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Register a new userControlling the Photoelectric Effect in the Time Domain
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When an atom or molecule absorbs a high-energy photon, an electron is emitted with a well-defined energy and a highly-symmetric angular distribution, ruled by energy quantization and parity conservation. These rules seemingly break down when small quantum systems are exposed to short and intense light pulses, which raise the question of their universality for the simplest case of the photoelectric effect. Here we investigate the photoionization of helium by a sequence of attosecond pulses in the presence of a weak infrared dressing field. We continuously control the energy and introduce an asymmetry in the emission direction of the photoelectrons, thus contradicting well established quantum-mechanical predictions. This control is possible due to an extreme temporal confinement of the light-matter interaction. Our work extends time-domain coherent control schemes to one of the fastest processes in nature, the photoelectric effect.
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We explore a counterfactual protocol for energy transfer. A modified version of a Mach-Zehnder interferometer dissociates a photons position and energy into separate channels, resulting in a photoelectric effect in one channel without the absorption of a photon. We use the quantum Zeno effect to extend our results by recycling the same photon through the system and obtain a stream of photoelectrons. If dissociation of properties such as energy can be demonstrated experimentally, there may be a variety of novel energy-related applications that may arise from the capacity to do non-local work. The dissociation of intrinsic properties, like energy, from elementary particles may also lead to theoretical discussions of the constitution of quantum objects.
Ultrafast processes in matter, such as the electron emission following light absorption, can now be studied using ultrashort light pulses of attosecond duration ($10^{-18}$s) in the extreme ultraviolet spectral range. The lack of spectral resolution due to the use of short light pulses may raise serious issues in the interpretation of the experimental results and the comparison with detailed theoretical calculations. Here, we determine photoionization time delays in neon atoms over a 40 eV energy range with an interferometric technique combining high temporal and spectral resolution. We spectrally disentangle direct ionization from ionization with shake up, where a second electron is left in an excited state, thus obtaining excellent agreement with theoretical calculations and thereby solving a puzzle raised by seven-year-old measurements. Our experimental approach does not have conceptual limits, allowing us to foresee, with the help of upcoming laser technology, ultra-high resolution time-frequency studies from the visible to the x-ray range.
We present here an analysis of the sensitivity of a time-domain atomic interferometer to the phase noise of the lasers used to manipulate the atomic wave-packets. The sensitivity function is calculated in the case of a three pulse Mach-Zehnder interferometer, which is the configuration of the two inertial sensors we are building at BNM-SYRTE. We successfully compare this calculation to experimental measurements. The sensitivity of the interferometer is limited by the phase noise of the lasers, as well as by residual vibrations. We evaluate the performance that could be obtained with state of the art quartz oscillators, as well as the impact of the residual phase noise of the phase-lock loop. Requirements on the level of vibrations is derived from the same formalism.
We investigate the effects of static electric and magnetic fields on the differential ac Stark shifts for microwave transitions in ultracold bosonic $^{87}$Rb$^{133}$Cs molecules, for light of wavelength $lambda = 1064~mathrm{nm}$. Near this wavelength we observe unexpected two-photon transitions that may cause trap loss. We measure the ac Stark effect in external magnetic and electric fields, using microwave spectroscopy of the first rotational transition. We quantify the isotropic and anisotropic parts of the molecular polarizability at this wavelength. We demonstrate that a modest electric field can decouple the nuclear spins from the rotational angular momentum, greatly simplifying the ac Stark effect. We use this simplification to control the ac Stark shift using the polarization angle of the trapping laser.
Low-order quantum resonances manifested by directed currents have been realized with cold atoms. Here we show that by increasing the strength of an experimentally achievable delta-kicking ratchet potential, quantum resonances of a very high order may naturally emerge and can induce larger ratchet currents than low-order resonances, with the underlying classical limit being fully chaotic. The results offer a means of controlling quantum transport of cold atoms.
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