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Register a new userHall coefficient diagnostics of surface state in pressurized SmB6
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In this study, we report the first results of the high-pressure Hall coefficient (RH) measurements in the putative topological Kondo insulator SmB6 up to 37 GPa. Below 10 GPa, our data reveal that RH(T) exhibits a prominent peak upon cooling below 20 K. Remarkably, the temperature at which surface conduction dominates coincides with the temperature of the peak in RH(T). The temperature dependent resistance and Hall coefficient can be well fitted by a two-channel model with contributions from the metallic surface and the thermally activated bulk states. When the bulk of SmB6 becomes metallic and magnetic at ~ 10 GPa, both the RH(T) peak and the resistance plateau disappear simultaneously. Our results indicate that the RH(T) peak is a fingerprint to diagnose the presence of a metallic surface state in SmB6. The high-pressure magnetic state of SmB6 is robust to 180 GPa, and no evidence of superconductivity is observed in the metallic phase.
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SmB6 is a mixed valence Kondo insulator that exhibits a sharp increase in resistance following an activated behavior that levels off and saturates below 4K. This behavior can be explained by the proposal of SmB6 representing a new state of matter, a Topological Kondo insulator, in which a Kondo gap is developed and topologically protected surface conduction dominates low-temperature transport. Exploiting its non-linear dynamics, a tunable SmB6 oscillator device was recently demonstrated, where a small DC current generates large oscillating voltages at frequencies from a few Hz to hundreds of MHz. This behavior was explained by a theoretical model describing the thermal and electronic dynamics of coupled surface and bulk states. However, a crucial aspect of this model, the predicted temperature oscillation in the surface state, hasnt been experimentally observed to date. This is largely due to the technical difficulty of detecting an oscillating temperature of the very thin surface state. Here we report direct measurements of the time-dependent surface state temperature in SmB6 with a RuO micro-thermometer. Our results agree quantitatively with the theoretically simulated temperature waveform, and hence support the validity of the oscillator model, which will provide accurate theoretical guidance for developing future SmB6oscillators at higher frequencies.
SmB6 is a promising candidate material that promises to elucidate the connection between strong correlations and topological electronic states, which is a major challenge in condensed matter physics. The electron correlations are responsible for the development of multiple gaps in SmB6, whose elucidation is sorely needed. Here we do so by studying the evolutions of the gaps and other corresponding behaviors under pressure. Our measurements of the valence, Hall effect and electrical resistivity clearly identify the gap which is associated with the bulk Kondo hybridization and, moreover, uncover a pressure-induced quantum phase transition from the putative topological Kondo insulating state to a Fermi-liquid state at ~4 GPa. We provide the evidences for the transition by a jump of inverse Hall coefficient, a diverging tendency of the electron-electron scattering coefficient and, thereby, a destruction of the Kondo entanglement in the ground state. These effects take place in a mixed-valence background. Our results raise the new prospect for studying topological electronic states in quantum critical materials settings.
Strongly correlated Kondo insulator SmB6 is known for its peculiar low temperature residual conduction, which has recently been demonstrated to arise from a robust metallic surface state, as predicted by the theory of topological Kondo insulator (TKI). Photoemission, quantum oscillation and magnetic doping experiments have provided evidence for the Dirac-like dispersion and topological protection. Questions arise as whether signatures of spin-momentum locking and electron interaction could be resolved in transport measurements. Here we report metallic conduction of surface state down to mK temperatures with saturation behaviors suggestive of Kondo effect. We observe in the surface state the weak-antilocalization (WAL) effect that is in agreement with a spin-momentum locked metallic surface. At larger perpendicular magnetic fields, the surface state exhibits an unusual linear magnetoresistance similar to those found in Bi-based topological insulators and in graphene. (Correspondence to: [email protected])
A recently developed formula for the Hall coefficient [A. Auerbach, Phys. Rev. Lett. 121, 66601 (2018)] is applied to nodal line and Weyl semimetals (including graphene), and to spin-orbit split semiconductor bands in two and three dimensions. The calculation reduces to a ratio of two equilibrium susceptibilities, where corrections are negligible at weak disorder. Deviations from Drudes inverse carrier density are associated with band degeneracies, Fermi surface topology, and interband scattering. Experiments which can measure these deviations are proposed.
The proximity effect at the interface between a topological insulator (TI) and a superconductor is predicted to give rise to chiral topological superconductivity and Majorana fermion excitations. In most TIs studied to date, however, the conducting bulk states have overwhelmed the transport properties and precluded the investigation of the interplay of the topological surface state and Cooper pairs. Here, we demonstrate the superconducting proximity effect in the surface state of SmB6 thin films which display bulk insulation at low temperatures. The Fermi velocity in the surface state deduced from the proximity effect is found to be as large as 10^5 m/s, in good agreement with the value obtained from a separate transport measurement. We show that high transparency between the TI and a superconductor is crucial for the proximity effect. The finding here opens the door to investigation of exotic quantum phenomena using all-thin-film multilayers with high-transparency interfaces.
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