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Register a new userExperimental discovery of bulk-disclination correspondence
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Most natural and artificial materials have crystalline structures from which abundant topological phases emerge [1-6]. The bulk-edge correspondence, widely-adopted in experiments to determine the band topology from edge properties, however, becomes inadequate in discerning various topological crystalline phases [7-17], leading to great challenges in the experimental classification of the large family of topological crystalline materials [4-6]. Theories predict that disclinations, ubiquitous crystallographic defects, provide an effective probe of crystalline topology beyond edges [18-21], which, however, has not yet been confirmed in experiments. Here, we report the experimental discovery of the bulk-disclination correspondence which is manifested as the fractional spectral charge and robust bound states at the disclinations. The fractional disclination charge originates from the symmetry-protected bulk charge patterns---a fundamental property of many topological crystalline insulators (TCIs). Meanwhile, the robust bound states at disclinations emerge as a secondary, but directly observable property of TCIs. Using reconfigurable photonic crystals as photonic TCIs with higher-order topology, we observe those hallmark features via pump-probe and near-field detection measurements. Both the fractional charge and the localized states are demonstrated to emerge at the disclination in the TCI phase but vanish in the trivial phase. The experimental discovery of bulk-disclination correspondence unveils a novel fundamental phenomenon and a new paradigm for exploring topological materials.
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In the past decades, topological concepts have emerged to classify matter states beyond the Ginzburg-Landau symmetry breaking paradigm. The underlying global invariants are usually characterized by integers, such as Chern or winding numbers. Very recently, band topology characterized by non-Abelian topological charges has been proposed, which possess non-commutative and fruitful braiding structures with multiple (>1) bandgaps entangled together. Despite many potential exquisite applications including quantum computations, no experimental observation of non-Abelian topological charges has been reported. Here, we experimentally observe the non-Abelian topological charges in a PT (parity and time-reversal) symmetric system. More importantly, we propose non-Abelian bulk-edge correspondence, where edge states are found to be described by non-Abelian charges. Our work opens the door towards non-Abelian topological phase characterization and manipulation.
Three-dimensional (3D) topological nodal points, such as Weyl and Dirac nodes have attracted wide-spread interest across multiple disciplines and diverse material systems. Unlike nodal points that contain little structural variations, nodal lines can have numerous topological configurations in the momentum space, forming nodal rings, nodal chains and potentially nodal links and nodal knots. However, nodal lines have much less development for the lack of ideal material platforms. In condensed matter for example, nodal lines are often fragile to spin-orbit-coupling, locating off the Fermi level, coexisting with energy-degenerate trivial bands and dispersing strongly in energy of the line degeneracy. Here, overcoming all above difficulties, we theoretically predict and experimentally observe nodal chains in a metallic-mesh photonic crystal having frequency-isolated linear bandtouching rings chained across the entire Brillouin zone (BZ). These nodal chains are protected by mirror symmetries and have a frequency variation less than 1%. We used angle-resolved transmission (ART) to probe the projected bulk dispersions and performed Fourier-transformed field scan (FTFS) to map out the surface dispersions, which is a quadratic touching between two drumhead surface bands. Our results established an ideal nodal-line material for further studies of topological line-degeneracies with nontrivial connectivities, as well as the consequent wave dynamics richer than 2D Dirac and 3D Weyl materials.
Weyl semimetals are a class of materials that can be regarded as three-dimensional analogs of graphene breaking time reversal or inversion symmetry. Electrons in a Weyl semimetal behave as Weyl fermions, which have many exotic properties, such as chiral anomaly and magnetic monopoles in the crystal momentum space. The surface state of a Weyl semimetal displays pairs of entangled Fermi arcs at two opposite surfaces. However, the existence of Weyl semimetals has not yet been proved experimentally. Here we report the experimental realization of a Weyl semimetal in TaAs by observing Fermi arcs formed by its surface states using angle-resolved photoemission spectroscopy. Our first-principles calculations, matching remarkably well with the experimental results, further confirm that TaAs is a Weyl semimetal.
In 1929, Hermann Weyl derived the massless solutions from the Dirac equation - the relativistic wave equation for electrons. Neutrinos were thought, for decades, to be Weyl fermions until the discovery of the neutrino mass. Moreover, it has been suggested that low energy excitations in condensed matter can be the solutions to the Weyl Hamiltonian. Recently, photons have also been proposed to emerge as Weyl particles inside photonic crystals. In all cases, two linear dispersion bands in the three-dimensional (3D) momentum space intersect at a single degenerate point - the Weyl point. Remarkably, these Weyl points are monopoles of Berry flux with topological charges defined by the Chern numbers. These topological invariants enable materials containing Weyl points to exhibit a wide variety of novel phenomena including surface Fermi arcs, chiral anomaly, negative magnetoresistance, nonlocal transport, quantum anomalous Hall effect, unconventional superconductivity[15] and others [16, 17]. Nevertheless, Weyl points are yet to be experimentally observed in nature. In this work, we report on precisely such an observation in an inversion-breaking 3D double-gyroid photonic crystal without breaking time-reversal symmetry.
Topological insulators (TIs) host novel states of quantum matter, distinguished from trivial insulators by the presence of nontrivial conducting boundary states connecting the valence and conduction bulk bands. Up to date, all the TIs discovered experimentally rely on the presence of either time reversal or symmorphic mirror symmetry to protect massless Dirac-like boundary states. Very recently, it has been theoretically proposed that several materials are a new type of TIs protected by nonsymmorphic symmetry, where glide-mirror can protect novel exotic surface fermions with hourglass-shaped dispersion. However, an experimental confirmation of such new nonsymmorphic TI (NSTI) is still missing. Using angle-resolved photoemission spectroscopy, we reveal that such hourglass topology exists on the (010) surface of crystalline KHgSb while the (001) surface has no boundary state, which is fully consistent with first-principles calculations. We thus experimentally demonstrate that KHgSb is a NSTI hosting hourglass fermions. By expanding the classification of topological insulators, this discovery opens a new direction in the research of nonsymmorphic topological properties of materials.
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