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Register a new userRouting of valley photons in a WS2 monolayer via delocalized Bloch modes of in-plane inversion-symmetry broken photonic crystal slabs
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The valleys of two-dimensional transition metal dichalcogenides (TMDCs) offer a new degree of freedom for information processing. To take advantage of this valley degree of freedom, on one hand, it is feasible to control valleys by utilizing different external stimuli like optical and electric fields. On the other hand, nanostructures are also used to separate the valleys by near field coupling. However, for both above methods, either required low-temperature environment or low degree of coherence properties limit their further applications. Here, we demonstrate all-dielectric photonic crystal (PhC) slabs without in-plane inversion symmetry (C2 symmetry) could separate and route valley photons in a WS2 monolayer at room temperature. Coupling with circularly polarized photonic Bloch modes of such PhC slabs, valley photons emitted by a WS2 monolayer are routed directionally and efficiently separated in the far field. In addition, the far-field emission is directionally enhanced and with long-distance spatial coherence property.
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We perform phase-sensitive near-field scanning optical microscopy on photonic-crystal waveguides. The observed intricate field patterns are analyzed by spatial Fourier transformations, revealing several guided TE- and TM-like modes. Using the reconstruction algorithm proposed by Ha, et al. (Opt. Lett. 34 (2009)), we decompose the measured two-dimensional field pattern in a superposition of propagating Bloch modes. This opens new possibilities to study specific modes in near-field measurements. We apply the method to study the transverse behavior of a guided TE-like mode, where the mode extends deeper in the surrounding photonic crystal when the band edge is approached.
Photonic components based on structured metallic elements show great potential for device applications where field enhancement and confinement of the radiation on a subwavelength scale is required. In this paper we report a detailed study of a prototypical metallo-dielectric photonic structure, where features well known in the world of dielectric photonic crystals, like band gaps and defect modes, are exported to the metallic counterpart, with interesting applications to infrared science and technology, as for instance in quantum well infrared photodetectors, narrow-band spectral filters, and tailorable thermal emitters.
The H1 photonic crystal cavity supports two degenerate dipole modes of orthogonal linear polarization which could give rise to circularly polarized fields when driven with a $pi$/$2$ phase difference. However, fabrication errors tend to break the symmetry of the cavity which lifts the degeneracy of the modes, rendering the cavity unsuitable for supporting circular polarization. We demonstrate numerically, a scheme that induces chirality in the cavity modes, thereby achieving a cavity that supports intrinsic circular polarization. By selectively modifying two air holes around the cavity, the dipole modes could interact via asymmetric coherent backscattering which is a non-Hermitian process. With suitable air hole parameters, the cavity modes approach the exceptional point, coalescing in frequencies and linewidths as well as giving rise to significant circular polarization close to unity. The handedness of the chirality can be selected depending on the choice of the modified air holes. Our results highlight the prospect of using the H1 photonic crystal cavity for chiral-light matter coupling in applications such as valleytronics, spin-photon interfaces and the generation of single photons with well-defined spins.
Coherent light-matter interaction can be used to manipulate the energy levels of atoms, molecules and solids. When light with frequency {omega} is detuned away from a resonance {omega}o, repulsion between the photon-dressed (Floquet) states can lead to a shift of energy resonance. The dominant effect is the optical Stark shift (1/({omega}0-{omega})), but there is an additional contribution from the so-called Bloch-Siegert shift (1/({omega}o+{omega})). Although it is common in atoms and molecules, the observation of Bloch-Siegert shift in solids has so far been limited only to artificial atoms since the shifts were small (<1 {mu}eV) and inseparable from the optical Stark shift. Here we observe an exceptionally large Bloch-Siegert shift (~10 meV) in monolayer WS2 under infrared optical driving by virtue of the strong light-matter interaction in this system. Moreover, we can disentangle the Bloch-Siegert shift entirely from the optical Stark shift, because the two effects are found to obey opposite selection rules at different valleys. By controlling the light helicity, we can confine the Bloch-Siegert shift to occur only at one valley, and the optical Stark shift at the other valley. Such a valley-exclusive Bloch-Siegert shift allows for enhanced control over the valleytronic properties in two-dimensional materials, and offers a new avenue to explore quantum optics in solids.
Photonic crystals with a finite size can support surface modes when appropriately terminated. We calculate the dispersion curves of surface modes for different terminations using the plane wave expansion method. These non-radiative surface modes can be excited with the help of attenuated total reflection technique. We did experiments and simulations to trace the surface band curve, both in good agreement with the numerical calculations.
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