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Spin transport in the Quantum Spin Liquid State in the $S=1$ Kitaev model: role of the fractionalized quasiparticles

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 Added by Akihisa Koga
 Publication date 2020
  fields Physics
and research's language is English




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We investigate the real-time spin response of the $S=1$ Kitaev model upon stimuli of a pulsed magnetic field in one of the edges using the exact diagonalization method. It is found that the pulsed magnetic field has no effect on the appearance of the spin moments in the quantum spin liquid region, but induces the spin oscillations in the other edge region with a small magnetic field. This is understood by the existence of the itinerant quasiparticles, which carry the spin excitations without the spin polarization in the quantum spin liquid state. This suggests that the spin fractionalizations occur in the $S=1$ Kitaev model as well as the exactly solvable $S=1/2$ Kitaev one and the fractionalized quasiparticles play an essential role in the spin transport.

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Recent proposals for spin-1 Kitaev materials, such as honeycomb Ni oxides with heavy elements of Bi and Sb, have shown that these compounds naturally give rise to antiferromagnetic (AFM) Kitaev couplings. Conceptual interest in such AFM Kitaev systems has been sparked by the observation of a transition to a gapless $U(1)$ spin liquid at intermediate field strengths in the AFM spin-1/2 Kitaev model. However, all hitherto known spin-1/2 Kitaev materials exhibit ferromagnetic bond-directional exchanges. Here we discuss the physics of the spin-1 Kitaev model in a magnetic field and show, by extensive numerical analysis, that for AFM couplings it exhibits an extended gapless quantum spin liquid at intermediate field strengths. The close analogy to its spin-1/2 counterpart suggests that this gapless spin liquid is a $U(1)$ spin liquid with a neutral Fermi surface, that gives rise to enhanced thermal transport signatures.
We study a quantum spin Kitaev model with zigzag edges to clarify the effects of anisotropy in the exchange couplings on the spin propagation. We simulate the spin and Majorana dynamics triggered by a magnetic pulse, using the real-space time-dependent Majorana mean-field theory. When the anisotropy is small, the dispersion of the itinerant Majorana fermions remains gapless, where the velocity of the spin propagation matches the group velocity of the itinerant Majorana fermions at the nodal points. On the other hand, in the gapped system with a large anisotropy, the spin propagation is strongly suppressed although its nature depends on the shape of the pulse. The spin transport in the junction system described by the Kitaev models with distinct anisotropies is also dressed.
The search for fractionalization in quantum spin liquids largely relies on their decoupling with the environment. However, the spin-lattice interaction is inevitable in a real setting. While the Majorana fermion evades a strong decay due to the gradient form of spin-lattice coupling, the study of the phonon dynamics may serve as an indirect probe of fractionalization of spin degrees of freedom. Here we propose that the signatures of fractionalization can be seen in the sound attenuation and the Hall viscosity. Despite the fact that both quantities can be related to the imaginary part of the phonon self-energy, their origins are quite different, and the time-reversal symmetry breaking is required for the Hall viscosity. First, we compute the sound attenuation due to a phonon scattering off of a pair of Majorana fermions and show that it is linear in temperature ($sim T$). We argue that it has a particular angular dependence providing the information about the spin-lattice coupling and the low-energy Majorana fermion spectrum. The observable effects in the absence of time-reversal symmetry are then analyzed. We obtain the phonon Hall viscosity term from the microscopic Hamiltonian with time-reversal symmetry breaking term. Importantly, the Hall viscosity term mixes the longitudinal and transverse phonon modes and renormalize the spectrum in a unique way, which may be probed in spectroscopy measurement.
Recent experimental evidence for a field-induced quantum spin liquid (QSL) in $alpha$-RuCl$_3$ calls for an understanding for the ground state of honeycomb Kitaev model under a magnetic field. In this work we address the nature of an enigmatic gapless paramagnetic phase in the antiferromagnetic Kitave model, under an intermediate magnetic field perpendicular to the plane. Combining theoretical and numerical efforts, we identify this gapless phase as a $U(1)$ QSL with spinon Fermi surfaces. We also reveal the nature of continuous quantum phase transitions involving this $U(1)$ QSL, and obtain a phase diagram of the Kitaev model as a function of bond anisotropy and perpendicular magnetic field.
The elementary excitations from the conventional magnetic ordered states, such as ferromagnets and antiferromagnets, are magnons. Here, we elaborate a case where the well-defined magnons are absent completely and the spin excitation spectra exhibit an entire continuum in the itinerant edge ferromagnetic state of graphene arising from the flatband edge electronic states. Based on the further studies of the entanglement entropy and finite-size analysis, we show that the continuum other than the Stoner part results from the spin-1/2 spinons deconfined from magnons. The spinon continuum in a magnetically ordered state is ascribed to a ferromagnetic Luttinger liquid in this edge ferromagnet. The investigation is carried out by using the numerical exact diagonalization method with a projection of the interacting Hamiltonian onto the flat band.
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