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Gr{u}neisen parameter of quantum magnets with spin gap

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 Added by Abdulla Rakhimov
 Publication date 2018
  fields Physics
and research's language is English




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Using Hartree-Fock-Bogoliubov (HFB) approach we obtained analytical expressions for thermodynamic quantities of the system of triplons in spin gapped quantum magnets such as magnetization, heat capacity and the magnetic Gr{u}neisen parameter $Gamma_H$. Near the critical temperature, $Gamma_H$ is discontinuous and changes its sign upon the Bose-Einstein condensation (BEC) of triplons. On the other hand, in the widely used Hartree-Fock-Popov (HFP) approach there is no discontinuity neither in the heat capacity nor in the Gr{u}neisen parameter. We predict that in the low-temperature limit and near the critical magnetic field $H_c$, $Gamma_H$ diverges as $Gamma_Hsim 1/T^{2}$, while it scales as $Gamma_Hsim 1/(H-H_c)$ as the magnetic field approaches the quantum critical point at $H_c$.

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In solid state physics, the Gr{u}neisen parameter (GP), originally introduced in the study of the effect of changing the volume of a crystal lattice on its vibrational frequency, has been widely used to investigate the characteristic energy scales of systems with respect to the changes of external potentials. On the other hand, the GP is little investigated in a strongly interacting quantum gas systems. Here we report on our general results on the origin of GP, new identity and caloric effects in quantum gases of ultracold atoms. We prove that the symmetry of the dilute quantum gas systems leads to a simple identity among three different types of GPs, quantifying caloric effect induced respectively by variations of volume, magnetic field and interaction. Using exact Bethe ansatz solutions, we present a rigorous study of these different GPs and the quantum refrigeration in one-dimensional Bose and Femi gases. Based on the exact equations of states of these systems, we obtain analytic results for the singular behaviour of the GPs and the caloric effects at quantum criticality. We also predict the existence of the lowest temperature for cooling near a quantum phase transition. It turns out that the interaction ramp-up and -down in quantum gases provides a promising protocol of quantum refrigeration in addition to the usual adiabatic demagnetization cooling in solid state materials.
Complete expressions of the thermal-expansion coefficient $alpha$ and the Gr{u}neisen parameter $Gamma$ are derived on the basis of the self-consistent renormalization (SCR) theory. By considering zero-point as well as thermal spin fluctuation under the stationary condition, the specific heat for each class of the magnetic quantum critical point (QCP) specified by the dynamical exponent $z=3$ (FM) and $z=2$ (AFM) and the spatial dimension ($d=3$ and $2$) is shown to be expressed as $C_{V}=C_a-C_b$, where $C_a$ is dominant at low temperatures, reproducing the past SCR criticality endorsed by the renormalization group theory. Starting from the explicit form of the entropy and using the Maxwell relation, $alpha=alpha_a+alpha_b$ (with $alpha_a$ and $alpha_b$ being related to $C_a$ and $C_b$, respectively) is derived, which is proven to be equivalent to $alpha$ derived from the free energy. The temperature-dependent coefficient found to exist in $alpha_b$, which is dominant at low temperatures, contributes to the crossover from the quantum-critical regime to the Curie-Weiss regime and even affects the quantum criticality at 2d AFM QCP. Based on these correctly calculated $C_{V}$ and $alpha$, Gr{u}neisen parameter $Gamma=Gamma_a+Gamma_b$ is derived, where $Gamma_a$ and $Gamma_b$ contain $alpha_a$ and $alpha_b$, respectively. The inverse susceptibility coupled to the volume $V$ in $Gamma_b$ gives rise to divergence of $Gamma$ at the QCP for each class even though characteristic energy scale of spin fluctuation $T_0$ is finite at the QCP, which gives a finite contribution in $Gamma_a=-frac{V}{T_0}left(frac{partial T_0}{partial V}right)_{T=0}$. General properties of $alpha$ and $Gamma$ including their signs as well as the relation to $T_0$ and the Kondo temperature in temperature-pressure phase diagrams of Ce- and Yb-based heavy electron systems are discussed.
The mechanism of not diverging Gr{u}neisen parameter in the quantum critical heavy-fermion quasicrystal (QC) Yb$_{15}$Al$_{34}$Au$_{51}$ is analyzed. We construct the formalism for calculating the specific heat $C_V(T)$, the thermal-expansion coefficient $alpha(T)$, and the Gr{u}neisen parameter $Gamma(T)$ near the quantum critical point of the Yb valence transition. By applying the framework to the QC, we calculate $C_V(T)$, $alpha(T)$, and $Gamma(T)$, which explains the measurements. Not diverging $Gamma(T)$ is attributed to the robustness of the quantum criticality in the QC under pressure. The difference in $Gamma(T)$ at the lowest temperature between the QC and approximant crystal is shown to reflect the difference in the volume derivative of characteristic energy scales of the critical Yb-valence fluctuation and the Kondo temperature. Possible implications of our theory to future experiments are also discussed.
We study experimentally the far-from-equilibrium dynamics in ferromagnetic Heisenberg quantum magnets realized with ultracold atoms in an optical lattice. After controlled imprinting of a spin spiral pattern with adjustable wave vector, we measure the decay of the initial spin correlations through single-site resolved detection. On the experimentally accessible timescale of several exchange times we find a profound dependence of the decay rate on the wave vector. In one-dimensional systems we observe diffusion-like spin transport with a dimensionless diffusion coefficient of 0.22(1). We show how this behavior emerges from the microscopic properties of the closed quantum system. In contrast to the one-dimensional case, our transport measurements for two-dimensional Heisenberg systems indicate anomalous super-diffusion.
In the last decade, quantum simulators, and in particular cold atoms in optical lattices, have emerged as a valuable tool to study strongly correlated quantum matter. These experiments are now reaching regimes that are numerically difficult or impossible to access. In particular they have started to fulfill a promise which has contributed significantly to defining and shaping the field of cold atom quantum simulations, namely the exploration of doped and frustrated quantum magnets and the search for the origins of high-temperature superconductivity in the fermionic Hubbard model. Despite many future challenges lying ahead, such as the need to further lower the experimentally accessible temperatures, remarkable studies have already emerged. Among them, spin-charge separation in one-dimensional systems has been demonstrated, extended-range antiferromagnetism in two-dimensional systems has been observed, connections to modern day large-scale numerical simulations were made, and unprecedented comparisons with microscopic trial wavefunctions have been carried out at finite doping. In many regards, the field has acquired new realms, putting old ideas to a new test and producing new insights and inspiration for the next generation of physicists. In the first part of this paper, we review the results achieved in cold atom realizations of the Fermi-Hubbard model in recent years. In the second part of this paper, with the stage set and the current state of the field in mind, we propose a new direction for cold atoms to explore: namely mixed-dimensional bilayer systems, where the charge motion is restricted to individual layers which remain coupled through spin-exchange. We propose a novel, strong pairing mechanism in these systems, which puts the formation of hole pairs at experimentally accessible, elevated temperatures within reach.
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