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Register a new userEffect of topology on quasi-particle interactions in the Weyl semimetal WP$_2$
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We compare two crystallographic phases of the low-dimensional WP$_2$ to better understand features of electron-electron and electron-phonon interactions in topological systems. The topological $beta$-phase, a Weyl semimetal with a giant magneto-resistance, shows a larger intensity of electronic Raman scattering compared to the topologically trivial $alpha$-phase. This intensity sharply drops for $T < T^* = 20$ K which evidences a crossover in the topological phase from marginal quasiparticles to a coherent low temperature regime. In contrast, the non-topological $alpha$-phase shows more pronounced signatures of electron-phonon interaction. Here there exist generally enlarged phonon linewidths and deviations from conventional anharmonicity in an intermediate temperature regime. These effects provide evidence for an interesting interplay of electronic correlations and electron-phonon coupling. Both interband and intraband electronic fluctuations are involved in these effects. Their dependence on symmetry as well as momentum conservation are critical ingredients to understand this interplay.
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As conductors in electronic applications shrink, microscopic conduction processes lead to strong deviations from Ohms law. Depending on the length scales of momentum conserving ($l_{MC}$) and relaxing ($l_{MR}$) electron scattering, and the device size ($d$), current flows may shift from ohmic to ballistic to hydrodynamic regimes and more exotic mixtures thereof. So far, an in situ, in-operando methodology to obtain these parameters self-consistently within a micro/nanodevice, and thereby identify its conduction regime, is critically lacking. In this context, we exploit Sondheimer oscillations, semi-classical magnetoresistance oscillations due to helical electronic motion, as a method to obtain $l_{MR}$ in micro-devices even when $l_{MR}gg d$. This gives information on the bulk $l_{MR}$ complementary to quantum oscillations, which are sensitive to all scattering processes. We extract $l_{MR}$ from the Sondheimer amplitude in the topological semi-metal WP$_2$, at elevated temperatures up to $Tsim 50$~K, in a range most relevant for hydrodynamic transport phenomena. Our data on micrometer-sized devices are in excellent agreement with experimental reports of the large bulk $l_{MR}$ and thus confirm that WP$_2$ can be microfabricated without degradation. Indeed, the measured scattering rates match well with those of theoretically predicted electron-phonon scattering, thus supporting the notion of strong momentum exchange between electrons and phonons in WP$_2$ at these temperatures. These results conclusively establish Sondheimer oscillations as a quantitative probe of $l_{MR}$ in micro-devices in studying non-ohmic electron flow.
The non-centrosymmetric Weyl semimetal candidate, MoTe$_2$ was investigated through neutron diffraction and transport measurements at pressures up to 1.5 GPa and at temperatures down to 40 mK. Centrosymmetric and non-centrosymmetric structural phases were found to coexist in the superconducting state. Density Functional Theory (DFT) calculations reveal that the strength of the electron-phonon coupling is similar for both crystal structures. Furthermore, it was found that by controlling non-hydrostatic components of stress, it is possible to mechanically control the ground state crystal structure. This allows for the tuning of crystal symmetry in the superconducting phase from centrosymmetric to non-centrosymmetric. DFT calculations support this strain control of crystal structure. This mechanical control of crystal symmetry gives a route to tuning the band topology of MoTe$_2$ and possibly the topology of the superconducting state.
We systematically measured the Hall effect in the extremely large magnetoresistance semimetal WTe$_2$. By carefully fitting the Hall resistivity to a two-band model, the temperature dependencies of the carrier density and mobility for both electron- and hole-type carriers were determined. We observed a sudden increase of the hole density below $sim$160~K, which is likely associated with the temperature-induced Lifshitz transition reported by a previous photoemission study. In addition, a more pronounced reduction in electron density occurs below 50~K, giving rise to comparable electron and hole densities at low temperature. Our observations indicate a possible electronic structure change below 50~K, which might be the direct driving force of the electron-hole ``compensation and the extremely large magnetoresistance as well. Numerical simulations imply that this material is unlikely to be a perfectly compensated system.
Extremely large magnetoresistance (XMR) was recently discovered in many non-magnetic materials, while its underlying mechanism remains poorly understood due to the complex electronic structure of these materials. Here, we report an investigation of the $alpha$-phase WP$_2$, a topologically trivial semimetal with monoclinic crystal structure (C2/m), which contrasts to the recently discovered robust type-II Weyl semimetal phase in $beta$-WP$_2$. We found that $alpha$-WP$_2$ exhibits almost all the characteristics of XMR materials: the near-quadratic field dependence of MR, a field-induced up-turn in resistivity following by a plateau at low temperature, which can be understood by the compensation effect, and high mobility of carriers confirmed by our Hall effect measurements. It was also found that the normalized MRs under different magnetic fields has the same temperature dependence in $alpha$-WP$_2$, the Kohler scaling law can describe the MR data in a wide temperature range, and there is no obvious change in the anisotropic parameter $gamma$ value with temperature. The resistance polar diagram has a peanut shape when field is rotated in $textit{ac}$ plane, which can be understood by the anisotropy of Fermi surface. These results indicate that both field-induced-gap and temperature-induced Lifshitz transition are not the origin of up-turn in resistivity in the $alpha$-WP$_2$ semimetal. Our findings establish $alpha$-WP$_2$ as a new reference material for exploring the XMR phenomena.
Motivated by the proposal of a Weyl-semimetal phase in pyrochlore iridates, we consider a Hubbard-type model on the pyrochlore lattice. To shed light on the question as to why such a state has not been observed experimentally, its robustness is analyzed. On the one hand, we study the possible phases when the system is doped. Magnetic frustration favors several phases with magnetic and charge order that do not occur at half filling, including additional Weyl-semimetal states close to quarter filling. On the other hand, we search for density waves that break translational symmetry and destroy the Weyl-semimetal phase close to half filling. The uniform Weyl semimetal is found to be stable, which we attribute to the low density of states close to the Fermi energy.
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