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Register a new userPolarization tagging of two-photon double ionization by elliptically polarized XUVs
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We explore the influence of elliptical polarization on the (non)sequential two-photon double ionization of atomic helium with ultrashort extreme ultraviolet (XUV) light fields using time-dependent full ab-initio simulations. The energy and angular distributions of photoelectrons are found to be strongly dependent on the ellipticity. The correlation minimum in the joint angular distribution becomes more prominently visible with increasing ellipticity. In a pump-probe sequence of two subsequent XUV pulses with varying ellipticities, polarization tagging allows to discriminate between sequential and nonsequential photoionization. This clear separation demonstrates the potential of elliptically polarized XUV fields for improved control of electronic emission processes.
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We examine correlated electron and doubly charged ion momentum spectra from strong field double ionization of Neon employing intense elliptically polarized laser pulses. An ellipticity-dependent asymmetry of correlated electron and ion momentum distributions has been observed. Using a 3D semiclassical model, we demonstrate that our observations reflect the sub-cycle dynamics of the recollision process. Our work reveals a general physical picture for recollision-impact double ionization with elliptical polarization, and demonstrates the possibility of ultrafast control of the recollision dynamics.
We present accurate time-dependent ab initio calculations on fully differential and total integrated (generalized) cross sections for the nonsequential two-photon double ionization of helium at photon energies from 40 to 54 eV. Our computational method is based on the solution of the time-dependent Schroedinger equation and subsequent projection of the wave function onto Coulomb waves. We compare our results with other recent calculations and discuss the emerging similarities and differences. We investigate the role of electronic correlation in the representation of the two-electron continuum states, which are used to extract the ionization yields from the fully correlated final wave function. In addition, we study the influence of the pulse length and shape on the cross sections in time-dependent calculations and address convergence issues.
We report on non-sequential double ionization of Ar by a laser pulse consisting of two counter rotating circularly polarized fields (390 nm and 780 nm). The double ionization probability depends strongly on the relative intensity of the two fields and shows a knee-like structure as function of intensity. We conclude that double ionization is driven by a beam of nearly monoenergetic recolliding electrons, which can be controlled in intensity and energy by the field parameters. The electron momentum distributions show the recolliding electron as well as a second electron which escapes from an intermediate excited state of Ar$^+$.
Based on the strong-field approximation, we obtain analytical expressions for the initial momentum at the tunnel exit and instantaneous ionization rate of tunneling ionization in elliptically polarized laser fields with arbitrary ellipticity. The tunneling electron reveals a nonzero offset of the initial momentum at the tunnel exit in the elliptically polarized laser field. We find that the transverse and longitudinal components of this momentum offset with respect to the instantaneous field direction are directly related to the time derivatives of the instantaneous laser electric field along the angular and radial directions, respectively. We further show that the nonzero initial momentum at the tunnel exit has a significant influence on the laser phase dependence of the instantaneous ionization rate in the nonadiabatic tunneling regime.
We study the higher-harmonic generation (HHG) using elliptically polarized two-color driving fields. The HHG via bi-chromatic counter-rotating laser fields is a promising source of circularly polarized ultrashort XUV radiation at the attosecond time scale. The ellipticity or the polarization of the attosecond pulses can be tweaked by modifying the emitted harmonics ellipticity, which can be controlled by varying the driver fields. We propose a simple setup to control the polarization of the driving fields, which eventually changes the ellipticity of the attosecond pulses. A well-defined scaling law for the ellipticity of the attosecond pulse as a function of the rotation angle of the quarter-wave plate is also deduced by solving the time-dependent Schrodinger equation (TDSE) in two dimensions. The scaling law can further be explored to obtain the attosecond pulses of the desired degree of polarization, ranging from linear to elliptical to circular polarization.
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