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Register a new userMomentum spectroscopy for multiple ionization of cold rubidium in the elliptically polarized laser field
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Employing recent developed magneto-optical trap recoil ion momentum spectroscopy (MOTRIMS) combining cold atom, strong laser pulse, and ultrafast technologies, we study momentum distributions of the multiply ionized cold rubidium (Rb) induced by the elliptically polarized laser pulses (35 fs, $1.3 times 10^{15}$ W/cm$^2$). The complete vector momenta of Rbn+ ions up to charge state n = 4 are recorded with extremely high resolution (0.12 a.u. for Rb$^+$). Variations of characteristic multi-bands displayed in momentum distributions, as the ellipticity varies from the linear to circular polarization, are interpreted qualitatively with the classical over-barrier ionization model. Present momentum spectroscopy of cold heavy alkali atoms presents novel strong-field phenomena beyond the noble gases.
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Based on the strong-field approximation, we obtain analytical expressions for the initial momentum at the tunnel exit and instantaneous ionization rate of tunneling ionization in elliptically polarized laser fields with arbitrary ellipticity. The tunneling electron reveals a nonzero offset of the initial momentum at the tunnel exit in the elliptically polarized laser field. We find that the transverse and longitudinal components of this momentum offset with respect to the instantaneous field direction are directly related to the time derivatives of the instantaneous laser electric field along the angular and radial directions, respectively. We further show that the nonzero initial momentum at the tunnel exit has a significant influence on the laser phase dependence of the instantaneous ionization rate in the nonadiabatic tunneling regime.
We examine correlated electron and doubly charged ion momentum spectra from strong field double ionization of Neon employing intense elliptically polarized laser pulses. An ellipticity-dependent asymmetry of correlated electron and ion momentum distributions has been observed. Using a 3D semiclassical model, we demonstrate that our observations reflect the sub-cycle dynamics of the recollision process. Our work reveals a general physical picture for recollision-impact double ionization with elliptical polarization, and demonstrates the possibility of ultrafast control of the recollision dynamics.
The role of Coulomb focusing in above-threshold ionization in an elliptically polarized mid-infrared strong laser field is investigated within a semiclassical model incorporating tunneling and Coulomb field effects. It is shown that Coulomb focusing up to moderate ellipticity values is dominated by multiple forward scattering of the ionized electron by the atomic core that creates a characteristic low-energy structure in the photoelectron spectrum and is responsible for the peculiar energy scaling of the ionization normalized yield along the major polarization axis. At higher ellipticities, the electron continuum dynamics is disturbed by the Coulomb field effect mostly at the exit of the ionization tunnel. Due to the latter, the normalized yield is found to be enhanced, with the enhancement factor being sharply pronounced at intermediate ellipticities.
We perform high-resolution measurements of momentum distribution on Rb$^{n+}$ recoil ions up to charge state $n=4$, where laser-cooled rubidium atoms are ionized by femtosecond elliptically polarized lasers with the pulse duration of 35 fs and the intensity of 3.3$times$10$^{15}$ W/cm$^2$ in the over-barrier ionization (OBI) regime. The momentum distributions of the recoil ions are found to exhibit multi-band structures as the ellipticity varies from the linear to circular polarizations. The origin of these band structures can be explained quantitatively by the classical OBI model and dedicated classical trajectory Monte Carlo simulations with Heisenberg potential. Specifically, with back analysis of the classical trajectories, we reveal the ionization time and the OBI geometry of the sequentially released electrons, disentangling the mechanisms behind the tilted angle of the band structures. These results indicate that the classical treatment can describe the strong-field multiple ionization processes of alkali atoms.
We explore the influence of elliptical polarization on the (non)sequential two-photon double ionization of atomic helium with ultrashort extreme ultraviolet (XUV) light fields using time-dependent full ab-initio simulations. The energy and angular distributions of photoelectrons are found to be strongly dependent on the ellipticity. The correlation minimum in the joint angular distribution becomes more prominently visible with increasing ellipticity. In a pump-probe sequence of two subsequent XUV pulses with varying ellipticities, polarization tagging allows to discriminate between sequential and nonsequential photoionization. This clear separation demonstrates the potential of elliptically polarized XUV fields for improved control of electronic emission processes.
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