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Register a new userAbundant quadrupolar or nematic phases driven by the Heisenberg interactions in a spin-1 dimer system forming a bilayer
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We explore several classes of quadrupolar ordering in a system of antiferromagnetically coupled quantum spin-1 dimers, which are stacked in the triangular lattice geometry forming a bilayer. Low-energy properties of this model is described by an $mathcal{S}=1$ hard-core bosonic degrees of freedom defined on each dimer-bond, where the singlet and triplet states of the dimerized spins are interpreted as the vacuum and the occupancy of boson, respectively. The number of bosons per dimer and the magnetic and density fluctuations of bosons are controlled by the inter-dimer Heisenberg interactions. In a solid phase where each dimer hosts one boson and the inter-dimer interaction is weak, a conventional spin nematic phase is realized by the pair-fluctuation of bosons. Larger inter-dimer interaction favors Bose Einstein condensates (BEC) carrying quadrupolar moments. Among them, we find one exotic phase where the quadrupoles develop a spatially modulated structure on the top of a uniform BEC, interpreted in the original dimerized spin-1 model as coexistent $p$-type nematic and 120$^circ$-magnetic correlations. This may explain an intriguing nonmagnetic phase found in Ba$_{3}$ZnRu$_{2}$O$_{9}$.
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We examine the entanglement properties of the spin-half Heisenberg model on the two-dimensional square-lattice bilayer based on quantum Monte Carlo calculations of the second Renyi entanglement entropy. In particular, we extract the dominant area-law contribution to the bipartite entanglement entropy that shows a non-monotonous behavior upon increasing the inter-layer exchange interaction: a local maximum in the area-law coefficient is located at the quantum critical point separating the antiferromagnetically ordered region from the disordered dimer-singlet regime. Furthermore, we consider subleading logarithmic corrections to the Renyi entanglement entropy scaling. Employing different subregion shapes, we isolate the logarithmic corner term from the logarithmic contribution due to Goldstone modes that is found to be enhanced in the limit of decoupled layers. At the quantum critical point, we estimate a contribution of $0.016(1)$ due to each $90^{circ}$ corner. This corner term at the SU(2) quantum critical point deviates from the Gaussian theory value, while it compares well with recent numerical linked cluster calculations on the bilayer model.
It was suggested that the two consecutive metamagnetic transitions and the large residual resistivity discovered in Sr$_3$Ru$_2$O$_7$ can be understood via the nematic order and its domains in a single layer system. However, a recently reported anisotropy between two longitudinal resistivities induced by tilting the magnetic field away from the c-axis cannot be explained within the single layer nematic picture. To fill the gap in our understanding within the nematic order scenario, we investigate the effects of bilayer coupling and in-plane magnetic field on the electronic nematic phases in a bilayer system. We propose that the in-plane magnetic field in the bilayer system modifies the energetics of the domain formation, since it breaks the degeneracy of two different nematic orientations. Thus the system reveals a pure nematic phase with a resistivity anisotropy in the presence of an in-plane magnetic field. In addition to the nematic phase, the bilayer coupling opens a novel route to a hidden nematic phase that preserves the x-y symmetry of the Fermi surfaces.
Frustration in quantum spin systems promote a variety of novel quantum phases. An important example is the frustrated spin-$1$ model on the square lattice with the nearest-neighbor bilinear ($J_1$) and biquadratic ($K_1$) interactions. We provide strong evidence for a nematic spin liquid phase in a range of $K_1/J_1$ near the SU(3)-symmetric point ($J_1 = K_1$), based on the linear flavor-wave theory and extensive density matrix renormalization group calculation. This phase displays no spin dipolar or quadrupolar order, preserves translational symmetry but spontaneously breaks $C_4$ lattice rotational symmetry, and possesses fluctuations peaked at the wavevector $(pi, 2pi/3)$. The spin excitation gap drops rapidly with system size and appears to be gapless, and the nematic order is attributed to the dominant $(pi, 2pi/3)$ fluctuations. Our results provide a novel mechanism for electronic nematic order and, more generally, open up a new avenue to explore frustration-induced exotic ground states.
Neutron diffraction, magnetization, resistivity, and heat capacity measurements on the 6H-perovskite Ba3BiRu2O9 reveal simultaneous magnetic and structural dimerization driven by strong magnetoelastic coupling. An isostructural but strongly displacive first-order transition on cooling through T*=176 K is associated with a change in the nature of direct Ru-Ru bonds within Ru2O9 face-sharing octahedra. Above T*, Ba3BiRu2O9 is an S=1 magnetic dimer system with intradimer exchange interactions J0/kB=320 K and interdimer exchange interactions J/kB=-160 K. Below T*, a spin-gapped state emerges with Deltaapprox220 K. Ab initio calculations confirm antiferromagnetic exchange within dimers, but the transition is not accompanied by long range-magnetic order.
Highly frustrated spin systems such as the kagome lattice (KL) are a treasure trove of new quantum states with large entanglements. We thus study the spin-$frac{1}{2}$ Heisenberg model on a kagome-strip chain (KSC), which is one-dimensional KL, using the density-matrix renormalization group (DMRG) method. Calculating central charge and entanglement spectrum for the KSC, we find a novel gapless spin liquid state with doubly degenerate entanglement spectra in a 1/5 magnetization plateau. We also obtain a gapless low-lying continuum in the dynamic spin structure calculated by dynamical DMRG method. We propose a resonating dimer-monomer liquid state that would meet these features.
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