No Arabic abstract
Time and frequency transfer lies at the heart of the field of metrology. Compared to current microwave dissemination such as GPS, optical domain dissemination can provide more than one order of magnitude in terms of higher accuracy, which allows for many applications such as the redefinition of the second, tests of general relativity and fundamental quantum physics, precision navigation and quantum communication. Although optical frequency transfer has been demonstrated over thousand kilometers fiber lines, intercontinental time comparison and synchronization still requires satellite free space optical time and frequency transfer. Quite a few pioneering free space optical time and frequency experiments have been implemented at the distance of tens kilometers at ground level. However, there exists no detailed analysis or ground test to prove the feasibility of satellite-based optical time-frequency transfer. Here, we analyze the possibility of this system and then provide the first-step ground test with high channel loss. We demonstrate the optical frequency transfer with an instability of $10^{-18}$ level in 8,000 seconds across a 16-km free space channel with a loss of up to 70~dB, which is comparable with the loss of a satellite-ground link at medium earth orbit (MEO) and geostationary earth orbit (GEO).
High-precision time synchronization for remote clocks plays an important role in fundamental science and real-life applications. However, the current time synchronization techniques have been shown to be vulnerable to sophisticated adversaries. There is a compelling need for fundamentally new methods to distribute high-precision time information securely. Here we propose a satellite-based quantum-secure time transfer (QSTT) scheme based on two-way quantum key distribution (QKD) in free-space, and experimentally verify the key technologies of the scheme via the Micius quantum satellite. In QSTT, a quantum signal (e.g., single photon) is used as the carrier for both the time transfer and the secret-key generation, offering quantum-enhanced security for transferring time signal and time information. We perform a satellite-to-ground time synchronization using single-photon-level signals and achieve a quantum bit error rate of less than 1%, a time data rate of 9 kHz and a time-transfer precision of 30 ps. These results offer possibilities towards an enhanced infrastructure of time-transfer network, whose security stems from quantum physics.
We demonstrate a method that enables accurate timing jitter spectral density characterization of free-running mode-locked laser oscillators over more than 10-decade of Fourier frequency from mHz to tens MHz range. The method is based on analyzing both the input voltage noise to the slave laser and the output voltage noise from the balanced optical cross- correlator (BOC), when two mode-locked lasers are synchronized in repetition rate by the BOC. As a demonstration experiment, timing jitter spectrum of a free-running mode-locked Er-fiber laser with a dynamic range of >340 dB is measured over Fourier frequency ranging from 1 mHz to 38.5 MHz (Nyquist frequency). The demonstrated method can resolve different noise mechanisms that cause specific jitter characteristics in free-running mode-locked laser oscillators for a vast range of time scales from <100-ns to >1000-s.
The propagation distance of a pulsed beam in free space is ultimately limited by diffraction and space-time coupling. Space-time (ST) wave packets are pulsed beams endowed with tight spatio-temporal spectral correlations that render them propagation-invariant. Here we explore the limits of the propagation distance for ST wave packets. Making use of a specially designed phase plate inscribed by gray-scale lithography, we synthesize an ST light sheet of width $approx700$~$mu$m and bandwidth $sim20$~nm and confirm a propagation distance of $approx70$~m.
We present a novel, highly versatile, and self-referenced arrival time monitor for measuring the femtosecond time delay between a hard X-ray pulse from a free-electron laser and an optical laser pulse, measured directly on the same sample used for pump-probe experiments. Two chirped and picosecond long optical supercontinuum pulses traverse the sample with a mutually fixed time delay of 970 fs, while a femtosecond X-ray pulse arrives at an instant in between both pulses. Behind the sample the supercontinuum pulses are temporally overlapped to yield near-perfect destructive interference in the absence of the X-ray pulse. Stimulation of the sample with an X-ray pulse delivers non-zero contributions at certain optical wavelengths, which serve as a measure of the relative arrival time of the X-ray pulse with an accuracy of better than 25 fs. We find an excellent agreement of our monitor with the existing timing diagnostics at the SACLA XFEL with a Pearson correlation value of 0.98. We demonstrate a high sensitivity to measure X-ray pulses with pulse energies as low as 30 $mu$J. Using a free-flowing liquid jet as interaction sample ensures the full replacement of the sample volume for each X-ray/optical event, thus enabling its utility even at MHz repetition rate XFEL sources.
Diffraction-free optical beams propagate freely without change in shape and scale. Monochromatic beams that avoid diffractive spreading require two-dimensional transverse profiles, and there are no corresponding solutions for profiles restricted to one transverse dimension. Here, we demonstrate that the temporal degree of freedom can be exploited to efficiently synthesize one-dimensional pulsed optical sheets that propagate self-similarly in free space. By introducing programmable conical (hyperbolic, parabolic, or elliptical) spectral correlations between the beams spatio-temporal degrees of freedom, a continuum of families of axially invariant pulsed localized beams is generated. The spectral loci of such beams are the reduced-dimensionality trajectories at the intersection of the light-cone with spatio-temporal spectral planes. Far from being exceptional, self-similar axial propagation is a generic feature of fields whose spatial and temporal degrees of freedom are tightly correlated. These one-dimensional `space-time beams can be useful in optical sheet microscopy, nonlinear spectroscopy, and non-contact measurements.