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Register a new userHopfions emerge in ferroelectrics
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Paradigmatic knotted solitons, Hopfions, that are characterized by topological Hopf invariant, are widely investigated in the diverse areas ranging from high energy physics, cosmology and astrophysics to biology, magneto- and hydrodynamics and condensed matter physics. Yet, while holding high promise for applications, they remain elusive and under-explored. Here we demonstrate that Hopfions emerge as a basic configuration of polarization field in confined ferroelectric nanoparticles. Our findings establish that Hopfions govern a wealth of novel functionalities in the electromagnetic response of composite nanomaterials opening route to unprecedented technological applications.
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Topological solitons have been studied for decades in classical field theories, and have started recently to impact condensed matter physics. Among those solitons, magnetic skyrmions are two-dimensional particle-like objects with a continuous winding of the magnetization, and magnetic Hopfions are three-dimensional topological solitons that can be formed from a closed loop of a twisted skyrmion string. Whereas intense research is underway with magnetic skyrmions towards a fundamental understanding and potential applications in advanced storage and logic devices, the experimental creation and confirmation of magnetic Hopfions has been elusive so far. Theoretical models suggest that Hopfions can be stabilized in frustrated or chiral magnetic systems, and that target skymions can be transformed into Hopfions by adapting their perpendicular magnetic anisotropy. Here, we present experimental evidence of magnetic Hopfions that were created in magnetic Ir/Co/Pt multilayers shaped into nanoscale disks, which are known to host target skyrmions. The three-dimensional spin texture, which distinguishes magnetic Hopfions from target skyrmions was confirmed by combining two advanced element-specific magnetic X-ray microscopy techniques with about 20-30nm lateral resolution, using X-ray magnetic circular dichroism effect as magnetic contrast mechanism in surface-sensitive X-ray photoemission electron microscopy and bulk-sensitive soft x-ray transmission microscopy. We anticipate that these results will stimulate further investigations of Hopfions with different topologies and their potential application in three-dimensional spintronics devices.
Chirality, an intrinsic handedness, is one of the most intriguing fundamental phenomena in nature. Materials composed of chiral molecules find broad applications in areas ranging from nonlinear optics and spintronics to biology and pharmaceuticals. However, chirality is usually an invariable inherent property of a given material that cannot be easily changed at will. Here, we demonstrate that ferroelectric nanodots support skyrmions the chirality of which can be controlled and switched. We devise protocols for realizing control and efficient manipulations of the different types of skyrmions. Our findings open the route for controlled chirality with potential applications in ferroelectric-based information technologies.
Hopfions are an intriguing class of string-like solitons, named according to a classical topological concept classifying three-dimensional direction fields. The search of hopfions in real physical systems is going on for nearly half a century, starting with the seminal work of Faddeev. But so far realizations in solids are missing. Here, we present a theory that identifies magnetic materials featuring hopfions as stable states without the assistance of confinement or external fields. Our results are based on an advanced micromagnetic energy functional derived from a spin-lattice Hamiltonian. Hopfions appear as emergent particles of the classical Heisenberg model. Magnetic hopfions represent three-dimensional particle-like objects of nanometre-size dimensions opening the gate to a new generation of spintronic devices in the framework of a truly three-dimensional architecture. Our approach goes beyond the conventional phenomenological models. We derive material-realistic parameters that serve as concrete guidance in the search of magnetic hopfions bridging computational physics with materials science.
We study the influence of oxygen vacancies on the formation of charged 180$^circ$ domain walls in ferroelectric BaTiO$_3$ using first principles calculations. We show that it is favorable for vacancies to assemble in crystallographic planes, and that such clustering is accompanied by the formation of a charged domain wall. The domain wall has negative bound charge, which compensates the nominal positive charge of the vacancies and leads to a vanishing density of free charge at the wall. This is in contrast to the positively charged domain walls, which are nearly completely compensated by free charge from the bulk. The results thus explain the experimentally observed difference in electronic conductivity of the two types of domain walls, as well as the generic prevalence of charged domain walls in ferroelectrics. Moreover, the explicit demonstration of vacancy driven domain wall formation implies that specific charged domain wall configurations may be realized by bottom-up design for use in domain wall based information processing.
The problem of constructing internally rotating solitons of fixed angular frequency $omega$ in the Faddeev-Skyrme model is reformulated as a variational problem for an energy-like functional, called pseudoenergy, which depends parametrically on $omega$. This problem is solved numerically using a gradient descent method, without imposing any spatial symmetries on the solitons, and the dependence of the solitons energy on $omega$, and on their conserved total isospin $J$, studied. It is found that, generically, the shape of a soliton is independent of $omega$, and that its size grows monotonically with $omega$. A simple elastic rod model of time-dependent hopfions is developed which, despite having only one free parameter, accounts well for most of the numerical results.
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