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Register a new userEmergence of a nematic paramagnet via quantum order-by-disorder and pseudo-Goldstone modes in Kitaev magnets
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The appearance of nontrivial phases in Kitaev materials exposed to an external magnetic field has recently been a subject of intensive studies. Here, we elucidate the relation between the field-induced ground states of the classical and quantum spin models proposed for such materials, by using the infinite density matrix renormalization group (iDMRG) and the linear spin wave theory (LSWT). We consider the $K Gamma Gamma$ model, where $Gamma$ and $Gamma$ are off-diagonal spin exchanges on top of the dominant Kitaev interaction $K$. Focusing on the magnetic field along the $[111]$ direction, we explain the origin of the nematic paramagnet, which breaks the lattice-rotational symmetry and exists in an extended window of magnetic field, in the quantum model. This phenomenon can be understood as the effect of quantum order-by-disorder in the frustrated ferromagnet with a continuous manifold of degenerate ground states discovered in the corresponding classical model. We compute the dynamical spin structure factors using a matrix operator based time evolution and compare them with the predictions from LSWT. We, thus, provide predictions for future inelastic neutron scattering experiments on Kitaev materials in an external magnetic field along the $[111]$ direction. In particular, the nematic paramagnet exhibits a characteristic pseudo-Goldstone mode which results from the lifting of a continuous degeneracy via quantum fluctuations.
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We identify and discuss the ground state of a quantum magnet on a triangular lattice with bond-dependent Ising-type spin couplings, that is, a triangular analog of the Kitaev honeycomb model. The classical ground-state manifold of the model is spanned by decoupled Ising-type chains, and its accidental degeneracy is due to the frustrated nature of the anisotropic spin couplings. We show how this subextensive degeneracy is lifted by a quantum order-by-disorder mechanism and study the quantum selection of the ground state by treating short-wavelength fluctuations within the linked cluster expansion and by using the complementary spin-wave theory. We find that quantum fluctuations couple next-nearest-neighbor chains through an emergent four-spin interaction, while nearest-neighbor chains remain decoupled. The remaining discrete degeneracy of the ground state is shown to be protected by a hidden symmetry of the model.
We show that the topological Kitaev spin liquid on the honeycomb lattice is extremely fragile against the second-neighbor Kitaev coupling $K_2$, which has recently been shown to be the dominant perturbation away from the nearest-neighbor model in iridate Na$_2$IrO$_3$, and may also play a role in $alpha$-RuCl$_3$ and Li$_2$IrO$_3$. This coupling naturally explains the zigzag ordering (without introducing unrealistically large longer-range Heisenberg exchange terms) and the special entanglement between real and spin space observed recently in Na$_2$IrO$_3$. Moreover, the minimal $K_1$-$K_2$ model that we present here holds the unique property that the classical and quantum phase diagrams and their respective order-by-disorder mechanisms are qualitatively different due to the fundamentally different symmetries of the classical and quantum counterparts.
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We examine the Si(111) multi-valley quantum Hall system and show that it exhibits an exceptionally rich interplay of broken symmetries and quantum Hall ordering already near integer fillings $ u$ in the range $ u=0-6$. This six-valley system has a large $[SU(2)]^3rtimes D_3$ symmetry in the limit where the magnetic length is much larger than the lattice constant. We find that the discrete ${D}_3$ factor breaks over a broad range of fillings at a finite temperature transition to a discrete nematic phase. As $T rightarrow 0$ the $[SU(2)]^3$ continuous symmetry also breaks: completely near $ u =3$, to a residual $[U(1)]^2times SU(2)$ near $ u=2$ and $4$ and to a residual $U(1)times [SU(2)]^2$ near $ u=1$ and $5$. Interestingly, the symmetry breaking near $ u=2,4$ and $ u=3$ involves a combination of selection by thermal fluctuations known as order by disorder and a selection by the energetics of Skyrme lattices induced by moving away from the commensurate fillings, a mechanism we term order by doping. We also exhibit modestly simpler analogs in the four-valley Si(110) system.
In the first part of this paper, we study the spin-S Kitaev model using spin wave theory. We discover a remarkable geometry of the minimum energy surface in the N-spin space. The classical ground states, called Cartesian or CN-ground states, whose number grows exponentially with the number of spins N, form a set of points in the N-spin space. These points are connected by a network of flat valleys in the N-spin space, giving rise to a continuous family of classical ground states. Further, the CN-ground states have a correspondence with dimer coverings and with self avoiding walks on a honeycomb lattice. The zero point energy of our spin wave theory picks out a subset from a continuous family of classically degenerate states as the quantum ground states; the number of these states also grows exponentially with N. In the second part, we present some exact results. For arbitrary spin-S, we show that localized Z_2 flux excitations are present by constructing plaquette operators with eigenvalues pm 1 which commute with the Hamiltonian. This set of commuting plaquette operators leads to an exact vanishing of the spin-spin correlation functions, beyond nearest neighbor separation, found earlier for the spin-1/2 model [G. Baskaran, S. Mandal and R. Shankar, Phys. Rev. Lett. 98, 247201 (2007)]. We introduce a generalized Jordan-Wigner transformation for the case of general spin-S, and find a complete set of commuting link operators, similar to the spin-1/2 model, thereby making the Z_2 gauge structure more manifest. The Jordan-Wigner construction also leads, in a natural fashion, to Majorana fermion operators for half-integer spin cases and hard-core boson operators for integer spin cases, strongly suggesting the presence of Majorana fermion and boson excitations in the respective low energy sectors.
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