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Register a new userTunable optical nonlinearity for TMD polaritons dressed by a Fermi sea
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We study a system of a transition metal dichalcogenide (TMD) monolayer placed in an optical resonator, where strong light-matter coupling between excitons and photons is achieved. We present quantitative theory of the nonlinear optical response for exciton-polaritons for the case of doped TMD monolayer, and analyze in detail two sources of nonlinearity. The first nonlinear response contribution stems from the Coulomb exchange interaction between excitons. The second contribution comes from the reduction of Rabi splitting that originates from phase space filling at increased exciton concentration and the composite nature of excitons. We demonstrate that both nonlinear contributions are enhanced in the presence of free electrons. As free electron concentration can be routinely controlled by an externally applied gate voltage, this opens a way of electrical tuning of the nonlinear optical response.
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The dynamics of a mobile quantum impurity in a degenerate Fermi system is a fundamental problem in many-body physics. The interest in this field has been renewed due to recent ground-breaking experiments with ultra-cold Fermi gases. Optical creation of an exciton or a polariton in a two-dimensional electron system embedded in a microcavity constitutes a new frontier for this field due to an interplay between cavity-coupling favoring ultra-low mass polariton formation and exciton-electron interactions leading to polaron or trion formation. Here, we present cavity spectroscopy of gate-tunable monolayer MoSe$_2$ exhibiting strongly bound trion and polaron resonances, as well as non-perturbative coupling to a single microcavity mode. As the electron density is increased, the oscillator strength determined from the polariton splitting is gradually transferred from the higher-energy repulsive-exciton-polaron resonance to the lower-energy attractive-polaron manifold. Simultaneous observation of polariton formation in both attractive and repulsive branches indicate a new regime of polaron physics where the polariton impurity mass is much smaller than that of the electrons. Our findings shed new light on optical response of semiconductors in the presence of free carriers by identifying the Fermi polaron nature of excitonic resonances and constitute a first step in investigation of a new class of degenerate Bose-Fermi mixtures.
Second order optical nonlinear processes involve the coherent mixing of two electromagnetic waves to generate a new optical frequency, which plays a central role in a variety of applications, such as ultrafast laser systems, rectifiers, modulators, and optical imaging. However, progress is limited in the mid-infrared (MIR) region due to the lack of suitable nonlinear materials. It is desirable to develop a robust system with a strong, electrically tunable second order optical nonlinearity. Here we demonstrate theoretically that AB-stacked bilayer graphene (BLG) can exhibit a giant and tunable second order nonlinear susceptibility chi ^(2) once an in-plane electric field is applied. chi^(2) can be electrically tuned from 0 to ~ {10^5 pm/V}, three orders of magnitude larger than the widely used nonlinear crystal AgGaSe2. We show that the unusually large chi^(2) arises from two different quantum enhanced two-photon processes thanks to the unique electronic spectrum of BLG. The tunable electronic bandgap of BLG adds additional tunability on the resonance of chi^(2), which corresponds to a tunable wavelength ranging from ~2.6 {mu}m to ~3.1 {mu}m for the up-converted photon. Combined with the high electron mobility and optical transparency of the atomically thin BLG, our scheme suggests a new regime of nonlinear photonics based on BLG.
Neutral particles subject to artificial gauge potentials can behave as charged particles in magnetic fields. This fascinating premise has led to demonstrations of one-way waveguides, topologically protected edge states and Landau levels for photons. In ultracold neutral atoms effective gauge fields have allowed the emulation of matter under strong magnetic fields leading to realization of Harper-Hofstadter and Haldane models. Here we show that application of perpendicular electric and magnetic fields effects a tuneable artificial gauge potential for two-dimensional microcavity exciton polaritons. For verification, we perform interferometric measurement of the associated phase accumulated during coherent polariton transport. Since the gauge potential originates from the magnetoelectric Stark effect, it can be realized for photons strongly coupled to excitations in any polarizable medium. Together with strong polariton- polariton interactions and engineered polariton lattices, artificial gauge fields could play a key role in investigation of non-equilibrium dynamics of strongly correlated photons.
We report Shubnikov-de Haas oscillations measurements revealing experimental signatures of an annular Fermi sea that develops near the energy band edge of the excited subband of two-dimensional holes confined in a wide GaAs quantum well. As we increase the hole density, when the Fermi level reaches the excited subband edge, the low-field magnetoresistance traces show a sudden emergence of new oscillations at an unexpectedly large frequency whose value does $textit{not}$ correspond to the (negligible) density of holes in the excited subband. There is also a sharp and significant increase in zero-field resistance near this onset of subband occupation. Guided by numerical energy dispersion calculations, we associate these observations with the unusual shape of the excited subband dispersion which results in a ring of extrema at finite wavevectors and an annular Fermi sea. Such a dispersion and Fermi sea have long been expected from energy band calculations in systems with strong spin-orbit interaction but their experimental signatures have been elusive.
Achieving efficient nonlinear optical frequency conversion in small volumes is key for future on-chip photonic devices that would provide a higher-speed alternative to modern electronics. However, the already intrinsically low conversion efficiency severely limits miniaturization to nanoscale dimensions. Here we demonstrate that gradient-field effects can provide for an efficient, conventionally dipole-forbidden nonlinear response, offering a new approach for enhanced nonlinear optics in nanostructures. We show that a {em longitudinal} nonlinear source current can dominate the third-order optical nonlinearity of the free electron response in gold in the technologically important near-IR frequency range where the nonlinearities due to other mechanisms are particularly small. Using adiabatic nanofocusing to spatially confine the excitation fields, from measurements of the $2omega_1 - omega_2$ four-wave mixing response as a function of detuning $omega_1 - omega_2$, we find up to $10^{-5}$ conversion efficiency with a gradient field contribution to $chi^{(3)}_{mathrm{Au}}$ of up to $10^{-19}~mathrm{m}^2 / mathrm{V}^2$. The results are in good agreement with theory based on plasma hydrodynamics. Our results demonstrate an increase in nonlinear conversion efficiency with decreasing sample size that can offset and even overcompensate the volume decrease of conventional dipolar pathways. This will enable more efficient nonlinear optical devices and frequency converters and facilitate the extension of coherent multidimensional spectroscopies to the nanoscale.
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