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Register a new userNon-Divergent Gr{u}neisen Parameter in Quantum Critical Quasicrystal Yb$_{15}$Al$_{34}$Au$_{51}$: Reflection of Robustness of Quantum Criticality under Pressure
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The mechanism of not diverging Gr{u}neisen parameter in the quantum critical heavy-fermion quasicrystal (QC) Yb$_{15}$Al$_{34}$Au$_{51}$ is analyzed. We construct the formalism for calculating the specific heat $C_V(T)$, the thermal-expansion coefficient $alpha(T)$, and the Gr{u}neisen parameter $Gamma(T)$ near the quantum critical point of the Yb valence transition. By applying the framework to the QC, we calculate $C_V(T)$, $alpha(T)$, and $Gamma(T)$, which explains the measurements. Not diverging $Gamma(T)$ is attributed to the robustness of the quantum criticality in the QC under pressure. The difference in $Gamma(T)$ at the lowest temperature between the QC and approximant crystal is shown to reflect the difference in the volume derivative of characteristic energy scales of the critical Yb-valence fluctuation and the Kondo temperature. Possible implications of our theory to future experiments are also discussed.
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Complete expressions of the thermal-expansion coefficient $alpha$ and the Gr{u}neisen parameter $Gamma$ are derived on the basis of the self-consistent renormalization (SCR) theory. By considering zero-point as well as thermal spin fluctuation under the stationary condition, the specific heat for each class of the magnetic quantum critical point (QCP) specified by the dynamical exponent $z=3$ (FM) and $z=2$ (AFM) and the spatial dimension ($d=3$ and $2$) is shown to be expressed as $C_{V}=C_a-C_b$, where $C_a$ is dominant at low temperatures, reproducing the past SCR criticality endorsed by the renormalization group theory. Starting from the explicit form of the entropy and using the Maxwell relation, $alpha=alpha_a+alpha_b$ (with $alpha_a$ and $alpha_b$ being related to $C_a$ and $C_b$, respectively) is derived, which is proven to be equivalent to $alpha$ derived from the free energy. The temperature-dependent coefficient found to exist in $alpha_b$, which is dominant at low temperatures, contributes to the crossover from the quantum-critical regime to the Curie-Weiss regime and even affects the quantum criticality at 2d AFM QCP. Based on these correctly calculated $C_{V}$ and $alpha$, Gr{u}neisen parameter $Gamma=Gamma_a+Gamma_b$ is derived, where $Gamma_a$ and $Gamma_b$ contain $alpha_a$ and $alpha_b$, respectively. The inverse susceptibility coupled to the volume $V$ in $Gamma_b$ gives rise to divergence of $Gamma$ at the QCP for each class even though characteristic energy scale of spin fluctuation $T_0$ is finite at the QCP, which gives a finite contribution in $Gamma_a=-frac{V}{T_0}left(frac{partial T_0}{partial V}right)_{T=0}$. General properties of $alpha$ and $Gamma$ including their signs as well as the relation to $T_0$ and the Kondo temperature in temperature-pressure phase diagrams of Ce- and Yb-based heavy electron systems are discussed.
The elastic property of quantum critical quasicrystal (QC) Yb$_{15}$Al$_{34}$Au$_{51}$ is analyzed theoretically on the basis of the approximant crystal (AC) Yb$_{14}$Al$_{35}$Au$_{51}$. By constructing the realistic effective model in the AC, we evaluate the 4f-5d Coulomb repulsion at Yb as $U_{fd}approx 1.46$ eV realizing the quantum critical point (QCP) of the Yb-valence transition. The RPA analysis of the QCP shows that softening in elastic constants occurs remarkably for bulk modulus and longitudinal mode at low temperatures. Possible relevance of these results to the QC as well as the pressure-tuned AC is discussed.
Using Hartree-Fock-Bogoliubov (HFB) approach we obtained analytical expressions for thermodynamic quantities of the system of triplons in spin gapped quantum magnets such as magnetization, heat capacity and the magnetic Gr{u}neisen parameter $Gamma_H$. Near the critical temperature, $Gamma_H$ is discontinuous and changes its sign upon the Bose-Einstein condensation (BEC) of triplons. On the other hand, in the widely used Hartree-Fock-Popov (HFP) approach there is no discontinuity neither in the heat capacity nor in the Gr{u}neisen parameter. We predict that in the low-temperature limit and near the critical magnetic field $H_c$, $Gamma_H$ diverges as $Gamma_Hsim 1/T^{2}$, while it scales as $Gamma_Hsim 1/(H-H_c)$ as the magnetic field approaches the quantum critical point at $H_c$.
We report on ac magnetic susceptibility measurements under pressure of the Au-Al-Yb alloy, a crystalline approximant to the icosahedral quasicrystal that shows unconventional quantum criticality. In describing the susceptibility as $chi(T)^{-1} - chi(0)^{-1} propto T^{gamma}$, we find that $chi(0)^{-1}$ decreases with increasing pressure and vanishes to zero at the critical pressure $P_{rm c} simeq 2$ GPa, with $gamma~ (simeq 0.5)$ unchanged. We suggest that this quantum criticality emerges owing to critical valence fluctuations. Above $P_{rm c}$, the approximant undergoes a magnetic transition at $T simeq 100$ mK. These results are contrasted with the fact that, in the quasicrystal, the quantum criticality is robust against the application of pressure. The applicability of the so-called $T/H$ scaling to the approximant is also discussed.
Quasicrystals are metallic alloys that possess long-range, aperiodic structures with diffraction symmetries forbidden to conventional crystals. Since the discovery of quasicrystals by Schechtman et al. at 1984 (ref. 1), there has been considerable progress in resolving their geometric structure. For example, it is well known that the golden ratio of mathematics and art occurs over and over again in their crystal structure. However, the characteristic properties of the electronic states - whether they are extended as in periodic crystals or localized as in amorphous materials - are still unresolved. Here we report the first observation of quantum (T = 0) critical phenomena of the Au-Al-Yb quasicrystal - the magnetic susceptibility and the electronic specific heat coefficient arising from strongly correlated 4f electrons of the Yb atoms diverge as T -> 0. Furthermore, we observe that this quantum critical phenomenon is robust against hydrostatic pressure. By contrast, there is no such divergence in a crystalline approximant, a phase whose composition is close to that of the quasicrystal and whose unit cell has atomic decorations (that is, icosahedral clusters of atoms) that look like the quasicrystal. These results clearly indicate that the quantum criticality is associated with the unique electronic state of the quasicrystal, that is, a spatially confined critical state. Finally we discuss the possibility that there is a general law underlying the conventional crystals and the quasicrystals.
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