrates and complex metal oxide materials.
We propose a scheme for efficient cavity-enhanced nonlinear THz generation via difference-frequency generation (DFG) processes using a triply resonant system based on photonic crystal cavities. We show that high nonlinear overlap can be achieved by coupling a THz cavity to a doubly-resonant, dual-polarization near-infrared (e.g. telecom band) photonic-crystal nanobeam cavity, allowing the mixing of three mutually orthogonal fundamental cavity modes through a chi(2) nonlinearity. We demonstrate through coupled-mode theory that complete depletion of the pump frequency - i.e., quantum-limited conversion - is possible in an experimentally feasible geometry, with the operating output power at the point of optimal total conversion efficiency adjustable by varying the mode quality (Q) factors.
The terahertz spectral regime, ranging from about 0.1 to 15 THz, is one of the least explored yet most technologically transformative spectral regions. One current challenge is to develop efficient and compact terahertz emitters/detectors with a broadband and gapless spectrum that can be tailored for various pump photon energies. Here we demonstrate efficient single-cycle broadband THz generation, ranging from about 0.1 to 4 THz, from a thin layer of split-ring resonators with few tens of nanometers thickness by pumping at the telecommunications wavelength of 1.5 micrometer (200 THz). The terahertz emission arises from exciting the magnetic-dipole resonance of the split-ring resonators and quickly decreases under off-resonance pumping. This, together with pump polarization dependence and power scaling of the terahertz emission, identifies the role of optically induced nonlinear currents in split-ring resonators. We also reveal a giant sheet nonlinear susceptibility $sim$10$^{-16}$ m$^2$V$^{-1}$ that far exceeds thin films and bulk non-centrosymmetric materials.