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Register a new userSpintronic superconductor in a bulk layered material with natural spin-valve structure
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Multi-layered materials provide fascinating platforms to realize various functional properties, possibly leading to future electronic devices controlled by external fields. In particular, layered magnets coupled with conducting layers have been extensively studied recently for possible control of their transport properties via the spin structure. Successful control of quantum-transport properties in the materials with antiferromagnetic (AFM) layers, so-called natural spin-valve structure, has been reported for the Dirac Fermion and topological/axion materials. However, a bulk crystal in which magnetic and superconducting layers are alternately stacked has not been realized until now, and the search for functional properties in it is an interesting yet unexplored field in material science. Here, we discover superconductivity providing such an ideal platform in EuSn2As2 with the van der Waals stacking of magnetic Eu layers and superconducting Sn-As layers, and present the first demonstration of a natural spin-valve effect on the superconducting current. Below the superconducting transition temperature (Tc), the electrical resistivity becomes zero in the in-plane direction. In contrast, it, surprisingly, remains finite down to the lowest temperature in the out-of-plane direction, mostly due to the structure of intrinsic magnetic Josephson junctions in EuSn2As2. The magnetic order of the Eu layers (or natural spin-valve) is observed to be extremely soft, allowing one to easy control of the out-of-plane to in-plane resistivities ratio from 1 to infinity by weak external magnetic fields. The concept of multi-functional materials with stacked magnetic-superconducting layers will open a new pathway to develop novel spintronic devices with magnetically controllable superconductivity.
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Heterostructures consisting of a cuprate superconductor YBa2Cu3O7x and a ruthenate/manganite (SrRuO3/La0.7Sr0.3MnO3) spin valve have been studied by SQUID magnetometry, ferromagnetic resonances and neutron reflectometry. It was shown that due to the influence of magnetic proximity effect a magnetic moment is induced in the superconducting part of heterostructure and at the same time the magnetic moment is suppressed in the ferromagnetic spin valve. The experimental value of magnetization induced in the superconductor has the same order of magnitude with the calculations based on the induced magnetic moment of Cu atoms due to orbital reconstruction at the superconductor-ferromagnetic interface. It corresponds also to the model that takes into account the change in the density of states at a distance of order of the coherence length in the superconductor. The experimentally obtained characteristic length of penetration of the magnetic moment into superconductor exceeds the coherence length for cuprate superconductor. This fact points on the dominance of the mechanism of the induced magnetic moment of Cu atoms due to orbital reconstruction.
Superconductors with persistent zero-resistance currents serve as permanent magnets for high-field applications requiring a strong and stable magnetic field, such as magnetic resonance imaging (MRI). The recent global helium shortage has quickened research into high-temperature superconductors (HTSs) materials that can be used without conventional liquid-helium cooling to 4.2 K. Herein, we demonstrate that 40-K-class metallic HTS magnesium diboride (MgB2) makes an excellent permanent bulk magnet, maintaining 3 T at 20 K for 1 week with an extremely high stability (<0.1 ppm/h). The magnetic field trapped in this magnet is uniformly distributed, as for single-crystalline neodymium-iron-boron. Magnetic hysteresis loop of the MgB2 permanent bulk magnet was detrmined. Because MgB2 is a simple-binary-line compound that does not contain rare-earth metals, polycrystalline bulk material can be industrially fabricated at low cost and with high yield to serve as strong magnets that are compatible with conventional compact cryocoolers, making MgB2 bulks promising for the next generation of Tesla-class permanent-magnet applications.
We have studied the dependence of the superconducting (SC) transition temperature on the mutual orientation of magnetizations of Fe1 and Fe2 layers in the spin valve system CoO_x/Fe1/Cu/Fe2/Pb. We find that this dependence is nonmonotonic when passing from the parallel to the antiparallel case and reveals a distinct minimum near the orthogonal configuration. The analysis of the data in the framework of the SC triplet spin valve theory gives direct evidence for the long-range triplet superconductivity arising due to noncollinearity of the two magnetizations.
Superconducting spin valves based on the superconductor/ferromagnet (S/F) proximity effect are considered to be a key element in the emerging field of superconducting spintronics. Here, we demonstrate the crucial role of the morphology of the superconducting layer in the operation of a multilayer S/F1/F2 spin valve. We study two types of superconducting spin valve heterostructures, with rough and with smooth superconducting layers, using transmission electron microscopy in combination with transport and magnetic characterization. We find that the quality of the S/F interface is not critical for the S/F proximity effect, as regards the suppression of the critical temperature of the S layer. However, it appears to be of paramount importance in the performance of the S/F1/F2 spin valve. As the morphology of the S layer changes from the form of overlapping islands to a smooth case, the magnitude of the conventional superconducting spin valve effect significantly increases. We attribute this dramatic effect to a homogenization of the Green function of the superconducting condensate over the S/F interface in the S/F1/F2 valve with a smooth surface of the S layer.
We investigate heat and charge transport through a diffusive SIF1F2N tunnel junction, where N (S) is a normal (superconducting) electrode, I is an insulator layer and F1,2 are two ferromagnets with arbitrary direction of magnetization. The flow of an electric current in such structures at subgap bias is accompanied by a heat transfer from the normal metal into the superconductor, which enables refrigeration of electrons in the normal metal. We demonstrate that the refrigeration efficiency depends on the strength of the ferromagnetic exchange field h and the angle {alpha} between the magnetizations of the two F layers. As expected, for values of h much larger than the superconducting order parameter Delta, the proximity effect is suppressed and the efficiency of refrigeration increases with respect to a NIS junction. However, for h sim Delta the cooling power (i.e. the heat flow out of the normal metal reservoir) has a non-monotonic behavior as a function of h showing a minimum at h approx Delta. We also determine the dependence of the cooling power on the lengths of the ferromagnetic layers, the bias voltage, the temperature, the transmission of the tunneling barrier and the magnetization misalignment angle {alpha}.
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