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Register a new userProton-induced reactions on Fe, Cu, & Ti from threshold to 55 MeV
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Theoretical models often differ significantly from measured data in their predictions of the magnitude of nuclear reactions that produce radionuclides for medical, research, and national security applications. In this paper, we compare a priori predictions from several state-of-the-art reaction modeling packages (CoH, EMPIRE, TALYS, and ALICE) to cross sections measured using the stacked-target activation method. The experiment was performed using the LBNL 88-Inch Cyclotron with beams of 25 and 55 MeV protons on a stack of iron, copper, and titanium foils. 34 excitation functions were measured for 4 < Ep < 55 MeV, including the first measurement of the independent cross sections for natFe(p,x) 49,51Cr, 51,52m,52g,56Mn, and 58m,58gCo. All of the models failed to reproduce the isomer-to-ground state ratio for reaction channels at compound and pre-compound energies, suggesting issues in modeling the deposition or distribution of angular momentum in these residual nuclei.
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Double differential cross sections (DDCS) for light charged particles (proton, deuteron, triton, 3He, alpha) and neutrons produced by a proton beam impinging on a 238U target at 62.9 MeV were measured at the CYCLONE facility in Louvain-la-Neuve (Belgium). These measurements have been performed using two independent experimental set-ups ensuring neutron (DeMoN counters) and light charged particles (Si-Si-CsI telescopes) detection. The charged particle data were measured at 11 different angular positions from 25 degrees to 140 degrees allowing the determination of angle differential, energy differential and total production cross sections.
$^{72}$As is a promising positron emitter for diagnostic imaging that can be employed locally using a $^{72}$Se generator. However, current reaction pathways to $^{72}$Se have insufficient nuclear data for efficient production using regional 100-200 MeV high-intensity proton accelerators. In order to address this deficiency, stacked-target irradiations were performed at LBNL, LANL, and BNL to measure the production of the $^{72}$Se/$^{72}$As PET generator system via $^{75}$As(p,x) between 35 and 200 MeV. This work provides the most well-characterized excitation function for $^{75}$As(p,4n)$^{72}$Se starting from threshold. Additional focus was given to report the first measurements of $^{75}$As(p,x)$^{68}$Ge and bolster an already robust production capability for the highly valuable $^{68}$Ge/$^{68}$Ga PET generator. Thick target yield comparisons with prior established formation routes to both generators are made. In total, high-energy proton-induced cross sections are reported for 55 measured residual products from $^{75}$As, Cu, and Ti targets, where the latter two materials were present as monitor foils. These results were compared with literature data as well as the default theoretical calculations of the nuclear model codes TALYS, CoH, EMPIRE, and ALICE. Reaction modeling at these energies is typically unsatisfactory due to few prior published data and many interacting physics models. Therefore, a detailed assessment of the TALYS code was performed with simultaneous parameter adjustments applied according to a standardized procedure. Particular attention was paid to the formulation of the two-component exciton model in the transition between the compound and pre-equilibrium regions, with a linked investigation of level density models for nuclei off of stability and their impact on modeling predictive power.
Excitation functions for the production of the 181,182m,182g,183,184g,186Re and 183,184Ta radionuclides from proton bombardment on natural tungsten were measured using the stacked-foil activation technique for the proton energies up to 40 MeV. A new data set has been given for the formation of the investigated radionuclides. Results are in good agreement with the earlier reported experimental data and theoretical calculations based on the ALICE-IPPE code. The thick target integral yields were also deduced from the measured excitation functions. The deduced yield values were compared with the directly measured thick target yield (TTY), and found acceptable agreement. The investigated radionuclide 186Re has remarkable applications in the field of nuclear medicine, whereas the data of 183,184gRe and 183Ta have potential applications in thin layer activation analysis and biomedical tracer studies, respectively.
Beam asymmetry and differential cross section for the reaction gamma+p->eta+p were measured from production threshold to 1500 MeV photon laboratory energy. The two dominant neutral decay modes of the eta meson, eta->2g and eta->3pi0, were analyzed. The full set of measurements is in good agreement with previously published results. Our data were compared with three models. They all fit satisfactorily the results but their respective resonance contributions are quite different. The possible photoexcitation of a narrow state N(1670) was investigated and no evidence was found.
Gamma-ray excitation functions have been measured for 30, 42, 54 and 66 MeV proton beams accelerated onto C + O (Mylar), Mg, Si, and Fe targets of astrophysical interest at the separate-sector cyclotron of iThemba LABS in Somerset West (Cape Town, South Africa). A large solid angle, high energy resolution detection system of the Eurogam type was used to record Gamma-ray energy spectra. Derived preliminary results of Gamma-ray line production cross sections for the Mg, Si and Fe target nuclei are reported and discussed. The current cross section data for known, intense Gamma-ray lines from these nuclei consistently extend to higher proton energies previous experimental data measured up to Ep ~ 25 MeV at the Orsay and Washington tandem accelerators. Data for new Gamma-ray lines observed for the first time in this work are also reported.
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