No Arabic abstract
Frictional interfaces are abundant in natural and engineering systems, and predicting their behavior still poses challenges of prime scientific and technological importance. At the heart of these challenges lies the inherent coupling between the interfacial constitutive relation -- the macroscopic friction law -- and the bulk elasticity of the bodies that form the frictional interface. In this feature paper, we discuss the generic properties of the macroscopic friction law and the many ways in which its coupling to bulk elasticity gives rise to rich spatiotemporal frictional dynamics. We first present the widely used rate-and-state friction constitutive framework, discuss its power and limitations, and propose extensions that are supported by experimental data. We then discuss how bulk elasticity couples different parts of the interface, and how the range and nature of this interaction are affected by the systems geometry. Finally, in light of the coupling between interfacial and bulk physics, we discuss basic phenomena in spatially-extended frictional systems, including the stability of homogeneous sliding, the onset of sliding motion and a wide variety of propagating frictional modes (e.g. rupture fronts, healing fronts and slip pulses). Overall, the results presented and discussed in this feature paper highlight the inseparable roles played by interfacial and bulk physics in spatially-extended frictional systems.
Recent theories predict that discontinuous shear-thickening (DST) involves an instability, the nature of which remains elusive. Here, we explore unsteady dynamics in a dense cornstarch suspension by coupling long rheological measurements under constant shear stresses to ultrasound imaging. We demonstrate that unsteadiness in DST results from localized bands that travel along the vorticity direction with a specific signature on the global shear rate response. These propagating events coexist with quiescent phases for stresses slightly above DST onset, resulting in intermittent, turbulent-like dynamics. Deeper into DST, events proliferate, leading to simpler, Gaussian dynamics. We interpret our results in terms of unstable vorticity bands as inferred from recent model and numerical simulations.
Predicting when rupture occurs or cracks progress is a major challenge in numerous elds of industrial, societal and geophysical importance. It remains largely unsolved: Stress enhancement at cracks and defects, indeed, makes the macroscale dynamics extremely sensitive to the microscale material disorder. This results in giant statistical uctuations and non-trivial behaviors upon upscaling dicult to assess via the continuum approaches of engineering. These issues are examined here. We will see: How linear elastic fracture mechanics sidetracks the diculty by reducing the problem to that of the propagation of a single crack in an eective material free of defects, How slow cracks sometimes display jerky dynamics, with sudden violent events incompatible with the previous approach, and how some paradigms of statistical physics can explain it, How abnormally fast cracks sometimes emerge due to the formation of microcracks at very small scales.
We derive a connection between the intrinsic tribological properties and the electronic properties of a solid interface. In particular, we show that the adhesion and frictional forces are dictated by the electronic charge redistribution occurring due to the relative displacements of the two surfaces in contact. We define a figure of merit to quantify such charge redistribution and show that simple functional relations hold for a wide series of interactions including metallic, covalent and physical bonds. This suggests unconventional ways of measuring friction by recording the evolution of the interfacial electronic charge during sliding. Finally, we explain that the key mechanism to reduce adhesive friction is to inhibit the charge flow at the interface and provide examples of this mechanism in common lubricant additives.
The nonlinear dynamics associated with sliding friction forms a broad interdisciplinary research field that involves complex dynamical processes and patterns covering a broad range of time and length scales. Progress in experimental techniques and computational resources has stimulated the development of more refined and accurate mathematical and numerical models, capable of capturing many of the essentially nonlinear phenomena involved in friction.
Applications of commodity polymers are often hindered by their low thermal conductivity. In these systems, going from the standard polymers dictated by weak van der Waals interactions to biocompatible hydrogen bonded smart polymers, the thermal transport coefficient k varies between 0.1 - 0.4 W/Km. Combining all-atom molecular dynamics simulations with some experiments, we study thermal transport and its link to the elastic response of commodity plastics. We find that there exists a maximum attainable stiffness (or sound wave velocity), thus providing an upper bound of k for these solid polymers. The specific chemical structure and the glass transition temperature play no role in controlling k, especially when the microscopic interactions are hydrogen bonding based. Our results are consistent with the minimum thermal conductivity model and existing experiments. The effect of polymer stretching on k is also discussed.