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Phase diagram and thermal Hall conductivity of spin-liquid Kekul{e}-Kitaev model

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 Added by Mehdi Kargarian
 Publication date 2019
  fields Physics
and research's language is English




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In this work we study the phase diagram of Kekul{e}-Kitaev model. The model is defined on a honeycomb lattice with bond dependent anisotropic exchange interactions making it exactly solvable in terms of Majorana representation of spins in close analogy to the Kitaev model. However, the energy spectrum of Majorana fermions has a multi-band structure characterized by Chern numbers 0, $pm$1, and $pm2$. We obtained the phase diagram of the model in the plane of exchange couplings and in the presence of a magnetic field and found chiral topological and trivial spin-liquid ground states. In the absence of magnetic field most part of the phase diagram is a trivial gapped phase continuously connected to an Abelian phase, while in the presence of the magnetic field a topological phase arises. Furthermore, motivated by recent thermal measurements on the spin-liquid candidate $alpha$-RuCl$_{3}$, we calculated the thermal Hall conductivity at different regimes of parameters and temperatures and found the latter is quantized over a wide range of temperatures.



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We have measured temperature and magnetic field dependences of the thermal conductivity along the c-axis, kc, and that along the [110] direction, k110, of CuB2O4 single crystals in zero field and magnetic fields along the c-axis and along the [110] direction. It has been found that the thermal conductivity is nearly isotropic and very large in zero field and that the thermal conductivity due to phonons is dominant in CuB2O4. The temperature and field dependences of kc and k110 have markedly changed at phase boundaries in the magnetic phase diagram, which has been understood to be due to the change of the mean free path of phonons caused by the change of the phonon-spin scattering rate at the phase boundaries. It has been concluded that thermal conductivity measurements are very effective for detecting magnetic phase boundaries.
The quantum Hall effect (QHE) in two-dimensional (2D) electron gases, which is one of the most striking phenomena in condensed matter physics, involves the topologically protected dissipationless charge current flow along the edges of the sample. Integer or fractional electrical conductance are measured in units of $e^2/2pihbar$, which is associated with edge currents of electrons or quasiparticles with fractional charges, respectively. Here we discover a novel type of quantization of the Hall effect in an insulating 2D quantum magnet. In $alpha$-RuCl$_3$ with dominant Kitaev interaction on 2D honeycomb lattice, the application of a parallel magnetic field destroys the long-range magnetic order, leading to a field-induced quantum spin liquid (QSL) ground state with massive entanglement of local spins. In the low-temperature regime of the QSL state, we report that the 2D thermal Hall conductance $kappa_{xy}^{2D}$ reaches a quantum plateau as a function of applied magnetic field. $kappa_{xy}^{2D}/T$ attains a quantization value of $(pi/12)(k_B^2/hbar)$, which is exactly half of $kappa_{xy}^{2D}/T$ in the integer QHE. This half-integer thermal Hall conductance observed in a bulk material is a direct signature of topologically protected chiral edge currents of charge neutral Majorana fermions, particles that are their own antiparticles, which possess half degrees of freedom of conventional fermions. These signatures demonstrate the fractionalization of spins into itinerant Majorana fermions and $Z_2$ fluxes predicted in a Kitaev QSL. Above a critical magnetic field, the quantization disappears and $kappa_{xy}^{2D}/T$ goes to zero rapidly, indicating a topological quantum phase transition between the states with and without chiral Majorana edge modes. Emergent Majorana fermions in a quantum magnet are expected to have a major impact on strongly correlated topological quantum matter.
The Kitaev quantum spin liquid displays the fractionalization of quantum spins into Majorana fermions. The emergent Majorana edge current is predicted to manifest itself in the form of a finite thermal Hall effect, a feature commonly discussed in topological superconductors. Here we report on thermal Hall conductivity $kappa_{xy}$ measurements in $alpha$-RuCl$_3$, a candidate Kitaev magnet with the two-dimensional honeycomb lattice. In a spin-liquid (Kitaev paramagnetic) state below the temperature characterized by the Kitaev interaction $J_K/k_B sim 80$ K, positive $kappa_{xy}$ develops gradually upon cooling, demonstrating the presence of highly unusual itinerant excitations. Although the zero-temperature property is masked by the magnetic ordering at $T_N=7$ K, the sign, magnitude, and $T$-dependence of $kappa_{xy}/T$ at intermediate temperatures follows the predicted trend of the itinerant Majorana excitations.
A clear thermal Hall signal ($kappa_{xy}$) was observed in the spin liquid phase of the $S=1/2$ kagome antiferromagnet Ca kapellasite (CaCu$_3$(OH)$_6$Cl$_2cdot 0.6$H$_2$O). We found that $kappa_{xy}$ is well reproduced, both qualitatively and quantitatively, using the Schwinger-boson mean-field theory with the Dzyaloshinskii--Moriya interaction of $D/J sim 0.1$. In particular, $kappa_{xy}$ values of Ca kapellasite and those of another kagome antiferromagnet, volborthite, converge to one single curve in simulations modeled using Schwinger bosons, indicating a common temperature dependence of $kappa_{xy}$ for the spins of a kagome antiferromagnet.
307 - Satoshi Okamoto 2012
The global phase diagram of a doped Kitaev-Heisenberg model is studied using an SU(2) slave-boson mean-field method. Near the Kitaev limit, p-wave superconducting states which break the time-reversal symmetry are stabilized as reported by You {it et al.} [Phys. Rev. B {bf 86}, 085145 (2012)] irrespective of the sign of the Kitaev interaction. By further doping, a d-wave superconducting state appears when the Kitaev interaction is antiferromagnetic, while another p-wave superconducting state appears when the Kitaev interaction is ferromagnetic. This p-wave superconducting state does not break the time-reversal symmetry as reported by Hyart {it et al.} [Phys. Rev. B {bf 85}, 140510 (2012)], and such a superconducting state also appears when the antiferromagnetic Kitaev interaction and the ferromagnetic Heisenberg interaction compete. This work, thus, demonstrates the clear difference between the antiferromagnetic Kitaev model and the ferromagnetic Kitaev model when carriers are doped while these models are equivalent in the undoped limit, and how novel superconducting states emerge when the Kitaev interaction and the Heisenberg interaction compete.
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