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Register a new userA numerical ellipsometric analysis (NEA) of nanoscale layered systems
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Added by
Giuseppe Emanuele Lio
Publication date
2019
fields
Physics
and research's language is
English
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A simple and robust method able to predict, with high accuracy, the optical properties of single and multi-layer nanostructures is presented. The method exploits a COMSOL Multiphysics simulation platform and it has been validated by three case studies with increasing numerical complexity: i) a single thin layer (20 nm) of Ag deposited on a glass substrate; ii) a metamaterial composed of five bi-layers of Ag/ITO (Indium Tin Oxide), with a thickness of 20 nm each; iii) a system based on a three-materials unit cell (AZO/ITO/Ag), but without any thickness periodicity (AZO stands for Al$_2$O$_3$/Zinc Oxide). Numerical results have been compared with experimental data provided by real ellipsometric measurements performed on the above mentioned nanostructures ad-hoc fabricated. The obtained agreement is excellent suggesting this research as a valid approach to design materials able to work in a broad spectrum range.
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Nanoscale hydrodynamic instability of ring-like molten rims around ablative microholes produced in nanometer-thick gold films by tightly focused nanosecond-laser pulses was experimentally explored in terms of laser pulse energy and film thickness. These parametric dependencies of basic instability characteristics - order and period of the resulting nanocrowns - were analyzed, revealing its apparently Rayleigh-Plateau character, as compared to much less consistent possible van der Waals and impact origins. Along with fundamental importance, these findings will put forward pulsed laser ablation as an alternative facile inexpensive table-top approach to study such hydrodynamic instabilities developing at nanosecond temporal and nanometer spatial scales.
A method to perform spectrum analysis on low power signals between 0.1 and 10 THz is proposed. It utilizes a nanoscale antiferromagnetic tunnel junction (ATJ) that produces an oscillating tunneling anisotropic magnetoresistance, whose frequency is dependent on the magnitude of an evanescent spin current. It is first shown that the ATJ oscillation frequency can be tuned linearly with time. Then, it is shown that the ATJ output is highly dependent on matching conditions that are highly dependent on the dimensions of the dielectric tunneling barrier. Spectrum analysis can be performed by using an appropriately designed ATJ, whose frequency is driven to increase linearly with time, a low pass filter, and a matched filter. This method of THz spectrum analysis, if realized in experiment, will allow miniaturized electronics to rapidly analyze low power signals with a simple algorithm. It is also found by simulation and analytical theory that for an ATJ with a 0.09 $mu$m$^2$ footprint, spectrum analysis can be performed over a 0.25 THz bandwidth in just 25 ns on signals that are at the Johnson-Nyquist thermal noise floor.
Structured light enables the characterization of chirality of optically small nanoparticles by taking advantage of the helicity maximization concept recently introduced in[1]. By referring to fields with nonzero helicity density as chiral fields, we first investigate the properties of two chiral optical beams in obtaining helicity density localization and maximization requirements. The investigated beams include circularly polarized Gaussian beams and also an optical beam properly composed by a combination of a radially and an azi-muthally polarized beam. To acquire further enhancement and localization of helicity density beyond the diffraction limit, we also study chiral fields at the vicinity of a spherical dielectric nanoantenna and demon-strate that the helicity density around such a nanoantenna is a superposition of helicity density of the illu-minating field, scattered field, and an interference helicity term. Moreover, we illustrate when the nanoan-tenna is illuminated by a proper combination of azimuthal and radially polarized beams, the scattered nearfields satisfy the helicity maximization conditions beyond the diffraction limit. The application of the concept of helicity maximization to nanoantennas and generating optimally chiral nearfield result in helici-ty enhancement which is of great advantage in areas like detection of nanoscale chiral samples, microsco-py, and optical manipulation of chiral nanoparticles.
Color centers in solids are the fundamental constituents of a plethora of applications such as lasers, light emitting diodes and sensors, as well as the foundation of advanced quantum information and communication technologies. Their photoluminescence properties are usually studied under Stokes excitation, in which the emitted photons are at a lower energy than the excitation ones. In this work, we explore the opposite Anti-Stokes process, where excitation is performed with lower energy photons. We report that the process is sufficiently efficient to excite even a single quantum system, namely the germanium-vacancy center in diamond. Consequently, we leverage the temperature-dependent, phonon-assisted mechanism to realize an all-optical nanoscale thermometry scheme that outperforms any homologous optical method employed to date. Our results frame a promising approach for exploring fundamental light-matter interactions in isolated quantum systems, and harness it towards the realization of practical nanoscale thermometry and sensing.
Advances in graphene plasmonics offer numerous opportunities for enabling the design and manufacture of a variety of nanoelectronics and other exciting optical devices. However, due to the limitation of material properties, its operating frequency cannot drop to the microwave range. In this work, a new concept of microwave equivalent graphene based on the ultrathin monolayer plasmonic metasurface is proposed and demonstrated. Based on this concept, elliptical and hyperbolic dispersion can be theoretically obtained by stacking the equivalent graphene metasurfaces periodically. As proofs of the concept and method, an elliptical and an all-metal hyperbolic metamaterial are designed and numerically demonstrated. As a specified realization of the method, a practical hyperbolic metamaterial is fabricated and experimentally investigated with its validity verified by the directional propagation and photonic spin Hall effect. Furthermore, to investigate the validity of the method under extreme parameter conditions, a proof-of-concept hyperlens is designed and fabricated, with its near-field resolution of 0.05$lambda$ experimentally verified. Based on the proposed concept, diverse optical graphene metamaterials such as focusing lens, dispersion-dependent directional couplers, and epsilon-near-zero materials can also be realized in the microwave regime.
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