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Register a new userEnhanced spin triplet superconductivity due to Kondo destabilization
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In a Kondo lattice system, suppression of effective Kondo coupling leads to the breakdown of the heavy-electron metal and a change in the electronic structure. Spin triplet superconductivity in the Kondo lattice UTe2 appears to be associated with spin fluctuations originating from incipient ferromagnetic order. Here we show clear evidence of twofold enhancement of spin-triplet superconductivity near the pressure-driven suppression of the Kondo coherence, implying that superconductivity is strengthened by the affiliated growth of both spin and charge fluctuations. The coherent Kondo state discontinuously transitions to ferromagnetic order at higher pressures. Application of magnetic field tunes the system back across a first-order phase boundary. Straddling this phase boundary, we find another example of reentrant superconductivity in UTe2. In addition to spin fluctuations associated with ferromagnetism, our results show that a Kondo-driven Fermi surface instability may be playing a role in stabilizing spin triplet superconductivity.
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A spin-triplet superconductor can harbor Majorana bound states that can be used in topological quantum computing. Recently, K2Cr3As3 and its variants with critical temperature Tc as high as 8 K have emerged as a new class of superconductors with ferromagnetic spin fluctuations. Here we report a discovery in K2Cr3As3 single crystal that, the spin susceptibility measured by 75As Knight shift below Tc is unchanged with the magnetic field H0 applied in the ab plane, but vanishes toward zero temperature when H0 is along the c axis, which unambiguously establishes this compound as a spin-triplet superconductor described by a vector order-parameter d parallel to the c axis. Combining with points-nodal gap we show that K2Cr3As3 is a new platform for the study of topological superconductivity and its possible technical application.
We discuss general implications of the local spin-triplet pairing among fermions induced by local ferromagnetic exchange, example of which is the Hunds rule coupling. The quasiparticle energy and their wave function are determined for the three principal phases with the gap, which is momentum independent. We utilize the Bogolyubov-Nambu-De Gennes approach, which in the case of triplet pairing in the two-band case leads to the four-components wave function. Both gapless modes and those with an isotropic gap appear in the quasiparticle spectrum. A striking analogy with the Dirac equation is briefly explored. This type of pairing is relevant to relativistic fermions as well, since it reflects the fundamental discrete symmetry-particle interchange. A comparison with the local interband spin-singlet pairing is also made.
When approaching the atomically thin limit, defects and disorder play an increasingly important role in the properties of two-dimensional materials. Superconductivity is generally thought to be vulnerable to these effects, but here we demonstrate the contrary in the case of oxygenation of ultrathin tantalum disulfide (TaS$_2$). Our first-principles calculations show that incorporation of oxygen into the TaS$_2$ crystal lattice is energetically favourable and effectively heals sulfur vacancies typically present in these crystals, thus restoring the carrier density to the intrinsic value of TaS$_2$. Strikingly, this leads to a strong enhancement of the electron-phonon coupling, by up to 80% in the highly-oxygenated limit. Using transport measurements on fresh and aged (oxygenated) few-layer TaS$_2$, we found a marked increase of the superconducting critical temperature ($T_{mathrm{c}}$) upon aging, in agreement with our theory, while concurrent electron microscopy and electron-energy loss spectroscopy confirmed the presence of sulfur vacancies in freshly prepared TaS$_2$ and incorporation of oxygen into the crystal lattice with time. Our work thus reveals the mechanism by which certain atomic-scale defects can be beneficial to superconductivity and opens a new route to engineer $T_{mathrm{c}}$ in ultrathin materials.
Electrical magnetoresistance and tunnel diode oscillator measurements were performed under external magnetic fields up to 41 T applied along the crystallographic b-axis (hard axis) of UTe$_2$ as a function of temperature and applied pressures up to 18.8 kbar. In this work, we track the field-induced first-order transition between superconducting and magnetic field-polarized phases as a function of applied pressure, showing a suppression of the transition with increasing pressure until the demise of superconductivity near 16 kbar and the appearance of a pressure-induced ferromagnetic-like ground state that is distinct from the field-polarized phase and stable at zero field. Together with evidence for the evolution of a second superconducting phase and its upper critical field with pressure, we examine the confinement of superconductivity by two orthogonal magnetic phases and the implications for understanding the boundaries of triplet superconductivity.
This review presents a summary and evaluations of the superconducting properties of the layered ruthenate Sr2RuO4 as they are known in the autumn of 2011. This paper appends the main progress that has been made since the preceding review by Mackenzie and Maeno was published in 2003. Here, special focus is placed on the critical evaluation of the spin-triplet, odd-parity pairing scenario applied to Sr2RuO4. After an introduction to superconductors with possible odd-parity pairing, accumulated evidence for the pairing symmetry of Sr2RuO4 is examined. Then, significant recent progress on the theoretical approaches to the superconducting pairing by Coulomb repulsion is reviewed. A section is devoted to some experimental properties of Sr2RuO4 that seem to defy simple explanations in terms of currently available spin-triplet scenario. The next section deals with some new developments using eutectic boundaries and micro-crystals, which reveals novel superconducting phenomena related to chiral edge states, odd-frequency pairing states, and half-fluxoid states. Some of these properties are intimately connected with the properties as a topological superconductor. The article concludes with a summary of knowledge emerged from the study of Sr2RuO4 that are now more widely applied to understand the physics of other unconventional superconductors, as well as with a brief discussion of relatively unexplored but promising areas of ongoing and future studies of Sr2RuO4.
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