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Quantum metamaterials with magnetic response at optical frequencies

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 Added by Rasoul Alaee
 Publication date 2020
  fields Physics
and research's language is English




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We propose novel quantum antennas and metamaterials with strong magnetic response at optical frequencies. Our design is based on the arrangement of natural atoms with only electric dipole transition moments at distances smaller than a wavelength of light but much larger than their physical size. In particular, we show that an atomic dimer can serve as a magnetic antenna at its antisymmetric mode to enhance the decay rate of a magnetic transition in its vicinity by several orders of magnitude. Furthermore, we study metasurfaces composed of atomic bilayers with and without cavities and show that they can fully reflect the electric and magnetic fields of light, thus, forming nearly perfect electric/magnetic mirrors. The proposed quantum metamaterials can be fabricated with available state-of-the-art technologies and promise several applications both in classical optics and quantum engineering.

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We report on the fabrication and mid-infrared transmission properties of free-standing thin metal films, periodically patterned with holes at periods down to 2 microns and area of 3x3 mm2. Square grids were fabricated by electron beam lithography and deep-etching techniques and display substrateless holes, with the metal being supported by a patterned dielectric silicon nitride membrane. The mid-infrared transmission spectra of the substrateless grid display extraordinary transmission peaks and resonant absorption lines with a Q-factor up to 22. These spectral features are due to the interaction of the radiation with surface plasmon modes. The high transmittivity and the negative value of the dielectric constant at selected frequencies make our substrateless structures ideal candidates for the fabrication of mid-infrared metamaterials.
Optical materials with vanishing dielectric permittivity, known as epsilon-near-zero (ENZ) materials, have been shown to possess enhanced nonlinear optical responses in their ENZ region. These strong nonlinear optical properties have been firmly established in homogeneous materials; however, it is as of yet unclear whether metamaterials with effective optical parameters can exhibit a similar enhancement. Here, we probe an optical ENZ metamaterial composed of a subwavelength periodic stack of alternating Ag and SiO$_2$ layers and measure a nonlinear refractive index $n_2 = (1.2 pm 0.1) times 10^{-12}$ m$^2$/W and nonlinear absorption coefficient $beta = (-1.5 pm 0.2) times 10^{-5}$ m/W at its effective zero-permittivity wavelength. The measured $n_2$ is $10^7$ times larger than $n_2$ of fused silica and four times larger than that the $n_2$ of silver. We observe that the nonlinear enhancement in $n_2$ scales as $1/(n_0 mathrm{Re}[n_0])$, where $n_0$ is the linear effective refractive index. As opposed to homogeneous ENZ materials, whose optical properties are dictated by their intrinsic material properties and hence are not widely tunable, the zero-permittivity wavelength of the demonstrated metamaterials may be chosen to lie anywhere within the visible spectrum by selecting the right thicknesses of the sub-wavelength layers. Consequently, our results offer the promise of a means to design metamaterials with large nonlinearities for applications in nanophotonics at any specified optical wavelength.
Arrays of gold split-rings with 50-nm minimum feature size and with an LC resonance at 200-THz frequency (1500-nm wavelength) are fabricated. For normal incidence conditions, they exhibit a pronounced fundamental magnetic mode, arising from a coupling via the electric component of the incident light. For oblique incidence, a coupling via the magnetic component is demonstrated as well. Moreover, we identify a novel higher-order magnetic resonance at around 370 THz (800-nm wavelength) that evolves out of the Mie resonance for oblique incidence. Comparison with theory delivers good agreement and also shows that the structures allow for a negative magnetic permeability.
Using detailed simulations we investigate the magnetic response of metamaterials consisting of pairs of parallel slabs or combinations of slabs with wires (including the fishnet design) as the length-scale of the structures is reduced from mm to nm. We observe the expected saturation of the magnetic resonance frequency when the structure length-scale goes to the sub-micron regime, as well as weakening of the effective permeability resonance and reduction of the spectral width of the negative permeability region. All these results are explained by using an equivalent resistor-inductor-capacitor (RLC) circuit model, taking into account the current-connected kinetic energy of the electrons inside the metallic parts through an equivalent inductance, added to the magnetic field inductance in the unit-cell. Using this model we derive simple optimization rules for achieving optical negative permeability metamaterials of improved performance. Finally, we analyze the magnetic response of the fishnet design and we explain its superior performance regarding the high attainable magnetic resonance frequency, as well as its inferior performance regarding the width of the negative permeability region.
172 - Zheng-Gao Dong , Hui Liu , Tao Li 2008
We demonstrate that left-handed resonance transmission from metallic metamaterial, composed of periodically arranged double rings, can be extended to visible spectrum by introducing an active medium layer as the substrate. The severe ohmic loss inside metals at optical frequencies is compensated by stimulated emission of radiation in this active system. Due to the resonance amplification mechanism of recently proposed lasing spaser, the left-handed transmission band can be restored up to 610 nm wavelength, in dependence on the gain coefficient of the active layer. Additionally, threshold gains for different scaling levels of the double-ring unit are investigated to evaluate the gain requirement of left-handed transmission restoration at different frequency ranges.
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