No Arabic abstract
The magneto-optic Voigt effect is observed in a synthetic diamond membrane with a substitutional nitrogen defect concentration in the order of 200 ppm and a nitrogen-vacancy defect sub-ensemble generated through neutron irradiation and annealing. The measured polarisation rotation in the reflected light is observed to be quadratically proportional to the applied magnetic field and to the incident reflection angle. Additionally, it is observed to be modifiable by illuminating the diamond with a 532 nm laser. Spectral analysis of the reflected light under 532 nm illumination shows a slow narrowing of the spectral distribution, indicating a small increase in the overall magnetisation, as opposed to magnetisation degradation caused by heating. Further analysis of the optical power dependence suggest this may be related to a shift in the spin ensembles charge state equilibrium and, by extension, the resulting ensemble magnetisation.
In weakly spin-orbit coupled materials, the spin-selective nature of recombination can give rise to large magnetic-field effects, for example on electro-luminescence from molecular semiconductors. While silicon has weak spin-orbit coupling, observing spin-dependent recombination through magneto-electroluminescence is challenging due to the inefficiency of emission due to silicons indirect band-gap, and to the difficulty in separating spin-dependent phenomena from classical magneto-resistance effects. Here we overcome these challenges to measure magneto-electroluminescence in silicon light-emitting diodes fabricated via gas immersion laser doping. These devices allow us to achieve efficient emission while retaining a well-defined geometry thus suppressing classical magnetoresistance effects to a few percent. We find that electroluminescence can be enhanced by up to 300% near room temperature in a seven Tesla magnetic field showing that the control of the spin degree of freedom can have a strong impact on the efficiency of silicon LEDs.
Large surface plasmon polariton assisted enhancement of the magneto-optical activity has been observed in the past, through spectral measurements of the polar Kerr rotation in Co hexagonal antidot arrays. Here, we report a strong thickness dependence, which is unexpected given that the Kerr effect is considered a surface sensitive phenomena. The maximum Kerr rotation was found to be -0.66 degrees for a 100 nm thick sample. This thickness is far above the typical optical penetration depth of a continuous Co film, demonstrating that in the presence of plasmons the critical lengthscales are dramatically altered, and in this case extended. We therefore establish that the plasmon enhanced Kerr effect does not only depend on the in-plane structuring of the sample, but also on the out-of-plane geometrical parameters, which is an important consideration in magnetoplasmonic device design.
The Landau-Lifshitz-Gilbert (LLG) equation, used to model magneto-dynamics in ferromagnets, tacitly assumes that the angular momentum associated with spin precession can relax instantaneously when the real or effective magnetic field causing the precession is turned off. This neglect of spin inertia is unphysical and would violate energy conservation. Recently, the LLG equation was modified to account for inertia effects. The consensus, however, seems to be that such effects would be unimportant in slow magneto-dynamics that take place over time scales much longer that the relaxation time of the angular momentum, which is typically few fs to perhaps ~100 ps in ferromagnets. Here, we show that there is at least one very serious and observable effect of spin inertia even in slow magneto-dynamics. It involves the switching error probability associated with flipping the magnetization of a nanoscale ferromagnet with an external agent, such as a magnetic field. The switching may take ~ns to complete when the field strength is close to the threshold value for switching, which is much longer than the angular momentum relaxation time, and yet the effect of spin inertia is felt in the switching error probability. This is because the ultimate fate of a switching trajectory, i.e. whether it results in success or failure, is influenced by what happens in the first few ps of the switching action when nutational dynamics due to spin inertia holds sway. Spin inertia increases the error probability, which makes the switching more error-prone. This has vital technological significance because it relates to the reliability of magnetic logic and memory.
We investigated the magnetization dynamics of a patterned Co$_{25}$Fe$_{75}$-based heterostructure with a novel optical measurement technique that we call microfocused frequency-resolved magneto optic Kerr effect ($mu$FR-MOKE). We measured the magnetic field dependence of the dynamical spin-wave susceptibility and recorded a spatial map of the spin-waves excited by a microwave antenna. We compare these results to those obtained on the same sample with the established microfocused Brillouin light scattering technique. With both techniques, we find a spin-wave propagation length of 5.6$mu$m at 10GHz. Furthermore, we measured the dispersion of the wavevector and the spin-wave propagation length as a function of the external magnetic field. These results are in good agreement with existing literature and with the employed Kalinkos-Slavin model.
We report a magnetic field dependence of fluorescence of diamond single crystals containing NV$^-$ centers. In such spectra, numerous sharp lines are found, which correspond to Level Anti-Crossings (LACs) in coupled spins systems comprising an NV$^-$ center. Theoretical modeling of such LAC-spectra enables characterization of paramagnetic defect centers and determination of their magnetic resonance parameters, such as zero-field splitting and hyperfine coupling constants. The outlined method thus enables sensitive detection of paramagnetic impurities in diamond crystals.