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Register a new userControllable skyrmion chirality in ferroelectrics
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Chirality, an intrinsic handedness, is one of the most intriguing fundamental phenomena in nature. Materials composed of chiral molecules find broad applications in areas ranging from nonlinear optics and spintronics to biology and pharmaceuticals. However, chirality is usually an invariable inherent property of a given material that cannot be easily changed at will. Here, we demonstrate that ferroelectric nanodots support skyrmions the chirality of which can be controlled and switched. We devise protocols for realizing control and efficient manipulations of the different types of skyrmions. Our findings open the route for controlled chirality with potential applications in ferroelectric-based information technologies.
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Polar skyrmions are theoretically predicted to emerge resulting from the interplay of elastic, electrostatic and gradient energies, in contrast to the key role of the anti-symmetric Dzyalozhinskii-Moriya interaction in magnetic skyrmions. With the discovery of topologically stable polar skyrmions reported by Das et al., (Nature 568, 368, 2019), it is of both fundamental and practical interest to understand the microscopic nature and the possibility of temperature- and strain-driven phase transitions in ensembles of such polar skyrmions. Here, we explore the emergence of a two-dimensional, tetratic lattice of merons (with topological charge of +1/2) from a skyrmion state (topological charge of +1) upon varying the temperature and elastic boundary conditions in [(PbTiO$_3$)$_{16}$/(SrTiO$_3$)$_{16}$]$_8$ lifted-off membranes. Such a topological phase transition is accompanied by a change in chirality, e.g. from left-handed to zero-net chirality, as measured by four-dimensional scanning transmission electron microscopy (4D-STEM). We show how 4D-STEM provides a robust measure of the local polarization simultaneously with the strain state at sub-nm resolution, while directly revealing the origins of chirality in each skyrmion. Using this, we demonstrate strain as a crucial order parameter to drive isotropic-to-anisotropic structural transitions of chiral polar skyrmions to non-chiral merons, validated with X-ray reciprocal space mapping and theoretical phase-field simulations. These results provide the first illustration of systematic control of rich variety of topological dipole textures by altering the mechanical boundary conditions, which may offer a promising way to control their functionalities in ferroelectric nanodevices using the local and spatial distribution of chirality and order for potential applications.
Magnetic skyrmions have been the focus of intense research with promising applications in memory, logic and interconnect technology. Several schemes have been recently proposed and demonstrated to nucleate skyrmions. However, they either result in an uncontrolled skyrmion bubble production or are mostly targeted towards integration with racetrack memory device. In this work, we propose a novel scheme for a controlled single skyrmion nucleation in a confined nanowire geometry with sub-100 nm width using a generalized approach of localized spin current injection technique in material systems exhibiting low Dzyaloshinskii-Moriya interaction (DMI). Our proposed nucleation mechanism follows a pathway involving the creation of a reversed magnetic domain containing one or more pairs of vertical Bloch lines (VBLs) that form an edge-to-edge domain wall as the VBLs get annihilated at the edge of the nanowire. However, pinning of the edge domain walls within a narrow gap using notches or anti-notches results in the creation of a magnetic bubble with defect-free domain wall that eventually relaxes into a circular skyrmion structure. Our simulations predict that the proposed mechanism allows skyrmion nucleation on sub-nanosecond timescale, shows robustness to variations like local pinning sites and is applicable for any skyrmion-based logic, memory and interconnect application.
A magnetic skyrmion is a topological object that can exist as a solitary embedded in the vast ferromagnetic phase, or coexists with a group of its siblings in various stripy phases as well as skyrmion crystals (SkXs). Isolated skyrmions and skyrmions in an SkX are circular while a skyrmion in other phases is a stripe of various forms. Unexpectedly, the sizes of the three different types of skyrmions depend on material parameters differently. For chiral magnetic films with exchange stiffness constant $A$, the Dzyaloshinskii-Moriya interaction (DMI) strength $D$, and perpendicular magnetic anisotropy $K$, $kappaequivpi^2D^2/(16AK)=1$ separates isolated skyrmions from condensed skyrmion states. In contrast to isolated skyrmions whose size increases with $D/K$ and is insensitive to $kappall1$ and stripe skyrmions whose width increases with $A/D$ and is insensitive to $kappagg1$, the size of skyrmions in SkXs is inversely proportional to the square root of skyrmion number density and decreases with $A/D$. This finding has important implications in our search for stable smaller skyrmions at the room temperature in applications.
Skyrmions are nontrivial spiral spin textures considered as potential building blocks for ultrafast and power efficient spintronic memory and logic devices. Controlling their chirality would provide an additional degree of freedom and enable new functionalities in these devices. Achieving such control requires adjusting the interfacial Dzyaloshinskii-Moriya interaction (DMI). Thanks to Brillouin Light scattering measurements in Ta/FeCoB/TaOx trilayer, we have evidenced a DMI sign crossover when tuning TaOx oxidation and suspected another DMI sign crossover when tuning FeCoB thickness. Moreover, using polar magneto-optical Kerr effect microscopy, we demonstrate skyrmion chirality inversion through their opposite current induced motion direction either by changing FeCoB thickness or TaOx oxidation rate. This chirality inversion enables a more versatile manipulation of skyrmions, paving the way towards multidirectional devices.
Paradigmatic knotted solitons, Hopfions, that are characterized by topological Hopf invariant, are widely investigated in the diverse areas ranging from high energy physics, cosmology and astrophysics to biology, magneto- and hydrodynamics and condensed matter physics. Yet, while holding high promise for applications, they remain elusive and under-explored. Here we demonstrate that Hopfions emerge as a basic configuration of polarization field in confined ferroelectric nanoparticles. Our findings establish that Hopfions govern a wealth of novel functionalities in the electromagnetic response of composite nanomaterials opening route to unprecedented technological applications.
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